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We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

Van der Waals stacking presents new opportunities for nonlinear optics with its remarkable tunability and scalability. However, the fundamental role of interlayer interactions in modifying the overall nonlinear optical susceptibilities…

Materials Science · Physics 2026-03-11 Kanchan Shaikh , Taejun Yoo , Zeyuan Zhu , Qiuyang Li , Amalya C. Johnson , Hui Deng , Fang Liu , Yuki Kobayashi

Crystal symmetry plays a central role in governing a wide range of fundamental physical phenomena. One example is the nonlinear optical second harmonic generation (SHG), which requires inversion symmetry breaking. Here we report a unique…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Yuwei Shan , Yingguo Li , Di Huang , Qingjun Tong , Wang Yao , Wei-Tao Liu , Shiwei Wu

A new High Harmonic Generation (HHG) scheme, which doesn't rely on Tunnel-Ionization as the ionization mechanism but rather on Single-Photon Ionization, is theoretically proposed and numerically demonstrated. The scheme uses two driver…

Atomic Physics · Physics 2022-12-29 Jonathan Berkheim , Eliyahu Bordo , Eldar Ragonis , Lev Merensky , Avner Fleischer

Gallenene is a promising low-dimensional material with a structure down to the thickness of a single atom, similar to graphene. However, van der Waals stacking of two-dimensional (2D) gallenene under confinement remain poorly understood. In…

We propose a novel amplification mechanism for high harmonic generation (HHG) in solids by leveraging bandgap engineering with momentum k-gaps. By constructing a simple diatomic lattice featuring balanced, alternating gain and loss…

Optics · Physics 2025-03-28 Yiming Pan , Danni Chen , Xiaoxi Xu , Zhaopin Chen , Huaiqiang Wang

Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of…

Optics · Physics 2018-01-16 Burak Gerislioglu , Arash Ahmadivand , Nezih Pala

When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a "relativistic oscillating window". The diffracted…

Plasma Physics · Physics 2021-04-07 Longqing Yi

In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

Van der Waals materials enable the construction of atomically sharp interfaces between compounds with distinct crystal and electronic properties. This is dramatically exploited in moir\'e systems, where a lattice mismatch or twist between…

The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Hannah Jürß , Dieter Bauer

Chiral discrimination with high harmonic generation (cHHG method) has been introduced in the recent work by R. Cireasa et al ( Nat. Phys. 11, 654 - 658, 2015). In its original implementation, the cHHG method works by detecting high harmonic…

Optics · Physics 2015-10-28 Olga Smirnova , Yann Mairesse , Serguei Patchkovskii

Phosphorene, a well-studied 2D allotrope of phosphorus, features unique properties such as widely tunable bandgap, high carrier mobility, and remarkable intrinsic in-plane anisotropy. Utilizing these structural and electronic properties, we…

Materials Science · Physics 2024-04-12 Saibabu Madas , Subhendu Kahaly , Mousumi Upadhyay Kahaly

The interaction of light with matter serves as a fundamental tool for probing material properties across a wide range of energy regimes. Recent breakthroughs in tailoring the topology of coherent electromagnetic fields have opened new…

Optics · Physics 2025-03-31 C. Granados , B. Kumar Das , M. F. Ciappina , W. Gao

We report second-harmonic generation (SHG) from thick hexagonal boron nitride (hBN) flakes with approximately 109-111 layers. The resulting effective second-order susceptibility is similar to previously reported few-layer experiments. This…

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…

Titanium diselenide (TiSe$_{2}$) is a transition-metal dichalcogenide material that undergoes a charge-density-wave (CDW) transition at $T_{c}\approx 200\,\mathrm{K}$. In a recent experiment [I. Tyulnev {\it et al.}, Commun. Mater. 6, 152…

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

In this work, the nonlinear optical response, and in particular, the high harmonic generation of semiconductors is addressed by using the Wannier gauge. One of the main problems in the time evolution of the Semiconductor Bloch equations…

Mesoscale and Nanoscale Physics · Physics 2019-11-20 R. E. F. Silva , F. Martín , M. Ivanov

High-quality ultrafast light sources are critical for developing advanced time- and angle-resolved photoemission spectroscopy (TrARPES). While the application of high harmonic generation (HHG) light sources in TrARPES has increased…

Mesoscale and Nanoscale Physics · Physics 2025-10-21 Haoyuan Zhong , Xuanxi Cai , Changhua Bao , Fei Wang , Tianyun Lin , Yudong Chen , Sainan Peng , Lin Tang , Chen Gu , Zhensheng Tao , Hongyun Zhang , Shuyun Zhou
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