Related papers: Combined time and frequency spectroscopy with engi…
Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers…
An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision…
High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…
We present an experimental and theoretical investigation of two-photon direct frequency-comb spectroscopy performed through velocity-selective excitation. In particular, we explore the effect of repetition rate on the…
The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…
A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…
Measurements of ultrahigh-fidelity absorption spectra can help validate quantum theory, engineer ultracold chemistry, and remotely sense atmospheres. Recent achievements in cavity-enhanced spectroscopy using either frequency-based…
We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to…
Multidimensional coherent spectroscopy (MDCS) has been established in quantum chemistry as a powerful tool for studying the nonlinear response and nonequilibrium dynamics of molecular systems. More recently, the technique has also been…
Optical spectroscopy, in particular dual-comb (DC) spectroscopy, is a critical, non-invasive tool for combustion diagnostics, offering high precision and calibration-free advantages. However, its implementation remains challenging,…
Diffuse correlation spectroscopy (DCS) is an emerging noninvasive technique that measures the tissue blood flow, by using near-infrared coherent point-source illumination to detect spectral changes. While machine learning has demonstrated…
We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…
Probing an atomic resonance without disturbing it is an ubiquitous issue in physics. This problem is critical in high-accuracy spectroscopy or for the next generation of atomic optical clocks. Ultra-high resolution frequency metrology…
Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates,…
Compressed sensing (CS) is a powerful method routinely employed to accelerate image acquisition. It is particularly suited to situations when the image under consideration is sparse but can be sampled in a basis where it is non-sparse. Here…
A train of periodic optical pulses gives an optical frequency "comb" that acts as a precise ruler for light measurement due to its equally spaced frequencies. Today, such pulses last millionths of a billionth of a second (Femtoseconds/fs)…
Two-photon resonance transition technology has been proven to have a wide range of applications,it's limited by the available wavelength of commercial lasers.The application of optical comb technology with direct two-photon transition…
Advances in mid-infrared (MIR) dual-comb spectroscopy (DCS) have significantly enhanced molecular detection in recent years. The capability of DCS to precisely identify and quantify atmospheric trace gases makes it attractive for field…
We demonstrate high resolution coherent control of cold atomic Rubidium utilizing spectral phase manipulation of a femtosecond optical frequency comb. Transient coherent accumulation is directly manifested by the enhancement of signal…
We present an innovative frequency comb methodology utilizing pulsed lasers for Rydberg atoms and implement it for electric field measurement. It achieves the Rydberg state population of multi-velocity group atoms through the two-photon…