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Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…

Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is presented as a viable method for fast measurements of molecular spectra. The method is based on the short spatial extension of femtosecond pulses and maps time delays…

Optics · Physics 2009-11-13 Yuri Paskover , I. Sh. Averbukh , Yehiam Prior

Direct frequency-comb spectroscopy is used to probe the absolute frequencies of $6S_{1/2}$-$8S_{1/2}$ two-photon transitions of atomic cesium in hot vapor environment. By utilizing the coherent control method of temporally splitting the…

Atomic Physics · Physics 2018-01-15 Kyung-tae Kim , Jaewook Ahn

Compressive sensing (CS) is a method of sampling which permits some classes of signals to be reconstructed with high accuracy even when they were under-sampled. In this paper we explore a phenomenon in which bandwise CS sampling of a…

Image and Video Processing · Electrical Eng. & Systems 2019-06-28 Henry Kvinge , Elin Farnell , Julia R. Dupuis , Michael Kirby , Chris Peterson , Elizabeth C. Schundler

Nuclear magnetic resonance spectroscopy (MRS) allows for the determination of atomic structures and concentrations of different chemicals in a biochemical sample of interest. MRS is used in vivo clinically to aid in the diagnosis of several…

Medical Physics · Physics 2021-05-04 Zohaib Iqbal , Dan Nguyen , M. Albert Thomas , Steve Jiang

Rotation symmetry of microresonators supports the generation of phase-locked counter-propagating (CP) solitons that can potentially miniaturize dual-comb systems. Realization of these dual-comb compatible solitons in photonic integrated…

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…

One of the essential goals of molecular spectroscopy is to measure all fundamental molecular vibrations simultaneously. To this end, one needs to measure broadband infrared (IR) absorption and Raman scattering spectra, which provide…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

A multispeckle technique for efficiently measuring correctly ensemble-averaged intensity autocorrelation functions of scattered light from non-ergodic and/or non-stationary systems is described. The method employs a CCD camera as a…

Soft Condensed Matter · Physics 2009-11-07 Virgile. Viasnoff , Francois Lequeux , D. J. Pine

The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…

Understanding optical responses of topological matter is a central problem for enabling optoelectronic applications based on topological physics, which is of fundamental concern for photocurrents control and spectroscopy. Currently, schemes…

Other Condensed Matter · Physics 2026-04-24 Osamah Sufyan , Ofer Neufeld

Single-beam spectrally controlled (SBSC) two-dimensional (2D) Raman spectroscopy is a unique 2D vibrational measurement technique utilizing trains of short pulses that are generated from a single broadband pulse by pulse shaping. This…

Chemical Physics · Physics 2021-03-30 Ju-Yeon Jo , Yoshitaka Tanimura

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

We present a detection scheme for diffusing wave spectroscopy (DWS) based on a two cell geometry that allows efficient ensemble averaging. This is achieved by putting a fast rotating diffuser in the optical path between laser and sample. We…

Soft Condensed Matter · Physics 2009-11-11 P. Zakharov , F. Cardinaux , F. Scheffold

Dissipative Kerr solitons (DKSs) intrinsically exhibit two degrees of freedom through their group and phase rotation velocity. Periodic extraction of the DKS into a waveguide produces a pulse train and yields the resulting optical frequency…

Optical frequency combs based on mode-locked lasers have revolutionised the field of metrology and precision spectroscopy by providing precisely calibrated optical frequencies and coherent pulse trains. Amplification of the pulsed output…

Atomic Physics · Physics 2014-01-17 Jonas Morgenweg , Itan Barmes , Kjeld S. E. Eikema

In a recent study [1], we demonstrated a multi-heterodyne differential absorption lidar (DIAL) for greenhouse gas monitoring utilizing solid targets. The multi-frequency absorption measurement was achieved using electro-optic dual-comb…

Optics · Physics 2024-06-27 William Patiño Rosas , Nicolas Cézard

Differential dynamic microscopy (DDM) is increasingly used in the fields of soft matter physics and biophysics to extract the dynamics of microscopic objects across a range of wavevectors using optical microscopy. Standard DDM is limited to…

Soft Condensed Matter · Physics 2021-02-24 Ruilin You , Ryan McGorty

We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser