Related papers: Nanosecond time-resolved dual-comb absorption spec…
We achieve a quantum-noise-limited absorption sensitivity of 1.7/times10$^{-12}$ cm$^{-1}$ per spectral element at 400 s of acquisition time with cavity-enhanced frequency comb spectroscopy, the highest demonstrated for a comb-based…
An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…
Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…
A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…
Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…
A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…
Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…
Frequency combs, specialized laser sources emitting multiple equidistant frequency lines, have revolutionized science and technology with unprecedented precision and versatility. Recently, integrated frequency combs are emerging as scalable…
Coherent laser beams in the 3 to 20 {\mu}m region of the spectrum are most applicable for chemical sensing by addressing the strongest vibrational absorption resonances of the media. Broadband frequency combs in this spectral range are of…
Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…
Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…
Optical frequency combs provide the clockwork to relate optical frequencies to radio frequencies. Hence, combs allow to measure optical frequencies with respect to a radio frequency where the accuracy is limited only by the reference…
Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…
Mid-infrared frequency comb spectroscopy enables measurement of molecular at megahertz spectral resolution, sub-hertz frequency accuracy and microsecond acquisition speed. However, the widespread adoption of this technique has been hindered…
Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…
Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…
Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…
Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…
Frequency combs, broadband light sources whose spectra consist of coherent, discrete modes, have become essential in many fields. Miniaturizing frequency combs would be a significant advance in these fields, enabling the deployment of…
Optical frequency combs have revolutionized the field of frequency metrology within the last decade and have become enabling tools for atomic clocks, gas sensing and astrophysical spectrometer calibration. The rapidly increasing number of…