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Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Strong field ionization of benzene, fluorobenzene, benzonitrile and 1-chloro-2-fluorobenzene, is studied within the framework of real-space and real-time time-dependent density functional theory. Analysis of the ionization rates as function…

Chemical Physics · Physics 2018-11-20 Eldad Yahel , Amir Natan

We analyze atomic photoelectron momentum distributions induced by bichromatic and monochromatic laser fields within the strong field approximation (SFA), separable Coulomb-Volkov approximation (SCVA), and ab initio treatment. We focus on…

Atomic Physics · Physics 2009-06-11 Denys I. Bondar , Michael Spanner , Wing-Ki Liu , Gennady L. Yudin

Here the ionization and high harmonic generation in Hydrogen and Helium by using quantum (hydrodynamic) trajectories is analyzed theoretically. The quantum trajectories allow a self-contained treatment of the electron exchange and…

Atomic Physics · Physics 2025-02-07 Ivan P. Christov

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

High-resolution photoelectron momentum distributions of Xe atoms ionized by 800-nm linearly polarized laser fields have been traced at intensities from 1.1*1013 to 3.5*1013W/cm2 using velocity-map imaging techniques. At certain laser…

Atomic Physics · Physics 2015-12-09 Min Li , Peng Zhang , Siqiang Luo , Yueming Zhou , Qingbin Zhang , Pengfei Lan , Peixiang Lu

The nondipole under-the-barrier dynamics of the electron during strong-field tunneling ionization is investigated, examining the role of the Coulomb field of the atomic core. The common analysis in the strong field approximation is…

Atomic Physics · Physics 2022-04-06 Pei-Lun He , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Relativistic strong-field ionization of hydrogen-like atoms or ions in a constant crossed electromagnetic field is studied. The transition amplitude is formulated within the strong-field approximation in G\"oppert-Mayer gauge, with initial…

Atomic Physics · Physics 2023-03-29 A. Eckey , M. Klaiber , A. B. Voitkiv , C. Müller

Electron-electron correlation effects play an instrumental role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced…

We consider the final stage of multiple ionization of atoms in a strong linearly polarized laser field within a classical model. We propose that non-sequential multiple ionization is dominated by symmetric escape from a highly excited…

Atomic Physics · Physics 2007-05-23 Krzysztof Sacha , Bruno Eckhardt

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct…

A model describing the electronic transitions in an atom subject to a strong high frequency laser pulse is proposed in the velocity gauge. The model accounts for the initial state coupling with the the remaining discrete and continuum…

Atomic Physics · Physics 2016-05-10 V. D. Rodríguez

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We study the real-time evolution of an electron influenced by intense electromagnetic fields using the time-dependent basis light-front quantization (tBLFQ) framework. We focus on demonstrating the non-perturbative feature of the tBLFQ…

Nuclear Theory · Physics 2017-06-07 Guangyao Chen , Xingbo Zhao , Yang Li , Kirill Tuchin , James P. Vary

We measure the dynamics of a non-classical optical field using two-time second-order correlations in conjunction with pulsed excitation. The technique quantifies single-photon purity and coherence during the excitation-decay cycle of an…

Quantum Physics · Physics 2015-05-25 Edward B. Flagg , Sergey V. Polyakov , Tim Thomay , Glenn S. Solomon

Photoelectron momentum distributions (PMDs) from atoms and molecules undergo qualitative changes as laser parameters are varied. We present a model to interpret the shape of the PMDs. The electron's motion is guided by a fictitious particle…

Chaotic Dynamics · Physics 2018-09-19 Jonathan Dubois , Simon Berman , Cristel Chandre , Turgay Uzer

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

Atomic Physics · Physics 2024-12-25 J. Z. Kamiński , K. Krajewska

The interaction of strong pulsed femtosecond laser field with atoms having three equivalent electrons in the outer shell ($p^3$ configuration, e.g. nitrogen) is studied via numerical integration of a time-dependent Schr\"{o}dinger equation…

We present the results of experimental studies of photon-negative ion interactions involving the dynamics of two electrons. Resonances associated with doubly excited states of Li^- and He^- have been observed using laser photodetachment…

Atomic Physics · Physics 2015-06-26 D. Hanstorp , G. Haeffler , A. E. Klinkmueller , U. Ljungblad , U. Berzinsh , I. Yu. Kiyan , D. J. Pegg