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Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and…

Quantum Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Thanh-Tung Nguyen Dang , Eric Charron

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

We discuss the final stages of the simultaneous ionization of two or more electrons due to a strong laser pulse. An analysis of the classical dynamics suggests that the dominant pathway for non-sequential escape has the electrons escaping…

Quantum Physics · Physics 2009-11-06 Bruno Eckhardt , Krzysztof Sacha

With a classical ensemble model that including electron correlations during the whole ionization process, we investigated strong-field sequential double ionization of Ar by elliptically polarized pulses at the quantitative level. The…

Atomic Physics · Physics 2015-06-04 Yueming Zhou , Cheng Huang , Qing Liao , Peixiang Lu

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

We introduce a unified and simplified theory of atomic double ionization. Our results show that at high laser intensities ($I \ge 10^{14}$ watts/cm$^2$) purely classical correlation is strong enough to account for all of the main features…

Atomic Physics · Physics 2007-05-23 Phay J. Ho , R. Panfili , S. L. Haan , J. H. Eberly

We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…

Atomic Physics · Physics 2015-05-28 J. H. Bauer

The total cross section for double ionization of lithiumlike ions by a high-energy photon is calculated in leading order of the nonrelativistic perturbation theory. The partial contributions due to simultaneous and sequential emissions of…

Atomic Physics · Physics 2009-11-11 A. I. Mikhailov , I. A. Mikhailov , A. V. Nefiodov , G. Plunien

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

Atomic Physics · Physics 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

For two-electron diatomic molecules, we investigate magnetic field effects in non-sequential double ionization where recollisions prevail. We do so by formulating a three-dimensional semi-classical model that fully accounts for the Coulomb…

We consider the final stage of triple ionization of atoms in a strong linearly polarized laser field. We propose that for intensities below the saturation value for triple ionization the process is dominated by the simultaneous escape of…

Quantum Physics · Physics 2009-11-07 Krzysztof Sacha , Bruno Eckhardt

We investigate the application of deep learning to the retrieval of the internuclear distance in the two-dimensional H$_2^{+}$ molecule from the momentum distribution of photoelectrons produced by strong-field ionization. We study the…

Atomic Physics · Physics 2023-03-29 N. I. Shvetsov-Shilovski , M. Lein

We build a transient multidimensional multiphysical model based on continuum theories, involving the coupled mechanical, thermal and electrochemical phenomena occurring simultaneously in the discharge or charge of lithium-ion batteries. The…

Numerical Analysis · Mathematics 2024-03-26 Jaime Mora-Paz

In this work we present a new method of approximating the continuum wavefunctions with a discrete basis set. This method aims to be at least compatible with other well known methods of the electronic structure theory to describe processes…

Chemical Physics · Physics 2019-09-18 Mateusz S. Szczygieł , Michał Lesiuk , Robert Moszynski

The evolution of an electron beam colliding head-on with a strong plane-wave field is investigated in the framework of strong-field QED including radiation-reaction effects due to photon emission. Employing a kinetic approach to describe…

High Energy Physics - Phenomenology · Physics 2014-08-07 Norman Neitz , Antonino Di Piazza

A detailed analysis of the process of two photon emission by an electron scattered from a high-intensity laser pulse is presented. The calculations are performed in the framework of strong-field QED and include exactly the presence of the…

High Energy Physics - Phenomenology · Physics 2013-02-13 F. Mackenroth , A. Di Piazza

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao