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Transition metal oxides are considered promising thermoelectric materials for harvesting high-temperature waste heat due to their stability, abundance and low toxicity. Despite their typically strong ionic character, they can exhibit…

Materials Science · Physics 2019-12-04 Simon Thébaud , Christophe Adessi , Georges Bouzerar

A variety of nickel oxide compounds have long been studied for their manifestation of various correlated electron phenomena. Recently, superconductivity was observed in nanoscale infinite layer nickelate thin films of…

The performances of lithium-ion batteries are set by the electrodes materials capacity to exchange lithium ions and electrons faster and reversibly. To this goal Ni-rich layered metal oxides, especially LiNiO2, are attractive electrode…

Using the DFT+dynamical mean-field theory method we revisit the pressure-temperature phase diagram of the prototypical correlated insulator NiO. We study the pressure-induced evolution of the electronic structure, magnetic state, and…

Strongly Correlated Electrons · Physics 2024-12-03 G. M. Gaifutdinov , I. V. Leonov

For decades transition-metal oxides have generated a huge interest due to the multitude of physical phenomena they exhibit. In this class of materials, the rare-earth nickelates, $R$NiO$_3$, stand out for their rich phase diagram stemming…

Strongly Correlated Electrons · Physics 2023-09-18 Luca Binci , Michele Kotiuga , Iurii Timrov , Nicola Marzari

Nickel-based superconductors provide a long-awaited experimental platform to explore possible cuprate-like superconductivity. Despite similar crystal structure and $d$ electron filling, these systems exhibit several differences. Nickelates…

We present a structural and magnetic study on two batches of polycrystalline LiNi$_{0.8}$Mn$_{0.1}$Co$_{0.1}$O$_2$ (commonly known as Li NMC 811), a Ni-rich Li ion battery cathode material, using elemental analysis, X-ray and neutron…

Materials Science · Physics 2021-01-19 P. Mukherjee , J. A. M. Paddison , C. Xu , Z. Ruff , A. R. Wildes , D. A. Keen , R. I. Smith , C. P. Grey , S. E. Dutton

Here we study the transport properties of a nickelate compound, namely LaNiO2 using density functional theory (DFT) in conjunction with dynamical mean field theory (DMFT). An interacting multi-orbital spin-resolved scenario for LaNiO2…

Strongly Correlated Electrons · Physics 2021-10-04 Mijanur Islam , Sudipta Koley , Saurabh Basu

A new superstructure of layered pristine LiNiO2 (LNO) was obtained optimizing a large supercell of the 166 space group, the one observed experimentally by XRD, and relaxing both cell parameters and internal positions. The crystal structure…

Materials Science · Physics 2023-10-19 Saleem Yousuf , Md Maruf Mridha , Rita Magri

The observation of superconductivity in infinite layer nickelate (Nd,Sr)NiO$_{2}$ thin films has led to rapid theoretical and experimental investigations of these copper-oxide-analogue systems [1-15]. Superconductivity has also been found…

We report nuclear magnetic resonance data in the bilayer nickelate La3Ni2O6. This material belongs to a family of low valence nickel oxides with square planar coordination of the Ni ions and is isoelectronic to the high temperature…

Strongly Correlated Electrons · Physics 2013-08-16 N. apRoberts-Warren , J. Crocker , A. P. Dioguardi , K. R. Shirer , V. V. Poltavets , M. Greenblatt , P. Klavins , N. J. Curro

Metallic strontium titanate (SrTiO$_3$) is known to have both normal-state and superconducting properties that vary strongly over a wide range of charge carrier densities. This indicates the importance of nonlinear dynamics, and has…

Strongly Correlated Electrons · Physics 2025-01-27 A. Najev , N. Somun , M. Spaić , I. Khayr , M. Greven , A. Klein , M. N. Gastiasoro , D. Pelc

Upon insertion and extraction of lithium, materials important for electrochemical energy storage can undergo changes in thermal conductivity (${\Lambda}$) and elastic modulus ($\it M$). These changes are attributed to evolution of the…

Applied Physics · Physics 2022-01-10 Jungwoo Shin , Sanghyeon Kim , Hoonkee Park , Ho Won Jang , David G. Cahill , Paul V. Braun

We have investigated the electronic, vibrational, optical, thermal and piezoelectric properties of LiNbO$_3$, LiTaO$_3$ and Li$_2$NbTaO$_6$ using the first-principles calculation based on the density functional theory. It also shows…

Materials Science · Physics 2025-03-28 Debidutta Pradhan , Rojalin Swain , Souvagya Kumar Biswal , Jagadish Kumar

Heavily oxygen deficient NdNiO$_3$ (NNO) films, which are insulating due to electron localization, contain pristine regions that undergo a hidden metal-insulator transition. Increasing oxygen content increases the connectivity of the…

Strongly Correlated Electrons · Physics 2021-09-01 Qikai Guo , Beatriz Noheda

Ni/Al reactive multilayers are promising materials for applications requiring controlled local energy release and superior mechanical performance. This study systematically investigates the impact of compositional variations, ranging from…

Materials Science · Physics 2026-04-14 Nensi Toncich , Fabian Schwarz , Rebecca A. Gallivan , Jemma Gillon , Ralph Spolenak

Layered-oxide $\mathrm{LiNi_xMn_yCo_{1-x-y}O_2}$ (NMC) positive electrodes with high Nickel content, deliver high voltages and energy densities. However, a high nickel content, e.g., $x$ = 0.8 (NMC 811), can lead to high surface reactivity,…

Materials Science · Physics 2023-07-11 Hengning Chen , Zeyu Deng , Yuheng Li , Pieremanuele Canepa

The intimate correlation between the local atomic arrangement and electronic states in Li-ion battery cathode materials plays a crucial role in determining their electrochemical properties, including capacity, cycling stability, and rate…

Lithium-intercalated layered transition-metal oxides, LixTMO2, brought about a paradigm change in rechargeable batteries in recent decades and show promise for use in memristors, a type of device for future neural computing and on-chip…

Materials Science · Physics 2021-05-31 Tianli Feng , Andrew O'Hara , Sokrates T. Pantelides

Lattice dynamics and molecular dynamics studies of the oxides UO2 and Li2O in their normal as well as superionic phase are reported. Lattice dynamics calculations have been carried out using a shell model in the quasiharmonic approximation.…

Materials Science · Physics 2011-11-10 Prabhatasree Goel , N. Choudhury , S. L. Chaplot