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Level-crossing spectroscopy involves lifting the degeneracy of an excited state and using the interference of two nearly degenerate levels to measure the excited state lifetime. Here we use the idea of interference between different…

Optics · Physics 2016-04-27 R. Glenn , M. Dantus

In a prevous paper (Phys. Rev. Lett. 96, 150403 (2006)) we have proposed a new way to generate an observable geometric phase on a quantum system by means of a completely incoherent phenomenon. The basic idea was to force the ground state of…

Quantum Physics · Physics 2009-11-13 Angelo Carollo , G. Massimo Palma

The study of geometric phase in quantum mechanics has so far be confined to discrete (or continuous) spectra and trace preserving evolutions. Consider only the transmission channel, a scattering process with internal degrees of freedom is…

Quantum Physics · Physics 2013-05-29 H. D. Liu , X. X. Yi

We study the geometric phase of an open two-level quantum system under the influence of a squeezed, thermal environment for both non-dissipative as well as dissipative system-environment interactions. In the non-dissipative case, squeezing…

Quantum Physics · Physics 2009-11-13 Subhashish Banerjee , R. Srikanth

Interactions govern the flow of information and the formation of correlations in quantum systems, dictating the phases of matter found in nature and the forms of entanglement generated in the laboratory. Typical interactions decay with…

Quantum interference between multiple pathways in molecular photodissociation often results in angular momentum polarization of atomic products and this can give deep insight into fundamental physical processes. For dissociation of diatomic…

Chemical Physics · Physics 2022-04-26 Chaya Weeraratna , Arthur G. Suits , Oleg S. Vasyutinskii

The concepts of geometric phase and wave-particle duality are interlinked to several fundamental phenomena in quantum physics, but their mutual relationship still forms an uncharted open problem. Here we address this question by studying…

Quantum Physics · Physics 2023-11-01 Elvis Pillinen , Atri Halder , Ari T. Friberg , Tero Setälä , Andreas Norrman

The discovery of topological phases in condensed matter systems has changed the modern conception of phases of matter. The global nature of topological ordering makes these phases robust and hence promising for applications. However, the…

We theoretically investigate internal conversion processes of a photoexcited molecule in a condensed phase. The molecular system is described by two-dimensional adiabatic ground and excited potential energy surfaces (PESs) that are coupled…

Chemical Physics · Physics 2019-03-22 Tatsushi Ikeda , Yoshitaka Tanimura

Ultrafast optical techniques allow to study ultrafast molecular dynamics involving both nuclear and electronic motion.To support interpretation, theoretical approaches are needed that can describe both the nuclear and electron…

Computational Physics · Physics 2021-04-14 Thomas Schnappinger , Regina de Vivie-Riedle

Quantum mechanics dominates various effects in modern research from miniaturizing electronics, up to potentially ruling solid-state physics, quantum chemistry and biology. To study these effects experimental quantum systems may provide the…

Quantum Physics · Physics 2019-09-11 Frederick Hakelberg , Philip Kiefer , Matthias Wittemer , Ulrich Warring , Tobias Schaetz

All-atom simulations can provide molecular-level insights into the dynamics of gas-phase, condensed-phase and surface processes. One important requirement is a sufficiently realistic and detailed description of the underlying intermolecular…

Chemical Physics · Physics 2022-06-15 K. Töpfer , M. Upadhyay , M. Meuwly

We suggest that the ultrarelativistic collisions of heavy ions provide the simplest situation for the study of strong interactions which can be understood from first principles and without any model assumptions about the microscopic…

High Energy Physics - Phenomenology · Physics 2009-10-31 A. Makhlin

Electronic wave-functions in the adiabatic representation acquire nontrivial geometric phases (GPs) when corresponding potential energy surfaces undergo conical intersection (CI). These GPs have profound effects on the nuclear quantum…

Chemical Physics · Physics 2016-07-04 Artur F. Izmaylov , Jiaru Li , Loic Joubert-Doriol

By viewing entanglement as a state function, a new kind of phase transition takes place: the geometric phase transition. This phenomenon occurs due to singularities in the shape of the entangled states set. It is shown how this result can…

Quantum Physics · Physics 2007-05-23 Daniel Cavalcanti , Fernando G. S. L. Brandao , Marcelo O. Terra Cunha

Current experimental and theoretical studies on the effect of intermolecular interactions on molecular conduction appear to be in conflict with each other. In particular, some experimental results, e.g., the observation of 2-dimensional…

Mesoscale and Nanoscale Physics · Physics 2007-07-23 A. Landau , L. Kronik , A. Nitzan

Attochemistry aims to exploit the properties of coherent electronic wavepackets excited via attosecond pulses, to control the formation of photoproducts. Such molecular processes can in principle be simulated with various nonadiabatic…

Chemical Physics · Physics 2024-05-28 Thierry Tran , Anthony Ferté , Morgane Vacher

Examples of geometric phases abound in many areas of physics. They offer both fundamental insights into many physical phenomena and lead to interesting practical implementations. One of them, as indicated recently, might be an inherently…

The state of a quantum system, adiabatically driven in a cycle, may acquire a measurable phase depending only on the closed trajectory in parameter space. Such geometric phases are ubiquitous, and also underline the physics of robust…

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…

Atomic Physics · Physics 2021-07-14 Frederic Hummel , Matthew T. Eiles , Peter Schmelcher