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2D magnetic semiconductors, which intrinsically couple a rich landscape of magnetic orders with tightly bound electron-hole pairs (excitons), present an exciting platform to investigate the interplay between optical and magnetic phenomena…

Coherent interaction between matter and periodic light field induces both optical Stark effect (OSE) and Bloch-Siegert shift (BSS). Observing the BSS has been historically challenging, not only because it is weak but it is often accompanied…

Mesoscale and Nanoscale Physics · Physics 2022-10-12 Yuxuan Li , Yaoyao Han , Wenfei Liang , Boyu Zhang , Yulu Li , Yuan Liu , Yupeng Yang , Jingyi Zhu , Kaifeng Wu

The electronic band structure of V$_2$O$_5$ is calculated using an all-electron quasiparticle self-consistent (QS) $GW$ method, including electron-hole ladder diagrams in the screening of $W$. The optical dielectric function calculated with…

Materials Science · Physics 2024-07-31 Claudio Garcia , Santosh Kumar Radha , Swagata Acharya , Walter R. L. Lambrecht

The optical properties of bulk ZrSiS nodal-line semimetal are theoretically studied within a many-body formalism. The G0W0 bands are similar to those calculated within the density functional theory, except near the {\Gamma} point; in…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Juan J. Meléndez , Andrés Cantarero

In a recent letter [J. -H. Choi et al. Phys. Rev. Lett. 115, 066403 (2015)], a universal linear relation between the binding energy Eb of exciton and the band gap Eg is found in different quasi-2D semiconductors. However, when one…

Materials Science · Physics 2017-06-07 Mingliang Zhang , Ling-Yi Huang , Xu Zhang , Gang Lu

We study the size-dependent exciton fine structure in monolayer black phosphorus quantum dots (BPQDs) deposited on different substrates (isolated, Si and SiO$_2$) using a combination of tight-binding method to calculate the single-particle…

Mesoscale and Nanoscale Physics · Physics 2017-07-19 J. S. de Sousa , M. A. Lino , D. R. da Costa , A. Chaves , J. M. Pereira , G. A. Farias

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 Roland Gillen , Janina Maultzsch

Monolayer transition-metal dichalcogenides are direct gap semiconductors with great promise for optoelectronic devices. Although spatial correlation of electrons and holes plays a key role, there is little experimental information on such…

Materials Science · Physics 2015-06-23 A. T. Hanbicki , M. Currie , G. Kioseoglou , A. L. Friedman , B. T. Jonker

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…

Exciton-exciton interactions are key to understanding non-linear optical and transport phenomena in van der Waals heterobilayers, which emerged as versatile platforms to study correlated electronic states. We present a combined…

Excitons, electron-hole pairs bound by the Coulomb potential, are fundamental quasiparticles of coherent light-matter interaction energizing processes from photosynthesis to optoelectronics. Excitons are observed in semiconductors, and…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Xuefeng Cui , Cong Wang , Adam Argondizzo , Sean Garrett-Roe , Branko Gumhalter , Hrvoje Petek

We theoretically investigate lead iodide perovskites of general formula APbI$_3$ for a series of metallic cations (namely Cs$^+$, Rb$^+$, K$^+$, Na$^+$ and Li$^+$) by means of the density functional theory, GW method and Bethe-Salpeter…

Materials Science · Physics 2024-01-30 Małgorzata Wierzbowska , Juan J. Meléndez

Entanglement of the excitonic states in the system of two coupled semiconductor microcrystallites, whose sizes are much larger than the Bohr radius of exciton in bulk semiconductor but smaller than the relevant optical wavelength, is…

Quantum Physics · Physics 2009-08-03 Yu-xi Liu , Sahin K. Ozdemir , Adam Miranowicz , Masato Koashi , Nobuyuki Imoto

The multi-quantum well (MQW) organic-inorganic perovskite offer an approach of tuning the exciton binding energy based on the well-barrier dielectric mismatch effect, which called the image charge effect. The exfoliation from MQW…

Mesoscale and Nanoscale Physics · Physics 2017-08-02 Haitham Zahra , Aïda Hichri , Sihem Jaziri

Layered 2D organic-inorganic perovskite semiconductors support strongly confined excitons that offer significant potential for ultrathin polaritonic devices due to their tunability and huge oscillator strength. The application of a magnetic…

Mesoscale and Nanoscale Physics · Physics 2025-02-26 Jonas K. König , Jamie M. Fitzgerald , Ermin Malic

Moir\'e superlattices of transition-metal dichalcogenide bilayers host strong Coulomb interactions residing in narrow electron bands, leading to correlated insulating states at fractional carrier doping densities, known as generalized…

We present a detailed many-body ab initio study of the valence-skipper RbTlCl$_{3}$ perovskite compound for photovoltaic (PV) applications. The electronic and optical properties, both with and without spin-orbit coupling, have been…

Materials Science · Physics 2025-08-25 Siddharth , Vinod Kumar Solet , Sudhir K. Pandey

Electrons and holes can spontaneously form excitons and condense in a semimetal or semiconductor, as predicted decades ago. This type of Bose condensation can happen at much higher temperatures in comparison with dilute atomic gases.…

Mesoscale and Nanoscale Physics · Physics 2023-02-24 Qiang Gao , Yang-hao Chan , Yuzhe Wang , Haotian Zhang , Jinxu Pu , Shengtao Cui , Yichen Yang , Zhengtai Liu , Dawei Shen , Zhe Sun , Juan Jiang , Tai C. Chiang , Peng Chen

We use path integral Monte Carlo to study the energetics of excitons in layered, hybrid organic-inorganic perovskites in order to elucidate the relative contributions of dielectric confinement and electron-phonon coupling. While the…

Materials Science · Physics 2025-03-26 Rohit Rana , David T. Limmer
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