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A theoretical model for excitons confined in layered metal halide perovskites is presented. The model accounts for polaronic effects, dielectric and quantum confinement by means of effective mass theory, image charges and Haken potentials.…

Mesoscale and Nanoscale Physics · Physics 2023-08-08 Jose L. Movilla , Josep Planelles , Juan I. Climente

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…

Quantum interference between one- and two-photon absorption pathways allows coherent control of interband transitions in unbiased bulk semiconductors; carrier population, carrier spin polarization, photocurrent injection, and spin current…

Other Condensed Matter · Physics 2007-05-23 R. D. R. Bhat , J. E. Sipe

Excitons, bound electron-hole pairs, influence the optical properties in strongly interacting solid state systems. Excitons and their associated many-body physics are typically most stable and pronounced in monolayer materials. Bulk systems…

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

Materials Science · Physics 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation…

Mesoscale and Nanoscale Physics · Physics 2024-08-29 Kenneth Choo , Olivier Bleu , Jesper Levinsen , Meera M. Parish

Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Thomas Mueller , Ermin Malic

Owing to both electronic and dielectric confinement effects, two-dimensional organic-inorganic hybrid perovskites sustain strongly bound excitons at room temperature. Here, we demonstrate that there are non-negligible contributions to the…

Exciton fine structures in cubic III-V semiconductor GaAs, InAs and GaN quantum dots are investigated systematically and the exciton spin relaxation in GaN quantum dots is calculated by first setting up the effective exciton Hamiltonian.…

Mesoscale and Nanoscale Physics · Physics 2011-06-15 H. Tong , M. W. Wu

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

We present a systematic investigation of the role and importance of excitonic effects on the optical properties of transitions metal oxide perovskites. A representative set of fourteen compounds has been selected, including 3$d$ (SrTiO$_3$,…

The excitonic spectra of single layer GeS and GeSe are predicted by ab initio GW-Bethe Salpeter equation calculations. G 0 W 0 calculations for the band structures find a fundamental band gap of 2.85 eV for GeS and 1.70 eV for GeSe…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 Lidia C. Gomes , P. E. Trevisanutto , A. Carvalho , A. S. Rodin , A. H. Castro Neto

Exciton-polaritons in semiconductor microcavities generate fascinating effects such as long-range spatial coherence and Bose-Einstein Condensation (BEC), which are attractive for their potential use in low threshold lasers, vortices and…

Mesoscale and Nanoscale Physics · Physics 2017-09-27 Shuai Zhang , Qiuyu Shang , Wenna Du , Jia Shi , Yang Mi , Jie Chen , Zhiyong Wu , Yuanzheng Li , Mei Liu , Qing Zhang , Xinfeng Liu

Layered halide perovskites exhibit remarkable optoelectronic properties and technological promise, driven by strongly bound excitons. The interplay of spin-orbit and exchange coupling creates a rich excitonic landscape, determining their…

Most semiconductors, in particular III-V compounds, have a complex valence band structure near the band edge, due to degeneracy at the zone center. One peculiar feature is the warping of the electronic dispersion relations, which are not…

Strongly Correlated Electrons · Physics 2023-07-12 Roland Combescot , Shiue-Yuan Shiau

We present a quantitative study of the nonlinear optical response of layered perovskites placed inside planar photonic microcavities in the regime of strong light matter coupling, when excitonic and photonic modes hybridize and give rise to…

Mesoscale and Nanoscale Physics · Physics 2022-11-15 A. D. Belogur , D. A. Baghdasaryan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

Layered hybrid perovskites containing larger organic cations have demonstrated superior environmental stability, but the presence of these insulating spacers also strengthens the exciton binding energy, which contributes to reduced carrier…

Excitonic stimulated emission provides a promising mechanism and route to achieve low-threshold semiconductor lasers for micro-nano optoelectronic integrations. However, excitonic stimulated emission from quantum structure-free…

Excitons are the neutral quasiparticles that form when Coulomb interactions create bound states between electrons and holes. Due to their bosonic nature, excitons are expected to condense and exhibit superfluidity at sufficiently low…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Hong-Yi Xie , Pouyan Ghaemi , Matteo Mitrano , Bruno Uchoa

The organic spacer cation plays a crucial role in determining the exciton fine structure in two-dimensional (2D) perovskites. Here, we use low-temperature magneto-optical spectroscopy to gain insight into the influence of the organic spacer…