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Quantum computers promise to revolutionise electronic simulations by overcoming the exponential scaling of many-electron problems. While electronic wave functions can be represented using a product of fermionic unitary operators, shallow…

Quantum Physics · Physics 2022-07-04 Hugh G. A. Burton , Daniel Marti-Dafcik , David P. Tew , David J. Wales

We present an efficient algorithm for twirling a multi-qudit quantum state. The algorithm can be used for approximating the twirling operation in an ensemble of physical systems in which the systems cannot be individually accessed. It can…

Quantum Physics · Physics 2007-05-23 Geza Toth , Juan Jose Garcia-Ripoll

The construction of the Hamiltonian matrix \textbf{H} is an essential, yet computationally expensive step in \textit{ab-initio} device simulations based on density-functional theory (DFT). In homogeneous structures, the fact that a unit…

Disordered Systems and Neural Networks · Physics 2026-02-03 Chen Hao Xia , Manasa Kaniselvan , Marko Mladenoivić , Mathieu Luisier

A central problem in biophysics and computational drug design is accurate modeling of biomolecules. The current molecular dynamics simulation methods can answer how a molecule inhibits a cancerous cell signaling pathway, or the role of…

Quantum Physics · Physics 2019-10-31 Anurag Mishra , Alireza Shabani

Working with trapped atoms at close distance to each other, we show that one can implement entangling gates based on non-independent qubits using a single pulse per qubit, or a single structured pulse. The optimal parameters depend on…

Quantum Physics · Physics 2023-10-19 Ignacio R. Sola , Seokmin Shin , Bo Y. Chang

In the near future, material and drug design may be aided by quantum computer assisted simulations. These have the potential to target chemical systems intractable by the most powerful classical computers. However, the resources offered by…

The fidelity of quantum circuits (QC) is influenced by several factors, including hardware characteristics, calibration status, and the transpilation process, all of which impact their susceptibility to noise. However, existing methods…

Quantum Physics · Physics 2025-05-22 Yikai Mao , Shaswot Shresthamali , Masaaki Kondo

Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White

Simulating the real-time dynamics of quantum field theories (QFTs) is one of the most promising applications of quantum simulators. Regularizing a bosonic QFT for quantum simulation purposes typically involves a truncation in Hilbert space…

Quantum Physics · Physics 2025-09-01 Gabriele Calliari , Marco Di Liberto , Hannes Pichler , Torsten V. Zache

The problem of simulating the thermal behavior of quantum systems remains a central open challenge in quantum computing. Unlike well-established quantum algorithms for unitary dynamics, \emph{provably efficient} algorithms for preparing…

Quantum Physics · Physics 2026-05-14 Dominik Hahn , Ryan Sweke , Abhinav Deshpande , Oles Shtanko

Deep neural networks (DNNs) have been used to successfully predict molecular properties calculated based on the Kohn--Sham density functional theory (KS-DFT). Although this prediction is fast and accurate, we believe that a DNN model for…

Chemical Physics · Physics 2020-11-17 Masashi Tsubaki , Teruyasu Mizoguchi

We formulate and implement Cyclic Density Functional Theory (Cyclic DFT) -- a self-consistent first principles simulation method for nanostructures with cyclic symmetries. Using arguments based on Group Representation Theory, we rigorously…

Materials Science · Physics 2017-03-16 Amartya S. Banerjee , Phanish Suryanarayana

Scalable quantum-classical embedding is essential for chemically meaningful simulations on near-term NISQ hardware. Using QDFT, we show systematic recovery of correlation energy relative to the DFT baseline, benchmarked against CCSD in a…

Quantum Physics · Physics 2026-02-03 Namrata Manglani , Samrit Kumar Maity , Ranjit Thapa , Sanjay Wandhekar

Quantum embedding schemes have the potential to significantly reduce the computational cost of first principles calculations, whilst maintaining accuracy, particularly for calculations of electronic excitations in complex systems. In this…

Materials Science · Physics 2022-03-10 Joseph C. A. Prentice

Kohn-Sham (KS) density functional theory (DFT) is a very efficient method for calculating various properties of solids as, for instance, the total energy, the electron density, or the electronic band structure. The KS-DFT method leads to…

Materials Science · Physics 2019-09-20 Fabien Tran , Jan Doumont , Leila Kalantari , Ahmad W. Huran , Miguel A. L. Marques , Peter Blaha

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

We introduce a distributed classical simulation algorithm for general quantum circuits, and present numerical results for calculating the output probabilities of universal random circuits. We find that we can simulate more qubits to greater…

Quantum Physics · Physics 2018-05-08 Jianxin Chen , Fang Zhang , Cupjin Huang , Michael Newman , Yaoyun Shi

We define formally decohered quantum computers (using density matrices), and present a simulation of them by a probabalistic classical Turing Machine. We study the slowdown of the simulation for two cases: (1) sequential quantum computers,…

Quantum Physics · Physics 2007-05-23 Dorit Aharonov , Michael Ben-Or

In the near future, a major challenge in quantum computing is to scale up robust qubit prototypes to practical problem sizes and to implement comprehensive error correction for computational precision. Due to inevitable quantum…

Quantum Physics · Physics 2018-03-28 Joni Ikonen , Juha Salmilehto , Mikko Möttönen

Quantum computing is a new technology that is expected to revolutionize the computation paradigm in the next few years. Qubits exploit the quantum physics proprieties to increase the parallelism and speed of computation. Unfortunately,…

Emerging Technologies · Computer Science 2022-04-12 Daniel Oliveira , Edoardo Giusto , Emanuele Dri , Nadir Casciola , Betis Baheri , Qiang Guan , Bartolomeo Montrucchio , Paolo Rech