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We theoretically investigate high harmonic generation (HHG) from silicon thin films with thicknesses from a few atomic layers to a few hundreds of nanometers, to determine the most efficient thickness for producing intense HHG in the…

Materials Science · Physics 2021-04-28 Shunsuke Yamada , Kazuhiro Yabana

The propagation-effects reshaping the excitation pulse are known to exhibit a strong influence on the high-harmonic generation (HHG) in solid-state media. Previous measurements showed that the mid-infrared pulse dynamics, most importantly…

Optics · Physics 2024-05-22 M. Kolesik

High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…

Optics · Physics 2018-04-26 Dieter Bauer , Kenneth K. Hansen

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Terahertz high harmonic generation (THz HHG) is a common property of nonlinear systems. Recently it has been used to investigate fundamental principles that govern transport and nonlinear dynamics in novel quantum materials like graphene,…

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

Applying the semiclassical model, we identify two connected effects in intraband high-harmonic generation (HHG): (1) propagation time from the point of emission at the source to the point of detection, (2) beyond-electric-dipole corrections…

Atomic Physics · Physics 2024-06-12 Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

The non-linear propagation of the intense near-infrared (NIR) driving field in wide bandgap materials pose a challenge and an opportunity to control the spectral properties of high harmonic generation (HHG) in solids. Here, we have…

Optics · Physics 2023-07-06 Mukhtar Hussain , Gareth O Williams , Tayyab Imran , Marta Fajardo

3D Dirac semimetals (DSMs) are promising materials for terahertz high harmonic generation (HHG). We show that 3D DSMs' high nonlinearity opens up a regime of nonlinear optics where extreme subwavelength current density features develop…

Optics · Physics 2021-06-21 Jeremy Lim , Yee Sin Ang , Lay Kee Ang , Liang Jie Wong

We present an exact treatment of wave propagation in some inhomogeneous thin films with highly space-dependent dielectric constant. It is based on a space transformation which replaces the physical space by the optical path. In the new…

Optics · Physics 2009-11-11 Guillaume Petite , Alexander Shvartsburg

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

Using a fully real-space perspective on high harmonic generation (HHG) in solids, we examine the relationship between microscopic response, macroscopic propagation of this response to the far field, and the extremely short dephasing times…

We report theoretical calculations of high harmonic generation (HHG) by intense infrared lasers in atomic and molecular targets taking into account the macroscopic propagation of both fundamental and harmonic fields. On the examples of Ar…

Atomic Physics · Physics 2011-02-28 Cheng Jin , Anh-Thu Le , C. D. Lin

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

The production of brighter coherent XUV radiation by intense laser pulses through the process of high-harmonic generation (HHG) is a central challenge in contemporary nonlinear optics. We study the generation and spatial propagation of high…

Optics · Physics 2025-06-03 Margarita Khokhlova , Vasily Strelkov

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

Materials Science · Physics 2020-12-23 G. P. Zhang , Y. H. Bai

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

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