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Liquid mixtures composed of colloidal particles and much smaller non-adsorbing linear homopolymers can undergo a gelation transition due to polymer-mediated depletion forces. We now show that the addition of linear polymers to suspensions…

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

Soft Condensed Matter · Physics 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

Several lattice models display a condensation transition in real space when the density of a suitable order parameter exceeds a critical value. We consider one of such models with two conservation laws, in a one-dimensional open setup where…

Statistical Mechanics · Physics 2022-12-01 Gabriele Gotti , Stefano Iubini , Paolo Politi

We study slow dynamics of particles moving in a matrix of immobile obstacles using molecular dynamics simulations. The glass transition point decreases drastically as the obstacle density increases. At higher obstacle densities, the…

Soft Condensed Matter · Physics 2009-11-17 Kang Kim , Kunimasa Miyazaki , Shinji Saito

The rapid collapse of a polymer, due to external forces or changes in solvent, yields a long-lived `crumpled globule.' The conjectured fractal structure shaped by hierarchical collapse dynamics has proved difficult to establish, even with…

Soft Condensed Matter · Physics 2015-10-07 Guy Bunin , Mehran Kardar

The Hamiltonian dynamics of chains of nonlinearly coupled particles is numerically investigated in two and three dimensions. Simple, off-lattice homopolymer models are used to represent the interparticle potentials. Time averages of…

Statistical Mechanics · Physics 2007-05-23 Alessandro Mossa , Marco Pettini , Cecilia Clementi

Systems undergoing an equilibrium phase transition from a liquid state to an amorphous solid state exhibit certain universal characteristics. Chief among these are the fraction of particles that are randomly localized and the scaling…

Disordered Systems and Neural Networks · Physics 2009-10-30 Weiqun Peng , Horacio E. Castillo , Paul M. Goldbart , Annette Zippelius

Simulating percolation and critical phenomena of labelled species inside films composed of single-component linear homogeneous macromolecules using molecular Monte Carlo method in 3 dimensions, we study dependence of these conducting…

Soft Condensed Matter · Physics 2019-09-05 Yuki Norizoe , Hiroshi Morita

Colloid-polymer mixtures may undergo either fluid-fluid phase separation or gelation. This depends on the depth of the quench (polymer concentration) and polymer-colloid size ratio. We present a real-space study of dynamics in phase…

Soft Condensed Matter · Physics 2012-09-19 Isla Zhang , C. Patrick Royall , Paul Bartlett , Malcolm A. Faers

We study reactions between end-functionalized chains at a polymer-polymer interface. For small chemical reactivities (the typical case) the number of diblocks formed, $R_t$, obeys 2nd order chemically controlled kinetics, $R_t \sim t$,…

Soft Condensed Matter · Physics 2009-10-31 Ben O'Shaughnessy , Dimitrios Vavylonis

Letting free polymers diffuse from solution into a crosslinked polymer gel is often a crucial processing step in the synthesis of multiphase polymer-based gels, e.g., core-shell microgels. Here we use coarse-grained molecular dynamics…

Soft Condensed Matter · Physics 2024-12-17 Jude Ann Vishnu , Torsten Gereon Linder , Sebastian Seiffert , Friederike Schmid

* ACTIVATED RANDOM WALK MODEL * This is a conservative particle system on the lattice, with a Markovian continuous-time evolution. Active particles perform random walks without interaction, and they may as well change their state to…

Probability · Mathematics 2011-03-15 Leonardo T. Rolla

There appears to be a longtime, very slowly evolving state in dense simple fluids which, for high enough density, approaches a glassy nonergodic state. The nature of the nonergodic state can be characterized by the associated static…

Statistical Mechanics · Physics 2014-02-19 Gene F. Mazenko

We analyze the crystallization and collapse transition of a simple model for flexible polymer chains on simple cubic and face-centered cubic lattices by means of sophisticated chain-growth methods. In contrast to bond-fluctuation polymer…

Soft Condensed Matter · Physics 2009-11-13 Thomas Vogel , Michael Bachmann , Wolfhard Janke

We studied the dynamics of isotropic-nematic transitions in liquid crystalline polymers by integrating time-dependent Ginzburg-Landau equations. In a concentrated solution of rodlike polymers, the rotational diffusion constant Dr of the…

Soft Condensed Matter · Physics 2015-05-28 Shunsuke Yabunaka , Takeaki Araki

We study an interacting box-particle system on a one-dimensional periodic ring involving two species of particles $A$ and $B$. In this model, from a randomly chosen site, a particle of species $A$ can hop to its right neighbor with a rate…

Statistical Mechanics · Physics 2017-03-06 Bijoy Daga

We once more specify an universality of a phase transition from smectic-A to nematic phase in the crosslinked polymer network with a smectic liquid crystal, basing on the X-ray and $^1H$-NMR spectroscopy experiments. Comparing the…

Soft Condensed Matter · Physics 2010-03-30 L. V. Elnikova

We theoretically investigate the looping dynamics of a linear polymer immersed in a viscoelastic fluid. The dynamics of the chain is governed by a Rouse model with a fractional memory kernel recently proposed by Weber et al. (S. C. Weber,…

Soft Condensed Matter · Physics 2012-07-09 Rajarshi Chakrabarti

We study the unfolding of a single polymer chain due to an external force. We use a simplified model which allows to perform all calculations in closed form without assuming a Boltzmann-Gibbs form for the equilibrium distribution.…

Statistical Mechanics · Physics 2009-11-13 Erik Van der Straeten , Jan Naudts

The past few years have seen many advances in our understanding of the dynamics of polymeric fluids. These include improvements on the successful reptation theory; an emerging molecular theory of semiflexible chain dynamics; and an…

Soft Condensed Matter · Physics 2007-05-23 Peter D. Olmsted