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We report the discovery of giant and anisotropic magnetoresistance due to the orbital rearrangement in a non-magnetic correlated metal. In particular, we measured the magnetoresistance under fields up to 31.4 T in the cubic Pr-based heavy…

Our single crystal study reveals that PrTr2Al20 (Tr = Ti and V) provides the first examples of a cubic {\Gamma}3 nonmagnetic ground doublet system that shows the Kondo effect including a -ln T dependent resistivity. The {\Gamma}3…

Strongly Correlated Electrons · Physics 2015-03-19 Akito Sakai , Satoru Nakatsuji

The cubic compound PrTi$_2$Al$_{20}$ is a quadrupolar Kondo lattice system that exhibits quadrupolar ordering due to the non-Kramers $\Gamma_3$ ground doublet and has strong hybridization between $4f$ and conduction electrons. Our study…

Strongly Correlated Electrons · Physics 2015-06-05 Akito Sakai , Kentaro Kuga , Satoru Nakatsuji

Heavy fermion metals hosting multipolar local moments set a new stage for exploring exotic spin-orbital entangled quantum phases. In such systems, the quadrupolar Kondo effect serves as the key ingredient in the orbital-driven non-Fermi…

Strongly Correlated Electrons · Physics 2020-01-14 Mingxuan Fu , Akito Sakai , Naoki Sogabe , Masaki Tsujimoto , Yosuke Matsumoto , Satoru Nakatsuji

We report thermal expansion and magnetostriction of the cubic non-Kramers system PrIr$_2$Zn$_{20}$ with a non-magnetic $\varGamma_{3}$ ground state doublet. In previous experiments, antiferroquadrupolar order at…

Strongly Correlated Electrons · Physics 2019-02-27 A. Wörl , T. Onimaru , Y. Tokiwa , Y. Yamane , K. T. Matsumoto , T. Takabatake , P. Gegenwart

Ferro-quadrupole (FQ) order in the non-Kramers $\Gamma_3$ doublet system PrTi$_2$Al$_{20}$ has been investigated via angle-resolved measurements of the specific heat, rotational magnetocaloric effect, and entropy, under a rotating magnetic…

Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior.…

Strongly Correlated Electrons · Physics 2018-03-08 Frederic Freyer , Jan Attig , SungBin Lee , Arun Paramekanti , Simon Trebst , Yong Baek Kim

Extremely large magnetoresistance (XMR) was recently discovered in many non-magnetic materials, while its underlying mechanism remains poorly understood due to the complex electronic structure of these materials. Here, we report an…

We report magnetic-field-induced first-order phase transitions in the ferro-quadrupole (FQ) ordered state of PrTi2Al20, in which non-Kramers Pr3+ ions with two 4f electrons have a non-magnetic Gamma3 doublet ground state in the cubic Td…

The two-dimensional electron system in (110)Al$_2$O$_{3-\delta}$/SrTiO$_3$ heterostructures displays anisotropic electronic transport. Largest and lowest conductivity and electron mobility $\mu$ are observed along the $[001]$ and…

Strongly Correlated Electrons · Physics 2018-09-19 K. Wolff , R. Eder , R. Schäfer , R. Schneider , D. Fuchs

A series of Pr(TM)$_2$X$_{20}$ (with TM=Ti,V,Rh,Ir and X=Al,Zn) Kondo materials, containing non-Kramers Pr$^{3+}$ $4f^2$ moments on a diamond lattice, have been shown to exhibit intertwined orders such as quadrupolar order and…

Strongly Correlated Electrons · Physics 2018-11-07 SungBin Lee , Simon Trebst , Yong Baek Kim , Arun Paramekanti

After growing successfully high quality VP$_2$ single crystals, we studied systematically their longitudinal $\rho_{xx}(T)$ and Hall resistivity $\rho_{yx}(T)$ at various magnetic fields, combining the electronic band and Fermi surface (FS)…

Strongly Correlated Electrons · Physics 2026-04-30 Chunxiang Wu , Shuijin Chen , Tingyu Zhou , Le Liu , Xin Peng , Jianjian Jia , Xinyu Yu , Hangdong Wang , Jinhu Yang , Jianhua Du , Minghu Fang

The extremely large magnetoresistance (XMR) observed in many topologically nontrivial and trivial semimetals has attracted much attention in relation to its underlying physical mechanism. In this paper, by combining the band structure and…

Heavy fermion (HF) materials exhibit a rich array of phenomena due to the strong Kondo coupling between their localized moments and itinerant electrons. A central question in their study is to understand the interplay between magnetic order…

Materials Science · Physics 2016-03-02 S. M. Thomas , P. F. S. Rosa , S. B. Lee , S. A. Parameswaran , Z. Fisk , J. Xia

We present a comprehensive first-principles study of the magnetoresistance in ZrSi$X$ ($X=$ S, Se, Te) topological nodal-line semimetals. Our study demonstrates that all primary features of the experimentally measured magnetoresistance in…

Materials Science · Physics 2025-10-31 ShengNan Zhang , Oleg V. Yazyev

Metallic amorphous ferrimagnets of 3d transition metals (TM) and rare earths (RE) with 4f electrons exhibit rich magneto transport behavior due to the interplay between the 3d and 4f magnetic sublattices and their interaction with mobile…

We report a detailed study of the electrical transport properties of single crystals of Pr$_4$Fe$_2$As$_2$Te$_{1-x}$O$_4$, a recently discovered iron-based superconductor. Resistivity, Hall effect and magnetoresistance are measured in a…

Superconductivity · Physics 2016-12-22 A. Pisoni , P. Szirmai , S. Katrych , B. Náfrádi , R. Gaál , J. Karpinski , L. Forró

We performed field-angle-resolved magnetostriction and thermal-expansion measurements on PrIr$_2$Zn$_{20}$, a cubic non-Kramers compound exhibiting antiferroquadrupolar order below $T_{\rm Q}=0.125$ K. Thermal expansion exhibits two…

Strongly Correlated Electrons · Physics 2025-12-23 Naoki Okamoto , Yohei Kono , Takahiro Onimaru , Keisuke T. Matsumoto , Kazumasa Hattori , Shunichiro Kittaka

Recent experiments have examined the impact of a magnetic field on ferroquadrupolar orders in the intermetallic Kondo material PrTi$_2$Al$_{20}$. Motivated by this, we use extensive Monte Carlo simulations to study a diamond lattice XY…

Strongly Correlated Electrons · Physics 2020-08-04 Frederic Freyer , SungBin Lee , Yong Baek Kim , Simon Trebst , Arun Paramekanti

We present a systematic study of the dc-resistivity, Hall effect, and magnetoresistance in the normal state of quasi 2D heavy fermion superconductors CeMIn5 (M: Rh and Co) under pressure. Here the electronic system evolves with pressure…

Strongly Correlated Electrons · Physics 2010-09-16 Y. Nakajima , H. Shishido , H. Nakai , T. Shibauch , K. Behnia , K. Izawa , M. Hedo , Y. Uwatoko , T. Matsumoto , R. Settai , Y. Onuki , H. Kontani , Y. Matsuda
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