Related papers: Zeeman-Sisyphus Deceleration for Heavy Molecules w…
We demonstrate sub-recoil Sisyphus cooling using the long-lived $^{3}\mathrm{P}_{0}$ clock state in alkaline-earth-like ytterbium. A 1388 nm optical standing wave nearly resonant with the…
We present a theoretical study of the Zeeman relaxation of the magnetically trappable lowest field seeking state of MnH(^7 \Sigma) in collisions with 3He. We analyze the collisional Zeeman transition mechanism as a function of the final…
We report the construction and characterization of an experimental setup for producing a cold gas of $^{40}$Ca atoms and excite them to high Rydberg states with a resonant three-photon-excitation scheme. The apparatus comprises four stages,…
Recently a number of diatomic and polyatomics molecules has been identified as a prospective systems for Doppler/Sisyphus cooling. Doppler/Sisyphus cooling allows to decrease the kinetic energy of molecules down to microkelvin temperatures…
The conversion of optical and electrical energy in novel materials is key to modern optoelectronic and light-harvesting applications. Here, we investigate the equilibration dynamics of photoexcited…
We present the first crossed beam scattering experiment using a Zeeman decelerated molecular beam. The narrow velocity spreads of Zeeman decelerated NO ($X ^2\Pi_{3/2}, j=3/2$) radicals result in high-resolution scattering images, thereby…
Precision spectroscopic measurements in atoms and molecules play an increasingly important role in chemistry and physics, e.g., to characterize structure and dynamics at long timescales, to determine physical constants, or to search for…
We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…
Rapid progress in cooling and trapping of molecules has enabled first experiments on high resolution spectroscopy of trapped diatomic molecules, promising unprecedented precision. Extending this work to polyatomic molecules provides unique…
We demonstrate a compact (0.25 L) system for laser cooling and trapping atoms from a heated dispenser source. Our system uses a nanofabricated diffraction grating to generate a magneto-optical trap (MOT) using a single input laser beam. An…
The YbOH triatomic molecule can be efficiently used to measure the electron electric dipole moment, which violates time-reversal (T) and spatial parity (P) symmetries of fundamental interactions [I. Kozyryev, N.R. Hutzler, Phys. Rev. Lett.…
Chemistry in the ultracold regime enables fully quantum-controlled interactions between atoms and molecules, leading to the discovery of the hidden mechanisms in chemical reactions which are usually curtained by thermal averaging in the…
We report on the sub-Doppler laser cooling of neutral $^{171}$Yb and $^{173}$Yb in a magneto-optical trap using the $^{1}S_{0}$-$^{1}P_{1}$ transition at 398.9nm. We use two independent means to estimate the temperature of the atomic cloud…
It is shown that in experiments on single molecule magnets (SMM's) in which transitions between two lowest spin states are induced by sweeping the applied magnetic field along the easy axis, the transitions are fully incoherent. Nuclear…
We demonstrate the deceleration of heavy polar molecules in low-field seeking states by combining a cryogenic source and a travelling-wave Stark decelerator. The cryogenic source provides a high intensity beam with low speed and…
We present a design of a spin-flip Zeeman slower controlled by a fast feedback circuit for a sodium Bose-Einstein condensate apparatus. We also demonstrate how the efficiency of the slower strongly depends on its intrinsic parameters, and…
We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…
We examine two approaches for significantly extending the velocity range of the optical bichromatic force (BCF), to make it useful for laser deceleration of atomic and molecular beams. First, we present experimental results and calculations…
We realize the first Zeeman slower of an atom in the Main Group III of the periodic table, otherwise known as the "triel elements". Despite that our atom of choice (namely indium) does not have a ground state cycling transition suitable for…
We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of…