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Systematic spectroscopic ellipsometry investigations have been performed in order to elucidate the asymmetric insulator-to-metal transition in thin VO$_2$ films. The comprehensive analysis of the obtained macroscopic optical response yields…

In this work, a thermal switch is proposed based on the phase-change material vanadium dioxide (VO2) within the framework of near-field radiative heat transfer (NFRHT). The radiative thermal switch consists of two metamaterials filled with…

Applied Physics · Physics 2023-09-21 Ming-Jian He , Xue Guo , Hong Qi , Lu Lu , He-Ping Tan

Thermochromic vanadium dioxide thin films have attracted much attention recently for constructing variable-emittance coatings upon its insulator-metal phase transition for dynamic thermal control. However, fabrication of high-quality…

Materials Science · Physics 2025-05-20 Vishwa Krishna Rajan , Jeremy Chao , Sydney Taylor , Liping Wang

We have studied electrical switching with S-shaped I-V characteristics in two-terminal MOM devices based on vanadium dioxide thin films. The switching effect is associated with the metal-insulator phase transition. Relaxation oscillations…

Applied Physics · Physics 2020-01-08 Alexander Pergament , Andrei Velichko , Maksim Belyaev , Vadim Putrolaynen

We have developed a new optical microscopy technique able to track micron-sized surface clusters as temperature is varied. Potential candidates for study include phase separated metal-insulator materials, ferroelectrics, and porous…

Ultrafast optical pump - optical probe and optical pump - terahertz probe spectroscopy were performed on vanadium dioxide (VO2) and vanadium sesquioxide (V2O3) thin films over a wide temperature range. A comparison of the experimental data…

An abrupt metal-insulator transition (MIT) was observed in VO2 thin films during the application of a switching voltage pulse to two-terminal devices. Any switching pulse over a threshold voltage for the MIT of 7.1 V enabled the device…

Strongly Correlated Electrons · Physics 2009-11-11 Byung-Gyu Chae , Hyun-Tak Kim , Doo-Hyeb Youn , Kwang-Yong Kang

We investigate optical forces on oscillating dipoles close to a phase-change vanadium dioxide (VO$_2$) film, which exhibits a metal-insulator transition around $340$ K and low thermal hysteresis. This configuration is related to one…

Mesoscale and Nanoscale Physics · Physics 2021-07-15 Daniela Szilard , Patrícia P. Abrantes , Felipe A. Pinheiro , Felipe S. S. Rosa , Carlos Farina , Wilton J. M. Kort-Kamp

VO2 material is promising for developing energy-saving "smart window", owing to its thermochromic property induced by metal-insulator transition (MIT). However, its practical application is greatly limited by the relatively high critical…

Applied Physics · Physics 2019-05-10 Shi Chen , Zhaowu Wang , Hui Ren , Yuliang Chen , Wensheng Yan , Chengming Wang , Bowen Li , Jun Jiang , Chongwen Zou

The popular dual electronic (Mott) and structural (Peierls) transitions in VO2 are explored using x-ray absorption spectromicroscopy with high spatial and spectral resolutions. It is found that during both heating and cooling, the…

Strongly Correlated Electrons · Physics 2015-11-20 Suhas Kumar , John Paul Strachan , Matthew D. Pickett , Alexander Bratkovsky , Yoshio Nishi , R. Stanley Williams

Vanadium dioxide (VO$_{2}$) undergoes a first-order metal-insulator transition (MIT) upon cooling near room temperature, concomitant with structural change from rutile to monoclinic. Accurate characterization of lattice vibrations is vital…

Materials Science · Physics 2017-11-22 Yi Xia , Maria K. Y. Chan

Methane (CH_4) gas sensing properties of novel vanadium dioxide (VO_2) nanostructured films is reported for the first time. The single phase nanostructures are synthesized by pulsed dc-magnetron sputtering of V target followed by oxidation…

Materials Science · Physics 2015-09-02 A. K. Prasad , S. Amirthapandian , S. Dhara , S. Dash , N. Murali , A. K. Tyagi

The transition voltage of an abrupt metal-insulator transition (MIT), observed by applying an electric field to two-terminal devices fabricated on a Mott insulator VO_2 film, decreases with increasing temperature up to 334K. The abrupt…

Strongly Correlated Electrons · Physics 2007-05-23 Hyun-Tak Kim , B. G. Chae , D. H. Youn , S. L. Maeng , K. Y. Kang

The metal-insulator transition (MIT) of V6O11 is studied by means of electronic structure calculations using the augmented spherical wave method. The calculations are based on density functional theory and the local density approximation.…

Strongly Correlated Electrons · Physics 2009-11-07 U. Schwingenschloegl , V. Eyert , U. Eckern

Dynamic radiative cooling with variable emissive power is experimentally demonstrated in this study by a wavelength-selective tunable metafilm emitter, which consists of an opaque aluminum film, a sputtered silicon spacer, and a…

We report the first application of critical cluster techniques to the Mott metal-insulator transition in vanadium dioxide. We show that the geometric properties of the metallic and insulating puddles observed by scanning near-field infrared…

Strongly Correlated Electrons · Physics 2016-01-27 Shuo Liu , B. Phillabaum , E. W. Carlson , K. A. Dahmen , N. S. Vidhyadhiraja , M. M. Qazilbash , D. N. Basov

We investigate the resistive switching behaviour of $\mathrm{VO_2}$ microbridges under current bias as a function of temperature and thermal coupling with the heat bath. Upon increasing the electrical current bias, the formation of the…

Strongly Correlated Electrons · Physics 2017-02-06 Nicola Manca , Teruo Kanki , Hidekazu Tanaka , Daniele Marré , Luca Pellegrino

$VO_2$ undergoes the insulator-metal transition (IMT) and monoclinic-rutile structural phase transition (SPT) near $67^oC$. The IMT switching has many applications. However, there is an unresolved issue whether the IMT is a Mott transition…

Strongly Correlated Electrons · Physics 2021-01-18 Chang-Yong Kim , Tetiana Slusar , Jinchul Cho , Hyun-Tak Kim

Vanadium dioxide (VO2) is a phase transition material that undergoes a reversible insulator-metal phase transition at ~ 68 C. Atmospheric pressure thermal oxidation (APTO) of vanadium (V) is a simple VO2 synthesis method in which V thin…

Materials Science · Physics 2021-07-06 Ashok P , Yogesh Singh Chauhan , Amit Verma

Neuromorphic functionalities in memristive devices are commonly associated with the ability to electrically create local conductive pathways by resistive switching. The archetypal correlated material, VO2, has been intensively studied for…

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