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Electronic coherence is of utmost importance for the access and control of quantum-mechanical solid-state properties. Using a purely electronic observable, the photocurrent, we measure an electronic coherence time of 22 +/- 4 fs in…

Mesoscale and Nanoscale Physics · Physics 2021-12-08 Christian Heide , Timo Eckstein , Tobias Boolakee , Constanze Gerner , Heiko B. Weber , Ignacio Franco , Peter Hommelhoff

We present an atomic-resolution observation and analysis of graphene constrictions and ribbons with sub-nanometer width. Graphene membranes are studied by imaging side spherical aberration-corrected transmission electron microscopy at 80…

Mesoscale and Nanoscale Physics · Physics 2009-08-20 A. Chuvilin , J. C. Meyer , G. Algara-Siller , U. Kaiser

Atomically precise graphene nanoribbons (GNRs) have emerged as promising candidates for nanoelectronic applications due to their widely tunable energy band gaps resulting from lateral quantum confinement and edge effects. Here we report on…

The hybrid graphene - hexagonal boron nitride (G-hBN) systems offer new routes in the design of nanoscale electronic devices. Using {\it ab initio} density functional theory calculations we investigate the dynamics of zig-zag nanoribbons a…

Materials Science · Physics 2016-09-21 George Alexandru Nemnes , Camelia Visan , Dragos Victor Anghel , Andrei Manolescu

Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that…

Quantum Physics · Physics 2009-11-13 Alexey Kalachev , Stefan Kroll

We measure molecular vibrations with femtometer precision using time-resolved x-ray absorption spectroscopy. For a demonstration, a Raman process excites the A$_{1g}$ mode in gas-phase SF$_6$ molecules with an amplitude of $\approx50$ fm,…

We present the results of an experimental and numerical investigation into temporally non-local coherent interactions between ultrashort pulses, mediated by Raman coherence, in gas-filled kagom\'{e}-style hollow-core photonic crystal fiber.…

We present a new general design approach of a broad-band detector of gravitational radiation that relies on two atom interferometers separated by a distance L. In this scheme, only one arm and one laser will be used for operating the two…

General Relativity and Quantum Cosmology · Physics 2015-05-18 Nan Yu , Massimo Tinto

Materials and devices used in space and advanced energy systems are continuously exposed to high-energy photons and particles, leading to gradual changes in their structural and electronic properties. Gamma-ray exposure is particularly…

We have generated and detected the radial-breathing mode of coherent lattice vibrations in single-walled carbon nanotubes using ultrashort laser pulses. Because the band gap is a function of diameter, these diameter oscillations cause…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Y. S. Lim , K. J. Yee , J. H. Kim , J. Shaver , E. H. Haroz , J. Kono , S. K. Doorn , R. H. Hauge , R. E. Smalley

The electronic and optical properties of graphene nanoribbons under uniaxial periodic strain have been explored using various nearest-neighbor hopping patterns. It is found that by properly selecting hopping patterns, momentum-resolved gaps…

Mesoscale and Nanoscale Physics · Physics 2024-11-05 Chunwen Zhang , W. X. Yan

In this paper, we investigate, by molecular dynamics simulations, the mechanical properties of a new carbon nanostructure, termed graphene nanochain, constructed by sewing up pristine or twisted graphene nanoribbons (GNRs) and interlocking…

Materials Science · Physics 2013-11-26 Yongping Zheng , Lanqing Xu , Zheyong Fan , Ning Wei , Zhigao Huang

An intense laser field in the high-frequency regime drives carriers in graphene nanoribbons (GNRs) out of equilibrium and creates topologically-protected edge states. Using Floquet theory on driven GNRs, we calculate the time evolution of…

Mesoscale and Nanoscale Physics · Physics 2017-06-26 Matteo Puviani , Franca Manghi , Andrea Bertoni

Molecular ro-vibronic coherences, joint energy-time distributions of quantum amplitudes, are selectively prepared, manipulated, and imaged in Time-Frequency-Resolved Coherent Anti-Stokes Raman Scattering (TFRCARS) measurements using…

Chemical Physics · Physics 2009-11-07 R. Zadoyan , D. Kohen , D. A. Lidar , V. A. Apkarian

We suggest an all-optical scheme for the storage, retrieval and processing of a single-photon wave packet through its off-resonant Raman interaction with a series of coherent control beams. These control beams, each with distinct carrier…

Quantum Physics · Physics 2016-12-09 Xiwen Zhang , Alexey Kalachev , Philip Hemmer , Olga Kocharovskaya

Surface plasmon, with its unique capability to concentrate light into sub-wavelength volume, has enabled great advances in photon science, ranging from nano-antenna and single-molecule Raman scattering to plasmonic waveguide and…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Jonghwan Kim , Hyungmok Son , David J. Cho , Baisong Geng , Will Regan , Sufei Shi , Kwanpyo Kim , Alex Zettl , Yuen-Ron Shen , Feng Wang

Among their amazing properties, graphene and related low-dimensional materials show quantized charge-density fluctuations--known as plasmons--when exposed to photons or electrons of suitable energies. Graphene nanoribbons offer an enhanced…

Strongly Correlated Electrons · Physics 2016-09-14 Cristian Vacacela Gomes , Michele Pisarra , Mario Gravina , Jose M. Pitarke , Antonello Sindona

Carbon nanoscroll is a unique topologically open configuration of graphene nanoribbon possessing outstanding properties and application perspectives due to its morphology. However molecular dynamics study of nanoscrolls with more than a few…

Mesoscale and Nanoscale Physics · Physics 2015-07-15 Alexander V. Savin , Elena A. Korznikova , Sergey V. Dmitriev

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

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