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The quest for quantum spin liquids has garnered significant attention due to their rich physics and disruptive prospects in quantum communication and computation. Spin-orbit coupling, electron correlation, and structural distortion play…

Strongly Correlated Electrons · Physics 2024-12-24 Deepak K Roy , Mukul Kabir

Quantum spin liquids (QSLs) represent an exotic quantum many-body state characterized by the suppression of long-range magnetic order due to strong quantum fluctuations. The kagome spin-1/2 antiferromagnet (AFM) is a prime candidate for…

Strongly Correlated Electrons · Physics 2024-07-24 S. Suetsugu , T. Asaba , S. Ikemori , Y. Sekino , Y. Kasahara , K. Totsuka , B. Li , Y. Zhao , Y. Li , Y. Kohama , Y. Matsuda

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

$\rm{Sr_2CuTe_{0.5}W_{0.5}O_6}$ is a square-lattice magnet with super-exchange between S=1/2 $\rm{Cu^{2+}}$ spins mediated by randomly distributed Te and W ions. Here, using sub-K temperature and 20 $\rm{\mu}$eV energy resolution neutron…

The honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has recently been proposed as a candidate material for hosting field-induced quantum spin liquid (QSL) behavior. Here, we present a comprehensive thermodynamic study of its low-temperature,…

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

We study excitations in weakly interacting pairs of quantum spin ladders coupled through geometrically frustrated bonds. The ground state is a disordered spin liquid, that at high fields is replaced by an ordered chiral helimagnetic phase.…

Strongly Correlated Electrons · Physics 2015-05-14 A. Zheludev , V. O. Garlea , A. Tsvelik , L. -P. Regnault , K. Habicht , K. Kiefer , B. Roessli

The Kitaev model with an applied magnetic field in the $H||[111]$ direction shows two transitions: from a non-abelian gapped quantum spin liquid (QSL) to a gapless QSL at $H_{c1} \simeq 0.2K$ and a second transition at a higher field…

Strongly Correlated Electrons · Physics 2019-06-11 Niravkumar D. Patel , Nandini Trivedi

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

Quantum spin liquids (QSLs) have become a key area of research in magnetism due to their remarkable properties, such as long-range entanglement, fractional excitations, pinch-point singularities, and topologically protected phenomena. In…

Strongly Correlated Electrons · Physics 2024-08-23 M. G. Gonzalez , V. Noculak , A. Sharma , V. Favre , J-R. Soh , A. Magrez , R. Bewley , H. O. Jeschke , J. Reuther , H. M. Rønnow , Y. Iqbal , I. Živković

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

YbZn$_2$GaO$_5$ is a promising candidate for realizing a quantum spin liquid (QSL) state, particularly owing to its lack of significant site disorder. Pulsed-field magnetometry at 0.5 K shows magnetization saturating near 15 T, with a…

Thermal signatures of fractionalized excitations are a fingerprint of quantum spin liquids (QSLs). In the $J_{eff}=1/2$ honeycomb magnet $\alpha$-RuCl$_3$, a QSL state emerges upon applying an in-plane magnetic field $H_{||}$ greater than…

Strongly Correlated Electrons · Physics 2022-06-01 J. A. N. Bruin , R. R. Claus , Y. Matsumoto , N. Kurita , H. Tanaka , H. Takagi

We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional…

A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

We have investigated the origin of the magnetic dipole correlations $\langle \sigma_{\boldsymbol{Q}}^z \sigma_{\boldsymbol{-Q}}^z \rangle$ characterized by the modulation wave vector $\boldsymbol{k} \sim…

Strongly Correlated Electrons · Physics 2022-02-09 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura

The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Remarkably, the spin ices provide one of very few…

Strongly Correlated Electrons · Physics 2014-07-29 Michel J. P. Gingras , Paul A. McClarty

Motivated by the recent synthesis of the spin-1 A-site spinel NiRh$_{\text 2}$O$_{\text 4}$, we investigate the classical to quantum crossover of a frustrated $J_1$-$J_2$ Heisenberg model on the diamond lattice upon varying the spin length…

Strongly Correlated Electrons · Physics 2018-02-01 Finn Lasse Buessen , Max Hering , Johannes Reuther , Simon Trebst

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…