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High temperature one-dimensional (1D) ferromagnetic (FM) chains in Ca3Co2O6 spin system are subjected to a magnetic field and temperature induced first order phase transition (FOPT) to 3D ferrimagnetic (FIM) ground state with decrease in…

Strongly Correlated Electrons · Physics 2026-04-29 Santanu De , V. R. Reddy , A. Banerjee

Alloyed MnxZn1_xPS3 samples have been grown covering the whole compositional range and studied by means of Raman spectroscopy at temperatures covering from 4K up to 850K. Our results, supported by SQUID magnetic measurements, allowed, from…

We investigate the electronic and magnetic properties as well as lattice dynamics and spin-phonon coupling of $\beta$-Na$_{0.33}$V$_2$O$_5$ using temperature-dependent Raman scattering, dc-magnetization and dc-resistivity, x-ray…

Materials Science · Physics 2022-11-23 Rishabh Shukla , Clemens Ulrich , R. S. Dhaka

Modeling spin-wave (magnon) dynamics in novel materials is important to advance spintronics and spin-based quantum technologies. The interactions between magnons and lattice vibrations (phonons) limit the length scale for magnon transport.…

Spin-phonon coupling effects, as reflected in phonon frequency shifts between ferromagnetic (FM) and G-type antiferromagnetic (AFM) configurations in cubic CaMnO$_3$, SrMnO$_3$, BaMnO$_3$, LaCrO$_3$, LaFeO$_3$ and La$_2$(CrFe)O$_6$, are…

Strongly Correlated Electrons · Physics 2012-11-20 Jiawang Hong , Alessandro Stroppa , Jorge Íñiguez , Silvia Picozzi , David Vanderbilt

We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman…

Strongly Correlated Electrons · Physics 2018-11-13 M. Cazayous , A. Sacuto , D. Lebeugle , D. Colson

We have measured polarized Raman scattering spectra of the Fe$_{1-x}$Co$_{x}$Sb$_{2}$ and Fe$_{1-x}$Cr$_{x}$Sb$_{2}$ (0$\leq x\leq $0.5) single crystals in the temperature range between 15 K and 300 K. The highest energy $B_{1g}$ symmetry…

Strongly Correlated Electrons · Physics 2016-09-20 N. Lazarević , Z. V. Popović , Rongwei Hu , C. Petrovic

Weak antiferromagnetic (AF) interaction in the ferromagnetic (FM) partially ordered La2CoMnO6 (LCMO) was detected by Raman spectroscopy by monitoring spin-phonon coupling. Because of the sensibility to probe short-range disorder and lattice…

Materials Science · Physics 2022-05-17 R. X. Silva , C. C. Santos , H. Reichlova , X. Marti , R. Paniago , C. W. A. Paschoal

The semimetal NbIrTe4 has been proposed to be a Type-II Weyl semimetal with 8 pairs of opposite Chirality Weyl nodes which are very close to the Fermi energy. This topological electronic structure is made possible because of the broken…

Spin-charge-lattice coupling mediated by multi-magnon processes is demonstrated in multiferroic BiFeO3. Experimental evidence of two and three magnons excitations as well as multimagnon coupling at electronic energy scales and high…

We study an extended model to describe the spin-lattice coupling, incorporating individual vibrations of bonds and atomic sites alongside distance-dependent exchange interactions. The proposed spin Hamiltonian can be effectively considered…

Strongly Correlated Electrons · Physics 2026-03-10 Masaki Gen , Hidemaro Suwa , Shusaku Imajo , Chao Dong , Hiroaki Ueda , Makoto Tachibana , Akihiko Ikeda , Koichi Kindo , Yoshimitsu Kohama

Electron-phonon interactions (EPIs) represent a fundamental cornerstone of condensed matter physics, commanding persistent attention due to their pivotal role in driving novel quantum phenomena within low-dimensional materials. Here, we…

Spin wave resonances with enormously large wave numbers corresponding to wave vectors 10^5-10^6 cm^{-1} are observed in thin plates of FeBO3. The study of spin wave resonances allows one to obtain information about the spin wave spectrum.…

Strongly Correlated Electrons · Physics 2011-03-03 H. -A. Krug von Nidda , L. E. Svistov , L. A. Prozorova

Polarized Raman scattering spectra of the K_xCo_{2-y}Se_2 single crystals reveal the presence of two phonon modes, assigned as of the A_{1g} and B_{1g} symmetry. Absence of additional modes excludes the possibility of vacancy ordering,…

We report results of Raman scattering experiments on twin-free BaFe$_{2}$As$_{2}$ with the main focus placed on understanding the influence of electronic and spin degrees of freedom on the lattice dynamics. In particular, we scrutinize the…

Strongly Correlated Electrons · Physics 2018-08-15 A. Baum , Ying Li , M. Tomić , N. Lazarević , D. Jost , F. Löffler , B. Muschler , T. Böhm , J. -H. Chu , I. R. Fisher , R. Valentí , I. I. Mazin , R. Hackl

MnV$_2$O$_4$ in the spinel structure is known to exhibit coupled orbital and spin ordering, and its Raman spectra show interesting anomalies in its low-temperature phase. With a goal to explain this behavior involving coupled spins and…

Materials Science · Physics 2020-05-27 Dibyendu Dey , T. Maitra , U. V. Waghmare , A. Taraphder

We have carried out temperature and pressure-dependent Raman and x-ray measurements on single crystals of Tb$_2$Ti$_2$O$_7$. We attribute the observed anomalous temperature dependence of phonons to phonon-phonon anharmonic interactions. The…

We report on the structural and spectroscopic characterization of the multiferroic Fe$_2$Mo$_3$O$_8$. Synchrotron x-ray and neutron diffraction, as well as thermal expansion measurements reveal a lattice anomaly at $T_{\mathrm{N}}\simeq…

Strongly Correlated Electrons · Physics 2020-09-28 S. Reschke , A. A. Tsirlin , N. Khan , L. Prodan , V. Tsurkan , I. Kézsmárki , J. Deisenhofer

Polycrystalline ceramic samples and a single crystal of EuTiO3 have been investigated by Raman spectroscopy in the temperature range 80-300 K. Although synchrotron XRD data clearly indicated the cubic to tetragonal phase transition around…

Materials Science · Physics 2021-04-21 P. Pappas , E. Liarokapis , M. Calamiotou , A. Bussmann-Holder

We performed a Raman scattering study of thin films of LiTi$_2$O$_4$ spinel oxide superconductor. We detected four out of five Raman active modes, with frequencies in good accordance with our first-principles calculations. Three T$_{2g}$…

Superconductivity · Physics 2017-09-13 D. Chen , Y. -L. Jia , T. -T. Zhang , Z. Fang , K. Jin , P. Richard , H. Ding
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