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In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman and dielectric spectroscopic study. Pr$_2$CoMnO$_6$ is a manganite compound , it undergoes a paramagnetic to…

Strongly Correlated Electrons · Physics 2021-04-13 Ilyas Noor Bhatti , Imtiaz Noor Bhatti

Synthetic powder, ore samples and mineral single crystals of goethite ($\alpha-$FeOOH) were investigated with polarized Raman spectroscopy at temperatures from 300 K to 473 K. The symmetry of the vibrational modes, observed in different…

Materials Science · Physics 2020-06-24 M. V. Abrashev , V. G. Ivanov , B. S. Stefanov , N. D. Todorov , J. Rosell , V. Skumryev

Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12…

We report experimental and theoretical studies on the magnetoelastic interactions in MnPS$_3$. Raman scattering response measured as a function of temperature shows a blue shift of the Raman active modes at 120.2 and 155.1 cm$^{-1}$, when…

We report detailed Raman spectroscopic and magnetic susceptibility studies on the spin-driven ferroelectric compounds Mn4Nb2O9 (MNO) and Mn4Ta2O9 (MTO). Both systems exhibit strong spin-phonon coupling below the short-range magnetic…

Materials Science · Physics 2026-02-09 Rajesh Jana , Alka Garg , Rekha Rao , Thomas Meier

We used Raman and terahertz spectroscopies to investigate lattice and magnetic excitations and their cross-coupling in the hexagonal YMnO3 multiferroic. Two phonon modes are strongly affected by the magnetic order. Magnon excitations have…

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

While the vibrational thermodynamics of materials with small anharmonicity at low temperatures has been understood well based on the harmonic phonons approximation; at high temperatures, this understanding must accommodate how phonons…

Materials Science · Physics 2015-10-20 Tian Lan

Two distinct ferromagnetic phases of LaMn$_{0.5}$Co$_{0.5}$O$_{3}$ having monoclinic structure with distinct physical properties have been studied. The ferromagnetic ordering temperature $\textit{T}_{c}$ is found to be different for both…

Strongly Correlated Electrons · Physics 2010-09-08 M. Viswanathan , P. S. Anil Kumar , Venkata Srinu Bhadram , Chandrabhas Narayana , A. K. Bera , S. M. Yusuf

Despite the tremendous progress in spintronic studies of van der Waals (vdW) room-temperature ferromagnet Fe3GaTe2, much less effort has been spent on its lattice dynamics and possible interaction with spintronic degrees of freedom. In this…

Materials Science · Physics 2025-06-12 Xia Chen , Xi Zhang , Wenjie He , Yu Li , Jiating Lu , Dinghua Yang , Deren Li , Li Lei , Yong Peng , Gang Xiang

We present results from light scattering experiments on tetragonal FeS with the focus placed on lattice dynamics. We identify the Raman active A1g and B1g phonon modes, a second order scattering process involving two acoustic phonons, and…

Polarization- and temperature-dependent Raman data along with theoretical simulations are presented for the Kagome ferromagnet Fe_3Sn_2. Eight out of nine expected phonon modes were identified. The experimental energies compare well with…

The quadruple Calcium manganite (CaMn7O12) is a multiferroic material that exhibits a giant magnetically-induced ferroelectric polarization which makes it very interesting for magnetoelectric applications. Here, we report the Raman…

Strongly Correlated Electrons · Physics 2019-01-16 C. Toulouse , C. Martin , M-A. Measson , Y. Gallais , A. Sacuto , M. Cazayous

We use density functional theory (DFT) calculations to study the lattice vibrations and electronic properties of the correlated metal LaNiO$_3$. To characterize the rhombohedral to cubic structural phase transition of perovskite LaNiO$_3$,…

Materials Science · Physics 2011-11-09 Gaoyang Gou , Ilya Grinberg , Andrew M. Rappe , James M. Rondinelli

The vibrational properties of 2H-TaSe$_{2-x}$S$_x$ ($0 \le x \le 2$) single crystals were probed using Raman spectroscopy and density functional theory calculations. The end members revealed two out of four symmetry-predicted Raman active…

One- and multi-phonon excitations of the single crystalline LaCoO3 were studied using Raman spectroscopy in the temperature region of 5 K - 300 K. First-order Raman spectra show a larger number of phonon modes than allowed for the…

Strongly Correlated Electrons · Physics 2022-05-31 V. Gnezdilov , K. -Y. Choi , Yu. Pashkevich , P. Lemmens , S. Shiryaev , G. Bychkov , S. Barilo , V. Fomin , A. V. Yeremenko

The strong coupling between spin, lattice and electronic degrees of freedom in magnetic materials can produce interesting phenomena, including multiferroic and magnetodielectric (MD) behavior, and exotic coupled excitations, such as…

Strongly Correlated Electrons · Physics 2019-05-08 A. Sethi , J. E. Slimak , T. Kolodiazhnyi , S. L. Cooper

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

The spin-phonon coupling in magnetic materials is due to the modulation of the exchange integral by lattice vibrations. BaFe12O19 M-type hexaferrite, which is the most used magnetic material as permanent magnet, transforms into ferromagnet…

Materials Science · Physics 2015-06-22 Flávio M. Silva Júnior , Carlos W. A. Paschoal

BaTiO3 is a classical ferroelectric studied for last one century for its ferroelectric properties. Lattice dynamics of BaTiO3 is crucial as the utility of devices is governed by phonons. In this work, we show that traditional…

Materials Science · Physics 2020-12-24 Vivek Dwij , Binoy Krishna De , Gaurav Sharma , D. K. Shukla , M. K. Gupta , R. Mittal , Vasant Sathe