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Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…

Magnetic proximity effects are crucial ingredients for engineering spintronic, superconducting, and topological phenomena in heterostructures. Such effects are highly sensitive to the interfacial electronic properties, such as electron wave…

Ferromagnetic van der Waals (vdW) insulators are of great scientific interest for their promising applications in spintronics. It has been indicated that in the two materials within this class, CrI$_3$ and VI$_3$, the magnetic ground state,…

Strongly Correlated Electrons · Physics 2020-12-15 Asish K. Kundu , Yu Liu , C. Petrovic , T. Valla

Van der Waals heterostructures have risen as a tunable platform to combine different electronic orders, due to the flexibility in stacking different materials with competing symmetry broken states. Among them, van der Waals ferromagnets…

Superconductivity · Physics 2022-02-09 Faluke Aikebaier , Tero T. Heikkilä , J. L. Lado

The discovery of two-dimensional (2D) systems hosting intrinsic long-range magnetic order represents a seminal addition to the rich physical landscape of van der Waals (vdW) materials. CrI3 has emerged as perhaps the most salient example,…

Recent years have seen a vast increase in research into van der Waals magnetic materials. In many of these systems, magnetism is introduced via light 3\textit{d}-transition metal elements, combined with chalcogenides or halogens. Despite…

Two-dimensional intrinsic ferromagnetic half-metal (HM) are important for the spintronics. Manipulating the interlayer magnetic coupling of van der Waals magnetic materials is an important method to control magnetoelectric properties, which…

Materials Science · Physics 2022-12-26 Zhaoyong Guan , Linhui Lv , Ziyuan An , Yanyan Jiang , Ya Su

Fe3-xGeTe2 is a layered magnetic van der Waals material of interest for both fundamental and applied research. Despite the observation of intriguing physical properties, open questions exist even on the basic features related to magnetism:…

We investigate the temperature-dependent electronic structure of the van der Waals ferromagnet, CrGeTe$_3$. Using angle-resolved photoemission spectroscopy, we identify atomic- and orbital-specific band shifts upon cooling through…

Recent experiments have demonstrated efficient spin transfer across layers in the van der Waals heterostructure composed of WTe2 and Fe3GeTe2, signaling a potential breakthrough in developing all-van der Waals spin-orbit torque devices.…

Materials Science · Physics 2025-11-24 H. L. Ning , M. Q. Dong , X. Zhang , J. S. Huang , B. Liu , Zhi-Xin Guo , Y. Dong

Charge transfer plays a key role at the interfaces of heterostructures, which can affect electronic structures and ultimately the physical properties of the materials. However, charge transfer is difficult to manipulate externally once the…

Materials Science · Physics 2023-02-08 Zi-Ao Wang , Weishan Xue , Faguang Yan , Wenkai Zhu , Yi Liu , Xinhui Zhang , Zhongming Wei , Kai Chang , Zhe Yuan , Kaiyou Wang

Low crystal symmetry of magnetic van der Waals materials naturally promotes spin-orbital complexity unachievable in common magnetic materials used for spin-orbit torque switching. Here, using first-principles methods, we demonstrate that an…

Materials Science · Physics 2022-11-09 Tom G. Saunderson , Dongwook Go , Stefan Blügel , Mathias Kläui , Yuriy Mokrousov

Despite serious effort, the nature of the magnetic interactions and the role of electron-correlation effects in magnetic two-dimensional (2D) van der Waals materials remain elusive. Using CrI$_3$ as a model system, we show that the…

Materials Science · Physics 2021-02-04 Liqin Ke , Mikhail I. Katsnelson

Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

Recently discovered ferromagnetism of the layered van der Waals material VI$_3$ attracts much research attention. Despite substantial progress,in the following important aspects no consensus has been reached: (i) a possible deviation of the…

Materials Science · Physics 2021-07-07 L. M. Sandratskii , K. Carva

Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

Materials Science · Physics 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

We investigate near-Fermi-energy (EF) element-specific electronic and spin states of ferromagnetic van der Waals (vdW) metal Fe5GeTe2. The soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) measurement provides spectroscopic…

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

Materials Science · Physics 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

van der Waals heterostructures consisting of transition metal dichalcogenides (TMDs) and two-dimensional (2D) magnets offer a versatile platform to study the coexistence and transformation of different excitons. By focusing on TMD WSe$_2$…

Materials Science · Physics 2025-09-29 Mushir Thodika , Dimitar Pashov , Igor Zutic , Mark van Schilfgaarde , Swagata Acharya

In this paper we investigate the intercalation effects of Iron (Fe) in the van der Waals gap of Bi$_2$Se$_3$ on the magnetic and transport properties using first-principles band structure estimations combined using dynamical mean-field…

Strongly Correlated Electrons · Physics 2019-12-24 S. Koley , Saurabh Basu
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