Low crystal symmetry of magnetic van der Waals materials naturally promotes spin-orbital complexity unachievable in common magnetic materials used for spin-orbit torque switching. Here, using first-principles methods, we demonstrate that an interplay of spin and orbital degrees of freedom has a profound impact on spin-orbit torques in a prototype van der Waals ferromagnet: Fe3GeTe2 (FGT). While we show that bulk FGT hosts strong "hidden" current-induced torques harvested by each of its layers, we uncover that their origin alternates between the conventional spin flux torque and the so-called orbital torque as the magnetization direction is varied. A drastic difference in the behavior of the two types of torques results in a non-trivial evolution of switching properties with doping. Our findings promote the design of non-equilibrium orbital properties as the guiding mechanism for crafting the properties of spin-orbit torques in layered van der Waals materials.
@article{arxiv.2204.13052,
title = {Hidden interplay of current-induced spin and orbital torques in bulk Fe$_3$GeTe$_2$},
author = {Tom G. Saunderson and Dongwook Go and Stefan Blügel and Mathias Kläui and Yuriy Mokrousov},
journal= {arXiv preprint arXiv:2204.13052},
year = {2022}
}