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Thermal conductivity of aligned polymer molecules can be exceptionally high along the alignment direction due to energy transport through strong covalent bonds. At the same time, it is highly sensitive to molecular conformation, varying by…

Chemical Physics · Physics 2026-04-29 Igor V. Parshin , Igor V. Rubtsov , Alexander L. Burin

Low-temperature magnetization curves and thermodynamics of a spin-1/2 Heisenberg octahedral chain with the intraplaquette and monomer-plaquette interactions are examined within a two-component lattice-gas model of hard-core monomers, which…

Statistical Mechanics · Physics 2018-11-19 Jozef Strecka , Johannes Richter , Oleg Derzhko , Taras Verkholyak , Katarina Karlova

Exchange interactions in spin systems can give rise to quantum entanglement in the ground and thermal states of the systems. In this paper, we consider a spin tetramer, with spins of magnitude 1/2, in which the spins interact via…

Strongly Correlated Electrons · Physics 2007-05-23 Indrani Bose , Amit Tribedi

Star polymer is a typical nonlinear macromolecule possessing special thermodynamic behaviors for the existence of a jointing point. The thermodynamic transitions of a single star polymer are systematically studied with bond fluctuation…

Soft Condensed Matter · Physics 2015-05-27 Zilu Wang , Xuehao He

Coupled, dynamical spin-lattice models provide a unique test ground for simulations investigating the finite-temperature magnetic properties of materials under the direct influence of the lattice vibrations. These models are constructed by…

Statistical Mechanics · Physics 2016-12-28 Dilina Perera , Thomas Vogel , David P. Landau

Despite the long-recognized fact that chemical structure and specific interactions greatly influence the thermodynamic properties of polymer systems, a predictive molecular theory that enables systematically addressing the role of chemical…

Soft Condensed Matter · Physics 2015-06-22 Wen-Sheng Xu , Karl F. Freed

We consider polymers made of magnetic monomers (Ising or Heisenberg-like) in a good solvent. These polymers are modeled as self-avoiding walks on a cubic lattice, and the ferromagnetic interaction between the spins carried by the monomers…

Statistical Mechanics · Physics 2009-10-31 T. Garel , H. Orland , E. Orlandini

We study numerically the tightness of prime flat knots in a model of self-attracting polymers with excluded volume. We find that these knots are localised in the high temperature swollen regime, but become delocalised in the low temperature…

Soft Condensed Matter · Physics 2009-11-07 E. Orlandini , A. L. Stella , C. Vanderzande

Recent advances in Generalized Ensemble simulations and microcanonical analysis allowed the investigation of structural transitions in polymer models over a broad range of local bending and torsion strengths. It is reasonable to argue that…

Soft Condensed Matter · Physics 2022-09-07 B. B. Rodrigues , J. C. S. Rocha , B. V. Costa

Molecular dynamics simulations are used to study the phase behavior of linear multiblock copolymers with two types of monomers, A and B, where the length of the polymer blocks $N_{A}$ and $N_{B}$ ($N_{A}=N_{B}=N$), the number of the blocks…

Soft Condensed Matter · Physics 2011-02-04 Panagiotis E. Theodorakis , Nikolaos G. Fytas

Topological constraints (TCs) between polymers determine the behaviour of complex fluids such as creams, oils and plastics. Most of the polymer solutions used every day life employ linear chains; their behaviour is accurately captured by…

Soft Condensed Matter · Physics 2020-10-07 Fabio Landuzzi , Takenobu Nakamura , Davide Michieletto , Takahiro Sakaue

Hydrodynamic interactions as modeled by Multi-Particle Collision Dynamics can dramatically influence the dynamics of fully flexible, ring-shaped polymers in ways not known for any other polymer architecture or topology. We show that steady…

Soft Condensed Matter · Physics 2019-09-09 M. Liebetreu , C. N. Likos

We present a hybrid quantum-classical simulation of charge-polaron transport in conjugated polymers. The charge, which couples to the angular rotations of the monomers, is modeled via the time-dependent Schr\"odinger equation, while the…

Statistical Mechanics · Physics 2022-01-11 Laszlo Berencei , William Barford , Stephen R. Clark

We study the statistical mechanics of double-stranded semi-flexible polymers using both analytical techniques and simulation. We find a transition at some finite temperature, from a type of short range order to a fundamentally different…

Statistical Mechanics · Physics 2009-10-30 T. B. Liverpool , R. Golestanian , K. Kremer

Using a structure-based coarse-grained model of proteins, we study the mechanism of unfolding of knotted proteins through heating. We find that the dominant mechanisms of unfolding depend on the temperature applied and are generally…

Biomolecules · Quantitative Biology 2017-01-23 Yani Zhao , Mateusz Chwastyk , Marek Cieplak

We study random copolymers consisted of two kinds of monomers with attraction between similar kinds. The mean field analysis of this system indicates a continuous phase transition into a phase with periodic microdomain structure. It is…

Condensed Matter · Physics 2009-10-22 A. M. Gutin , C. D. Sfatos , E. I. Shakhnovich

Stacking interactions in single stranded nucleic acids give rise to configurations of an annealed rod-coil multiblock copolymer. Theoretical analysis identifies the resulting signatures for long homopolynucleotides: A non monotonous…

Biomolecules · Quantitative Biology 2009-11-10 A. Buhot , A. Halperin

Topological constraints can affect both equilibrium and dynamic properties of polymer systems, and can play a role in the organization of chromosomes. Despite many theoretical studies, the effects of topological constraints on the…

Soft Condensed Matter · Physics 2014-12-12 Maxim Imakaev , Konstantin Tchourine , Sergei Nechaev , Leonid Mirny

The coil-globule transition has been studied for A-B copolymer chains both by means of lattice Monte Carlo simulations using bond fluctuation algorithm and by a numerical self-consistent field method. Copolymer chains of fixed length with A…

The viscous flow of polymer chains in dense melts is dominated by topological constraints whenever the single chain contour length, N, becomes larger than the characteristic scale Ne, defining comprehensively the macroscopic rheological…

Soft Condensed Matter · Physics 2023-07-19 Mattia Alberto Ubertini , Angelo Rosa