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In this paper, we investigate the use of variational quantum algorithms for simulating the thermodynamic properties of dinuclear metal complexes. Our study highlights the potential of quantum computing to transform advanced simulations and…

Quantum Physics · Physics 2024-10-28 Ana Clara das Neves Silva , Clebson Cruz

The efficient simulation of complex quantum systems remains a central challenge due to the exponential growth of Hilbert space with system size. Tensor network methods have long been established as powerful approximation schemes, and their…

Computational Physics · Physics 2026-03-16 Min Chen , Minzhao Liu , Changhun Oh , Liang Jiang , Yuri Alexeev , Junyu Liu

Accurate and efficient prediction of electronic wavefunctions is central to ab initio molecular dynamics (AIMD) and electronic structure theory. However, conventional ab initio methods require self-consistent optimization of electronic…

Chemical Physics · Physics 2025-11-12 Yanxian Tao , Lingyun Wan , Xiongzhi Zeng , Yingdi Jin , Jie Liu , Zhenyu Li , Jinlong Yang

We recall theoretical studies on transient transport through interacting mesoscopic systems. It is shown that a generalized master equation (GME) written and solved in terms of many-body states provides the suitable formal framework to…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Valeriu Moldoveanu , Andrei Manolescu , Vidar Gudmundsson

Quantum mechanics/molecular mechanics (QM/MM) molecular dynamics (MD) simulations have been developed to simulate molecular systems, where an explicit description of changes in the electronic structure is necessary. However, QM/MM MD…

Chemical Physics · Physics 2021-04-15 Lennard Böselt , Moritz Thürlemann , Sereina Riniker

We present a quantum-inspired solver for the one-dimensional Gross-Pitaevskii equation in the Quantics Tensor-Train (QTT) representation. By evolving the system entirely within a low-rank tensor manifold, the method sidesteps the memory and…

Quantum algorithms for simulating electronic ground states are slower than popular classical mean-field algorithms such as Hartree-Fock and density functional theory, but offer higher accuracy. Accordingly, quantum computers have been…

Predicting how a material's microscopic structure and dynamics determine its transport properties remains a fundamental challenge. To alleviate this task's often prohibitive computational expense, we propose a Mori-based generalized quantum…

Chemical Physics · Physics 2024-05-06 Srijan Bhattacharyya , Thomas Sayer , Andrés Montoya-Castillo

We study information storage in noisy quantum registers and computers using the methods of statistical dynamics. We develop the concept of a strictly contractive quantum channel in order to construct mathematical models of physically…

Quantum Physics · Physics 2009-09-29 Maxim Raginsky

Quantum machine learning could possibly become a valuable alternative to classical machine learning for applications in High Energy Physics by offering computational speed-ups. In this study, we employ a support vector machine with a…

The time-convolutionless (TCL) quantum master equation provides a powerful tool to simulate reduced dynamics of a quantum system coupled to a bath. The key quantity in the TCL master equation is the so-called kernel or generator, which…

Quantum Physics · Physics 2018-10-17 Yanying Liu , Yaming Yan , Meng Xu , Kai Song , Qiang Shi

Quantum computers (QC) could harbor the potential to significantly advance materials simulations, particularly at the atomistic scale involving strongly correlated fermionic systems where an accurate description of quantum many-body effects…

Many current problems of interest in quantum non-equilibrium are described by time-local master equations (TLMEs) for the density matrix that are not of the Lindblad form, that is, that are not strictly probability conserving and/or…

Quantum Physics · Physics 2015-03-25 Michael R. Hush , Igor Lesanovsky , Juan P. Garrahan

We present the Tensor Train Multiplication (TTM) algorithm for the elementwise multiplication of two tensor trains with bond dimension $\chi$. The computational complexity and memory requirements of the TTM algorithm scale as $\chi^3$ and…

Computational Physics · Physics 2024-10-30 Alexios A Michailidis , Christian Fenton , Martin Kiffner

Molecular dynamics (MD) simulations employing classical force fields constitute the cornerstone of contemporary atomistic modeling in chemistry, biology, and materials science. However, the predictive power of these simulations is only as…

Chemical Physics · Physics 2018-09-26 Stefan Chmiela , Huziel E. Sauceda , Klaus-Robert Müller , Alexandre Tkatchenko

The construction of the Hamiltonian matrix \textbf{H} is an essential, yet computationally expensive step in \textit{ab-initio} device simulations based on density-functional theory (DFT). In homogeneous structures, the fact that a unit…

Disordered Systems and Neural Networks · Physics 2026-02-03 Chen Hao Xia , Manasa Kaniselvan , Marko Mladenoivić , Mathieu Luisier

Nuclear quantum effects (NQEs) are often central to a predictive understanding of chemical reactions and rates. While their incorporation in gas-phase reactions is well established, studies involving condensed matter often neglect or…

Chemical Physics · Physics 2026-03-12 Jalen Macatangay , Alejandro Strachan

The tensor-train (TT) format is a data-sparse tensor representation commonly used in high dimensional function approximations arising from computational and data sciences. Various sequential and parallel TT decomposition algorithms have…

Numerical Analysis · Mathematics 2025-09-05 Tianyi Shi , Daniel Hayes , Jing-Mei Qiu

Efficient simulations of the dynamics of open systems is of wide importance for quantum science and tech-nology. Here, we introduce a generalization of the transfer-tensor, or discrete-time memory kernel, formalism to multi-time measurement…

Quantum Physics · Physics 2020-11-09 Mathias R. Jørgensen , Felix A. Pollock

Identifying variational wave functions that efficiently parametrize the physically relevant states in the exponentially large Hilbert space is one of the key tasks towards solving the quantum many-body problem. Powerful tools in this…

Quantum Physics · Physics 2019-04-19 Lorenzo Pastori , Raphael Kaubruegger , Jan Carl Budich