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The thermodynamic behavior of collapse transition in a fully flexible coarse-grained model of energy polydisperse polymer (EPP), a statistical model of random heteropolymer, is investigated in an implicit solvent by means of molecular…

Soft Condensed Matter · Physics 2025-03-04 Thoudam Vilip Singh , Lenin S. Shagolsem

The effect of topology on the collapse transition and instantaneous shape of an energy polydisperse polymer (a model heteropolymer) is studied by means of computer simulations. In particular, we consider three different chain topology,…

Soft Condensed Matter · Physics 2022-11-24 Thoudam Vilip Singh , Lenin S. Shagolsem

We investigate the structural and topological properties of hydrophobic homopolymer chains in aqueous solutions using molecular dynamics simulations and circuit topology (CT) analysis. By combining geometric observables, such as radius of…

Soft Condensed Matter · Physics 2026-01-01 Junichi Komatsu , Kenichiro Koga , Jonas Berx

The equilibrium thermodynamic properties of a linear polymer chain confined to a space between two impenetrable walls (lines) at a distance $D$ under various solvent conditions have been studied using series analysis and exact enumeration…

Statistical Mechanics · Physics 2007-05-23 P. K. Mishra , Sanjay Kumar

The coil-globule transition of hetero-polymer chains is studied here. By means of extensive Molecular Dynamics simulations, we show that the transition is directly linked to the complexity of the chain, which depends on the number of…

Soft Condensed Matter · Physics 2022-09-07 Fabrizio Tafuri , Andrea Maria Chiariello

In this paper we summarize some results of our theoretical investigations of helix-coil transition both in single-strand (polypeptides) and two-strand (polynucleotides) macromolecules. The Hamiltonian does not contain any parameter designed…

We present an off-lattice statistical model of a single polymer chain in mixed solvent media. Taking into account a polymer conformational entropy, renormalization of solvent composition near the polymer backbone, the universal…

Soft Condensed Matter · Physics 2016-06-09 Yu. A. Budkov , A. L. Kolesnikov , N. N. Kalikin , M. G. Kiselev

Simulations of five different coarse-grained models of symmetric diblock copolymer melts are compared to demonstrate a universal (i.e., model-independent) dependence of the free energy on the invariant degree of polymerization…

Soft Condensed Matter · Physics 2015-06-18 Jens Glaser , Pavani Medapuram , Thomas M. Beardsley , Mark W. Matsen , David C. Morse

The universality of the swelling of the radius of gyration of a homopolymer relative to its value in the $\theta$ state, independent of polymer-solvent chemistry, in the crossover regime between $\theta$ and athermal solvent conditions, is…

Soft Condensed Matter · Physics 2020-07-03 Aritra Santra , Kiran Kumari , R. Padinhateeri , B. Duenweg , J. Ravi Prakash

Polymers adopt extended coil and compact globule states according to the balance between entropy and interaction energies. The transition of a polymer between an extended coil state and compact globule state can be induced by changing…

Soft Condensed Matter · Physics 2015-10-28 Kenta Odagiri , Kazuhiko Seki

We report dynamic Monte Carlo simulation on conformational transition of H-shaped branched polymers by varying main chain (backbone) and side chain (branch) length. H-shaped polymers in comparison with equivalent linear polymers exhibit a…

Soft Condensed Matter · Physics 2015-06-17 Ashok Kumar Dasmahapatra , Venkata Mahanth Sanka

We present a statistical model of a dilute polymer solution in good solvent in the presence of low-molecular weight cosolvent. We investigate the conformational changes of the polymer induced by a change of the cosolvent concentration and…

Statistical Mechanics · Physics 2014-11-10 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , M. G. Kiselev

We investigate a lattice model of polymers where the nearest-neighbour monomer-monomer interaction strengths differ according to whether the local configurations have so-called ``hydrogen-like'' formations or not. If the interaction…

Soft Condensed Matter · Physics 2009-11-13 J Krawczyk , A L Owczarek , T Prellberg

We present results of Monte Carlo study of the monomer-monomer correlation functions, static structure factor and asphericity characteristics of a single homopolymer in the coil and globular states for three distinct architectures of the…

Soft Condensed Matter · Physics 2009-11-07 Edward G. Timoshenko , Yuri A. Kuznetsov , Ronan Connolly

Contrary to expectations based on Harris' criterion, chain disorder with frustration can modify the universality class of scaling at the theta transition of heteropolymers. This is shown for a model with random two-body potentials in 2D on…

Soft Condensed Matter · Physics 2009-10-31 Pietro Monari , Attilio L. Stella , Carlo Vanderzande , Enzo Orlandini

We study flexible polymer macromolecules in a crowded (porous) environment, modelling them as self-attracting self-avoiding walks (SASAW) on site-diluted percolative lattices in space dimensions d=2, 3. The influence of stretching force on…

Soft Condensed Matter · Physics 2009-12-09 V. Blavatska , W. Janke

The coil-globule transition has been studied for A-B copolymer chains both by means of lattice Monte Carlo simulations using bond fluctuation algorithm and by a numerical self-consistent field method. Copolymer chains of fixed length with A…

We study long polymer chains in a poor solvent, confined to the space between two parallel hard walls. The walls are energetically neutral and pose only a geometric constraint which changes the properties of the coil-globule (or…

Soft Condensed Matter · Physics 2009-11-10 Hsiao-Ping Hsu , Peter Grassberger

Long linear polymers in dilute solutions are known to undergo a collapse transition from a random coil (expand itself) to a compact ball (fold itself up) when the temperature is lowered, or the solvent quality deteriorates. A natural model…

Probability · Mathematics 2015-06-12 Gia Bao Nguyen , Nicolas Petrelis

The coil-globule transition of an isolated polymer has been well established to be a second-order phase transition described by a standard tricritical O(0) field theory. We provide compelling evidence from Monte Carlo simulations in four…

Statistical Mechanics · Physics 2009-10-31 A. L. Owczarek , T. Prellberg
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