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Determining quantum excited states is crucial across physics and chemistry but presents significant challenges for variational methods, primarily due to the need to enforce orthogonality to lower-energy states, often requiring…

Quantum Physics · Physics 2025-05-01 Shi-Xin Zhang , Lei Wang

We compute concurrence, a measure of bipartite entanglement, of the first excited state of the $1$-D Heisenberg frustrated $J_1$-$J_2$ spin-chain and observe a sudden change in the entanglement of the eigen state near the coupling strength…

Quantum Physics · Physics 2021-01-07 George Biswas , Anindya Biswas

We present an implementation of an efficient algorithm for the calculation of the spectrum of one-dimensional quantum systems with periodic boundary conditions. This algorithm is based on a matrix product representation for quantum states…

Statistical Mechanics · Physics 2016-12-05 Michael Weyrauch , Mykhailo V. Rakov

We use the matrix product state formalism to construct stationary scattering states of elementary excitations in generic one-dimensional quantum lattice systems. Our method is applied to the spin-1 Heisenberg antiferromagnet, for which we…

Strongly Correlated Electrons · Physics 2014-07-09 Laurens Vanderstraeten , Jutho Haegeman , Tobias J. Osborne , Frank Verstraete

Systematic properties of the first excited state are presented for various ring sizes and spin quantum numbers which are only partly covered by the theorem of Lieb, Schultz and Mattis. For odd ring sizes the first excited energy eigenvalue…

Materials Science · Physics 2009-10-31 J. Schnack

A variational approach for constructing an effective particle description of the low-energy physics of one-dimensional quantum spin chains is presented. Based on the matrix product state formalism, we compute the one- and two-particle…

Strongly Correlated Electrons · Physics 2015-10-09 Laurens Vanderstraeten , Frank Verstraete , Jutho Haegeman

We consider the preparation of single-spinon wave functions, relevant for one-dimensional $S=1/2$ spin models, in a quantum computer. We adopt the recently proposed ansatz \cite{kulk} for the single-spinon wave function, where a state with…

Quantum Physics · Physics 2025-08-19 D. Faílde , A. Gómez , J. Fernández-Rossier

We have developed an efficient computational method to treat long, one-dimensional systems of strongly-interacting atoms forming self-assembled spin chains. Such systems can be used to realize many spin chain model Hamiltonians tunable by…

Quantum Physics · Physics 2016-04-19 N. J. S. Loft , O. V. Marchukov , D. Petrosyan , N. T. Zinner

Artificial neural networks have been recently introduced as a general ansatz to compactly represent many- body wave functions. In conjunction with Variational Monte Carlo, this ansatz has been applied to find Hamil- tonian ground states and…

Strongly Correlated Electrons · Physics 2018-10-24 Kenny Choo , Giuseppe Carleo , Nicolas Regnault , Titus Neupert

Obtaining accurate ground and low-lying excited states of electronic systems is crucial in a multitude of important applications. One ab initio method for solving the Schr\"odinger equation that scales favorably for large systems is…

Chemical Physics · Physics 2023-01-19 Mike Entwistle , Zeno Schätzle , Paolo A. Erdman , Jan Hermann , Frank Noé

Excited states of molecules lie in the heart of photochemistry and chemical reactions. The recent development in quantum computational chemistry leads to inventions of a variety of algorithms that calculate the excited states of molecules…

Quantum Physics · Physics 2020-11-05 Hiroki Kawai , Yuya O. Nakagawa

The calculation of excited state energies of electronic structure Hamiltonians has many important applications, such as the calculation of optical spectra and reaction rates. While low-depth quantum algorithms, such as the variational…

Quantum Physics · Physics 2019-07-03 Oscar Higgott , Daochen Wang , Stephen Brierley

We provide an intuitive understanding of the collective low-energy spin excitation of the one-dimensional spin-1/2 antiferromagnetic Heisenberg chain, known as the spinon. To this end, we demonstrate how a single spinon can be excited by…

Strongly Correlated Electrons · Physics 2025-06-17 Teresa Kulka , Milosz Panfil , Mona Berciu , Krzysztof Wohlfeld

Quantum-mechanical correlations of interacting fermions result in the emergence of exotic phases. Magnetic phases naturally arise in the Mott-insulator regime of the Fermi-Hubbard model, where charges are localized and the spin degree of…

Mesoscale and Nanoscale Physics · Physics 2021-11-18 C. J. van Diepen , T. -K. Hsiao , U. Mukhopadhyay , C. Reichl , W. Wegscheider , L. M. K. Vandersypen

We propose how to generate genuine multipartite entanglement of electron spin qubits in a chain of quantum dots using the naturally available single-qubit rotations and two-qubit Heisenberg exchange interaction in the system. We show that…

Mesoscale and Nanoscale Physics · Physics 2007-11-14 F. Bodoky , M. Blaauboer

We show that efficient quantum computation is possible using a disordered Heisenberg spin-chain with `always-on' couplings. Such disorder occurs naturally in nanofabricated systems. Considering a simple chain setup, we show that an…

Quantum Physics · Physics 2007-05-23 Chiu Fan Lee , Neil F. Johnson

A method is presented in which the ground-state subspace is projected out of a Hamiltonian representation. As a result of this projection, an effective Hamiltonian is constructed where its ground-state coincides with an excited-state of the…

Quantum Physics · Physics 2023-08-14 P. Jouzdani , S. Bringuier , M. Kostuk

Using an NMR quantum computer, we experimentally simulate the quantum phase transition of a Heisenberg spin chain. The Hamiltonian is generated by a multiple pulse sequence, the nuclear spin system is prepared in its (pseudo-pure) ground…

Quantum Physics · Physics 2009-11-10 Xinhua Peng , Jiangfeng Du , Dieter Suter

We investigate entanglement properties of the excited states of the spin-1/2 Heisenberg (XXX) chain with isotropic antiferromagnetic interactions, by exploiting the Bethe ansatz solution of the model. We consider eigenstates obtained from…

Strongly Correlated Electrons · Physics 2014-10-28 Jan Mölter , Thomas Barthel , Ulrich Schollwöck , Vincenzo Alba

Assemblies of interacting quantum particles often surprise us with properties that are difficult to predict. One of the simplest quantum many-body systems is the spin 1/2 Heisenberg antiferromagnetic chain, a linear array of interacting…

Strongly Correlated Electrons · Physics 2013-07-02 M. Mourigal , M. Enderle , A. Klöpperpieper , J. -S. Caux , A. Stunault , H. M. Rønnow
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