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A complete knowledge of its excitation spectrum could greatly benefit efforts to understand the unusual form of superconductivity occurring in the lightly hole-doped copper-oxides. Here we use tunnelling spectroscopy to measure the T\to 0…

We investigate the relationship between the K-edge fine structure of isolated single-wall carbon nanotubes (SWCNTs) and the Van Hove singularities (VHSs) in the conduction band density of states. To this end, we model X-ray absorption…

Materials Science · Physics 2024-09-27 Martin Unzog , Alexey Tal , Pedro Melo , Ryosuke Senga , Kazu Suenaga , Thomas Pichler , Georg Kresse

Intense few-to-sub-femtosecond soft x-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge…

Chemical Physics · Physics 2023-06-28 Adam E. A. Fouda , Dimitris Koulentianos , Linda Young , Gilles Doumy , Phay J. Ho

Bound electron-hole excitonic states are generally not expected to form with charges of negative effective mass. We identify such excitons in a single layer of the semiconductor WSe2, where they give rise to narrow-band upconverted…

Protein electrostatics tune excitation energies in the Photosystem II reaction center (PSII-RC), yet a fully quantum-mechanical many-body description of how the surrounding protein environment renormalizes excitons has remained…

Chemical Physics · Physics 2026-02-25 Tucker Allen , Barry Y. Li , Nadine C. Bradbury , Daniel Neuhauser

A GW-BSE approximation scheme is assessed by applying it to a model of asymmetric two-dimensional (2D) interacting electron system. The model is assumed to have a parabolic band characterized by two independent effective mass parameters. A…

Materials Science · Physics 2026-05-26 Xiaoguang Wu

Halo effective field theory (Halo-EFT) has proved to be very efficient for describing halo nuclei within models of nuclear reactions. Its order-by-order expansion scheme enables us to single out the structure observables that are probed in…

Nuclear Theory · Physics 2025-07-21 Live-Palm Kubushishi , Pierre Capel

We propose a simple many-body based screening mixing strategy to considerably enhance the performance of the Bethe-Salpeter (BS) approach for prediction of excitation energies of molecular systems. This strategy enables us to nearly…

Chemical Physics · Physics 2017-11-15 Vafa Ziaei , Thomas Bredow

X-ray absorption spectroscopy (XAS) is a powerful experimental tool to probe the local structure in materials with the core hole excitations. Here, the oxygen K-edge XAS spectra of the NaCl solution and pure water are computed by using a…

Materials Science · Physics 2023-11-03 Fujie Tang , Kefeng Shi , Xifan Wu

To study the characteristic features of relativistic bound systems, the Bethe-Salpeter equation (BSE) for two equal mass spin 1/2 particles (like the deuteron) is solved in the cm-frame for a covariant separable interaction kernel. For that…

Nuclear Theory · Physics 2007-05-23 Frieder Kleefeld , Manfred Dillig

Given the growing significance of 2D materials in various optoelectronic applications, it is imperative to have simulation tools that can accurately and efficiently describe electron correlation effects in these systems. Here, we show that…

Strongly Correlated Electrons · Physics 2023-08-14 Oinam Romesh Meitei , Troy Van Voorhis

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

Accurate and efficient calculations of absorption spectra of molecules and materials are essential for the understanding and rational design of broad classes of systems. Solving the Bethe-Salpeter equation (BSE) for electron-hole pairs…

Materials Science · Physics 2021-02-18 Sijia S. Dong , Marco Govoni , Giulia Galli

We present a novel route for attaining unconventional superconductivity (SC) in a strongly correlated system without doping. In a simple model of a correlated band insulator (BI) at half-filling we demonstrate, based on a generalization of…

Superconductivity · Physics 2021-04-29 Anwesha Chattopadhyay , H. R. Krishnamurthy , Arti Garg

Like adiabatic time-dependent density-functional theory (TD-DFT), the Bethe-Salpeter equation (BSE) formalism of many-body perturbation theory, in its static approximation, is "blind" to double (and higher) excitations, which are…

Chemical Physics · Physics 2021-06-14 Enzo Monino , Pierre-François Loos

Charging up the surface of an insulator after beam impact can lead either to reverse sign of field between the surface and collector of electrons for case of thick sample or appearance of very high internal field for thin films. Both…

Accelerator Physics · Physics 2013-02-12 Y. Bozhko , J. Barnard , N. Hilleret

Within a joint experimental and theoretical research project, single photoionization of He-like B$^{3+}$ ions was investigated in the energy range from approximately 250 to 1200~eV. With the parent-ion beam in the experiment containing both…

We present a method for computing optical absorption spectra by means of a Bethe-Salpeter equation approach, which is based on a conserving linear response calculation for electron-hole coherences in the presence of an external…

Materials Science · Physics 2010-12-21 George Pal , Yaroslav Pavlyukh , Wolfgang Hübner , Hans Christian Schneider

We report on the use of the adaptively compressed exchange (ACE) operator to accelerate many-body perturbation theory (MBPT) calculations, including G$_0$W$_0$ and the Bethe Salpeter equation (BSE), for hybrid density functional theory…

Materials Science · Physics 2025-07-17 Victor Wen-zhe Yu , Marco Govoni

The band gaps of a few selected semiconductors/insulators are obtained from the self-consistent solution of the Hedin's equations. Two different schemes to include the vertex corrections are studied: (i) the vertex function of the…

Strongly Correlated Electrons · Physics 2017-05-17 Andrey L. Kutepov