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We present a table-top extreme ultraviolet (XUV) beamline for measuring time- and frequency-resolved XUV excited optical luminescence (XEOL) with additional femtosecond-resolution XUV transient absorption spectroscopy functionality. XUV…

High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…

Optics · Physics 2024-12-10 Qi Zeng , Yimin Deng , Xinyue Yang , Wei Cao , Peixiang Lu

Coherent diffractive imaging of individual free nanoparticles has opened novel routes for the in-situ analysis of their transient structural, optical, and electronic properties. So far, single-shot single-particle diffraction was assumed to…

In the last few decades the development of ultrafast lasers has revolutionized our ability to gain insight into light-matter interactions. The appearance of few-cycle light sources available from the visible to the mid-infrared spectral…

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Advanced three-dimensional manufacturing techniques are triggering new paradigms in the way we design and produce sophisticated parts on demand. Yet, to fully unravel its potential, a few limitations have to be overcome, one of them being…

Applied Physics · Physics 2024-07-01 Enrico Casamenti , Sacha Pollonghini , Yves Bellouard

A novel approach is used to enhance by nearly two orders of magnitude the conversion efficiency of a 125 nm-coherent source, based on four-wave mixing in room-temperature mercury vapor. Saturation issues are observed and discussed.

Optics · Physics 2007-05-23 Sebastien Chenais , Sebastien Forget , Marie-Claude Castex

We demonstrate experimentally the full tunability of a coherent femtosecond source in the whole ultraviolet spectral region. The experiment relies on the technique of high-order harmonic generation driven by a near-infrared parametric laser…

Advancing table-top attosecond sources in brightness and pulse duration is of immense interest and importance for an expanding sphere of applications. Recent theoretical studies [New J. Phys., 22 093030 (2020)] have found that high-order…

Optics · Physics 2022-08-31 V. A. Birulia , M. A. Khokhlova , V. V. Strelkov

We introduce an ultrafast all-optical approach for efficient chiral recognition which relies on the interference between two low-order nonlinear processes which are ubiquitous in nonlinear optics: sum-frequency generation and third-harmonic…

Optics · Physics 2023-06-09 Josh Vogwell , Laura Rego , Olga Smirnova , David Ayuso

A method is proposed for arbitrarily engineering the high-order harmonic generation phase achieved by shaping a laser pulse and employing xuv light or x rays for ionization. This renders the production of bandwidth-limited attosecond pulses…

Atomic Physics · Physics 2011-02-25 Markus C. Kohler , Christoph H. Keitel , Karen Z. Hatsagortsyan

High-harmonic generation (HHG) from a compact, solid-state medium is highly desirable for applications such as coherent attosecond pulse generation and extreme ultra-violet (EUV) spectroscopy, yet the typically weak conversion of pump light…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present…

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

Precise manipulation of fluids and objects on the micro scale is seldom a simple task, but nevertheless crucial for many applications in life sciences and chemical engineering. We present a microfluidic chip fabricated in silicon-glass,…

We study the generation of attosecond XUV pulses via high-order frequency mixing (HFM) of two intense generating fields, and compare this process with the more common high-order harmonic generation (HHG) process. We calculate the…

Optics · Physics 2023-08-07 V. A. Birulia , M. A. Khokhlova , V. V. Strelkov

Extreme ultraviolet (EUV) coherent sources below 120nm are of paramount significance for promoting next-generation nano-scale lithography,precision spectroscopy, and exploring the emerging physical phenomena in quantum materials. Nonlinear…

Optics · Physics 2025-08-08 Yanling Cheng , Bin Zhang , Fei Liang , Haohai Yu , Huaijin Zhang

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev

The use of UV light sources is highly relevant in many fields of science, being directly related to all those detection and diagnosis procedures which are based on fluorescence spectroscopy. Depending on the specific application, UV…

Materials Science · Physics 2015-11-17 Giovanni Morello , Rita Manco , Maria Moffa , Luana Persano , Andrea Camposeo , Dario Pisignano