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Deuteronium jarosite, (D_3O)Fe_3(SO_4)_2(OD)_6, contains a kagome lattice of Heisenberg spins, S=5/2, with a coverage of 97+-1%. DC and AC susceptibility measurements show strong in-plane antiferromagnetic exchange (\theta_CW=-1500+-300K)…

Condensed Matter · Physics 2007-05-23 A. S. Wills , A Harrison , S. A. M. Mentink , T. E. Mason , Z. Tun

We report polarized neutron scattering studies of spin-wave excitations and spin fluctuations in the S=5/2 kagome lattice antiferromagnet KFe3(OH)6(SO4)2 (jarosite). Inelastic polarized neutron scattering measurements at 10 K on a single…

Strongly Correlated Electrons · Physics 2009-08-20 K. Matan , J. S. Helton , D. Grohol , D. G. Nocera , S. Wakimoto , K. Kakurai , Y. S. Lee

We present a detailed study of the magnetic structure and spin waves in the Fe jarosite compound ${\rm KFe_3(SO_4)_2(OH)_6}$ for the most general Hamiltonian involving one- and two-spin interactions which are allowed by symmetry. We compare…

Materials Science · Physics 2009-11-11 T. Yildirim , A. B. Harris

The spin wave excitations of the ideal S=5/2 Kagome lattice antiferromagnet KFe3(OH)6(SO4)2 have been measured using high-resolution inelastic neutron scattering. We directly observe a flat mode which corresponds to a lifted "zero energy…

Strongly Correlated Electrons · Physics 2008-10-31 K. Matan , D. Grohol , D. G. Nocera , T. Yildirim , A. B. Harris , S. H. Lee , S. E. Nagler , Y. S. Lee

We report the study of high quality samples of the frustrated S = 1/2 kagome antiferromagnet vesignieite, Cu3Ba(VO5H)2. Neutron powder diffraction measurements evidence the high quality of the kagome lattice and show no sign of a transition…

A single crystal S=3/2 perfect kagome lattice antiferromagnet $\mathrm{KCr_3(OH)_6(SO_4)_2}$ (Cr-jarosite) has been studied by X-band and high-frequency electron spin resonance (ESR). The g-values perpendicular to the kagome plane (c-axis)…

We have found weak long range antiferromagnetic order in the quasi-two-dimensional insulating oxide $ KCr_3(OD)_6(SO_4)_2$ which contains Cr$^{3+}$ S=3/2 ions on a kagom\'{e} lattice. In a sample with $\approx$ 76% occupancy of the chromium…

Strongly Correlated Electrons · Physics 2009-10-30 S. -H. Lee , C. Broholm , M. F. Collins , L. Heller , A. P. Ramirez , C. Kloc , E. Bucher , R. W. Erwin , N. Lacevic

We report $^{35}$Cl NMR, ESR, $\mu$SR and specific heat measurements on the $S=1/2$ frustrated kagom\'e magnet kapellasite, $\alpha-$Cu$_3$Zn(OH)$_6$Cl$_2$, where a gapless spin liquid phase is stabilized by a set of competing exchange…

Sr$_2$CuWO$_6$ is a double perovskite proposed to be at the border between two and three dimensional magnetism, with a square lattice of $S=\frac{1}{2}$ Cu$^{2+}$ ions. We have used inelastic neutron scattering to investigate the spin wave…

Strongly Correlated Electrons · Physics 2016-08-24 H. C. Walker , O. Mustonen , S. Vasala , D. T. Adroja , M. Karppinen

We show the structures of magnetic excitations in spin-1/2 kagome-lattice antiferromagnets Cs$_2$Cu$_3$SnF$_{12}$ and Rb$_2$Cu$_3$SnF$_{12}$ investigated by inelastic neutron scattering in wide energy and momentum ranges. For…

Jarosite family compounds, KFe_3(OH)_6(SO_4)_2, (abbreviate Fe jarosite), and KCr_3(OH)_6(SO_4)_2, (Cr jarosite), are typical examples of the Heisenberg antiferromagnet on the kagome lattice and have been investigated by means of…

Materials Science · Physics 2009-10-31 M. Nishiyama , T. Morimoto , S. Maegawa , T. Inami , Y. Oka

It has been known that the spin-wave dispersion, which is usually symmetric in the momentum space with respect to ${\bf q}=0$, can be asymmetric in the presence of the Dzyaloshinskii-Moriya (DM) interaction and an applied magnetic field.…

Strongly Correlated Electrons · Physics 2025-04-16 Kazushi Aoyama , Hikaru Kawamura

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We present a $^{35}$Cl NMR study for spin $S=1/2$ perfect kagome antiferromagnet Ca-kapellasite (CaCu$_{3}$(OH)$_{6}$Cl$_{2}\cdot$0.6H$_{2}$O) with a magnetic transition at $T^{\ast}=7.2$ K. The static magnetic structure in the ground state…

Strongly Correlated Electrons · Physics 2020-07-01 Y. Ihara , K. Arashima , H. Yoshida , M. Hirata , T. Sasaki

We study the spin dynamics of classical Heisenberg antiferromagnet with nearest neighbor interactions on a quasi-two-dimensional kagome bilayer. This geometrically frustrated lattice consists of two kagome layers connected by a…

Strongly Correlated Electrons · Physics 2021-06-09 Preetha Saha , Depei Zhang , Seung-Hun Lee , Gia-Wei Chern

Using neutrons and x-rays we show the topological kagome antiferromagnet Mn$_3$Sn for $T<285$~K forms a homogeneous spin and charge ordered state comprising a longitudinally polarized spin density wave (SDW) with wavevector…

Strongly Correlated Electrons · Physics 2024-07-23 Y. Chen , J. Gaudet , G. G. Marcus , T. Nomoto , T. Chen , T. Tomita , M. Ikhlas , H. S. Suzuki , Y. Zhao , W. C. Chen , J. Strempfer , R. Arita , S. Nakatsuji , C. Broholm

Magnetic excitations in the spin-$\frac{1}{2}$ distorted kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$, which has an ordered ground state owing to the strong Dzyaloshinskii-Moriya interaction, were studied using inelastic neutron…

Strongly Correlated Electrons · Physics 2017-02-17 T. Ono , K. Matan , Y. Nambu , T. J. Sato , K. Katayama , S. Hirata , H. Tanaka

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K2Co(SeO3)2. Despite the presence of quasi-2D "supersolid" magnetic order, the…

Strongly Correlated Electrons · Physics 2024-11-04 M. Zhu , V. Romerio , N. Steiger , S. D. Nabi , N. Murai , S. Ohira-Kawamura , K. Yu. Povarov , Y. Skourski , R. Sibille , L. Keller , Z. Yan , S. Gvasaliya , A. Zheludev

The spin-$\frac{1}{2}$ kagome antiferromagnet is an archetypal frustrated system predicted to host a variety of exotic magnetic states. We show using neutron scattering measurements that deuterated vesignieite…

Strongly Correlated Electrons · Physics 2018-09-12 D. Boldrin , B. Fåk , E. Canévet , J. Ollivier , H. C. Walker , P. Manuel , D. Khalyavin , A. S. Wills

We study ground state degeneracy and spin-wave excitations in a 1D version of a Kagome antiferromagnet -- a Heisenberg antiferromagnet on a Kagome stripe. We show that for nearest-neighbor interaction, the classical ground state is…

Strongly Correlated Electrons · Physics 2009-11-13 A. Donkov , A. V. Chubukov
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