English

Intertwined Charge and Spin Density Waves in a Topological Kagome Material

Strongly Correlated Electrons 2024-07-23 v3

Abstract

Using neutrons and x-rays we show the topological kagome antiferromagnet Mn3_3Sn for T<285T<285~K forms a homogeneous spin and charge ordered state comprising a longitudinally polarized spin density wave (SDW) with wavevector kβ=kβc^\textbf{k}_{\beta}=k_\beta {\bf \hat{c}}, a helical modulated version of the room temperature anti-chiral magnetic order with kχ=kχc^\textbf{k}_{\chi}=k_\chi{\bf \hat{c}}, and charge density waves with wave vectors 2kβ,2kχ2\textbf{k}_\beta, 2\textbf{k}_\chi, and kβ+kχ\textbf{k}_\beta+\textbf{k}_\chi. Though kχ\textbf{k}_{\chi} and kβ\textbf{k}_\beta coincide for 200 K<T<230200~{\rm K}<T<230~K, they exhibit distinct continuous TT-dependencies before locking to commensurate values of kβ=112c\textbf{k}_{\beta} = \frac{1}{12}\textbf{c}^{*} and kχ=548c\textbf{k}_{\chi} = \frac{5}{48}\textbf{c}^{*} at lowT-T. Density functional theory indicates this complex modulated state may be associated with the nesting of Fermi surfaces from correlated flat kagome bands, which host Weyl nodes that are annihilated as it forms.

Keywords

Cite

@article{arxiv.2306.07822,
  title  = {Intertwined Charge and Spin Density Waves in a Topological Kagome Material},
  author = {Y. Chen and J. Gaudet and G. G. Marcus and T. Nomoto and T. Chen and T. Tomita and M. Ikhlas and H. S. Suzuki and Y. Zhao and W. C. Chen and J. Strempfer and R. Arita and S. Nakatsuji and C. Broholm},
  journal= {arXiv preprint arXiv:2306.07822},
  year   = {2024}
}

Comments

6 pages, 4 figures