Related papers: Simultaneous Enantiomer-Resolved Ramsey Spectrosco…
Chiroptical effects using circularly polarized light produce signals that change sign when switching either molecular handedness (enantiosensitivity) or the light helicity (circular dichroism). Here, we break this…
Precision measurement of magnetic fields is an important goal for fundamental science and practical sensing technology. Sensitive detection of a vector magnetic field is a crucial issue in quantum magnetometry, it remains a challenge to…
We discuss quantum variational optimization of Ramsey interferometry with ensembles of $N$ entangled atoms, and its application to atomic clocks based on a Bayesian approach to phase estimation. We identify best input states and generalized…
We study resonance contrast by a two-step pulse observation method to enhance the frequency stability of coherent population trapping (CPT) atomic clocks. The proposed method is a two-step Raman--Ramsey scheme with low intensity during…
Precision measurements of parity non-conserving (PNC) interactions in atoms, molecules and ions can lead to the discovery of new physics beyond the standard model and understanding of weak-force induced interactions in the nucleus. In this…
This paper reviews the recent results in high-resolution spectroscopy on cold molecules. Laser spectroscopy of cold molecules addresses issues of symmetry violation, like in the search for the electric dipole moment of the electron and the…
The highest precision in direct mass measurements is obtained with Penning trap mass spectrometry. Most experiments use the interconversion of the magnetron and cyclotron motional modes of the stored ion due to excitation by external…
We present a computational investigation of the parity-violating (PV) contributions to the vibrational transitions and nuclear magnetic resonance shieldings of helical osmocene. A number of promising transitions within the spectral window…
We introduce the use of superchiral surface waves for the all-optical separation of chiral compounds. Using a combination of electrodynamics modeling and analytical techniques, we show that the proposed approach provides chiral optical…
Estimating multiple parameters simultaneously is of great importance to measurement science and application. For a single parameter, atomic Ramsey interferometry (or equivalently optical Mach-Zehnder interferometry) is capable of providing…
Traditional Ramsey spectroscopy has the frequency resolution $2\pi/T$, where $T$ is the time separation between two light fields. Using squeezed states and two-atom excitation joint detection, we present a new scheme achieving a higher…
Quantum engineering of time-separated Raman laser pulses in three-level systems is presented to produce an ultra-narrow optical transition in bosonic alkali-earth clocks free from light shifts and with a significantly reduced sensitivity to…
Coherent population trapping (CPT) is a multi-level quantum coherence phenomenon of promising applications in atomic clocks and magnetometers. Particularly, multi-pulse CPT-Ramsey interferometry is a powerful tool for improving the…
Rapid and reliable detection and identification of unknown chemical substances is critical to homeland security. It is challenging to identify chemical components from a wide range of explosives. There are two key steps involved. One is a…
We propose an approach to sensitively probe the chirality of molecules by measuring their coherent optical absorption spectra. It is shown that quantum dynamics of the cyclic three-level chiral molecules driven by appropriately-designed…
Using a Ramsey-type setup, the lambda-doublet transition in the $J=1,\, \Omega=1$ level of the $a^3\Pi$ state of CO was measured to be 394 064 870(10) Hz. In our molecular beam apparatus, a beam of metastable CO is prepared in a single…
The recently introduced synthetic chiral light [D. Ayuso et al, Nat. Photon. 13, 866-871 (2019)] has opened up new opportunities for ultrafast and highly efficient imaging and control of chiral matter. Here we show that the giant…
We propose a novel high resolution microscopy technique for enantio-specific detection of chiral samples down to sub-100 nm size, based on force measurement. We delve into the differential photo-induced optical force exerted on an achiral…
Positronium and muonium, as purely leptonic atoms without internal structure, provide ideal systems for high-precision tests of quantum electrodynamics (QED) and measurements of fundamental constants. However, the high velocities of these…
The low frequency region of the spectrum is a challenging regime for quantum probes. We support the idea that, in this regime, performing Ramsey measurements carefully controlling the time at which each measurement is initiated is an…