Related papers: Simultaneous Enantiomer-Resolved Ramsey Spectrosco…
In optical detection of ultrasound, resonators with high Q-factors are often used to maximize sensitivity. However, in order to perform parallel interrogation, conventional interferometric techniques require an overlap between the resonator…
In phase-contrast magnetic resonance imaging (PC-MRI), the velocity of spins at a voxel is encoded in the image phase. The strength of the velocity encoding gradient offers a trade-off between the velocity-to-noise ratio (VNR) and the…
We investigate the resonant regime of a mesoscopic cavity made of graphene or a doped beam splitter. Using Non-Hermitian Quantum Mechanics, we consider the Bender-Boettcher assumption that a system must obey parity and time reversal…
We investigate Ramsey spectroscopy performed on a synchronized ensemble of two-level atoms. The synchronization is induced by the collective coupling of the atoms to a heavily damped mode of an optical cavity. We show that, in principle,…
Quantum computing, with its potential to enhance various machine learning tasks, allows significant advancements in kernel calculation and model precision. Utilizing the one-class Support Vector Machine alongside a quantum kernel, known for…
The topological response of matter to electromagnetic fields is a property in high demand in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding…
The measurement of circular dichroism (CD) has widely been exploited to distinguish the different enantiomers of chiral structures. It has been applied to natural materials (e.g. molecules) as well as to artificial materials (e.g.…
We study anisotropic undersampling schemes like those used in multi-dimensional NMR spectroscopy and MR imaging, which sample exhaustively in certain time dimensions and randomly in others. Our analysis shows that anisotropic undersampling…
We show that combining vibrational spectroscopy with signal processing can result in a scheme for ultrasensitive detection of molecules. We consider the vibrational spectrum as a signal on the energy axis and apply a matched filter on that…
An analytic gradient approach for the computation of derivatives of parity-violating (PV) potentials with respect to displacements of the nuclei in chiral molecules is described and implemented within a quasirelativistic mean-field…
Here we demonstrate that a term in the nuclear spin Hamiltonian, the antisymmetric \textit{J}-coupling, is fundamentally connected to molecular chirality. We propose and simulate a nuclear magnetic resonance (NMR) experiment to observe this…
Molecules that only differ by their chirality, so called enantiomers, often possess different properties with respect to their biological function. Therefore, the separation of enantiomers presents a prominent challenge in molecular biology…
Parity non-conservation (PNC) due to the weak interaction is predicted to give rise to enantiomer dependent vibrational constants in chiral molecules, but the phenomenon has so far eluded experimental observation. The enhanced sensitivity…
We calculate the eigenstates of a diatomic molecule in a range of model mean-field potentials, and evaluate the evolution of their associated Raman spectra with field strength. We demonstrate that dramatic changes in the appearance of the…
A novel chirped pulse control scheme is presented based on Coherent Anti-Stokes Raman Spectroscopy (C-CARS) aiming at maximizing the vibrational coherence in atoms and molecules. The scheme utilizes chirping of the three incoming pulses,…
An exact generalization of the Ramsey transition probability is derived to improve ultra-high precision measurement and quantum state engineering when a particle is subjected to independently-tailored separated oscillating fields. The…
Pulsed excitation of broad spectra requires very high field strengths if monochromatic pulses are used. If the corresponding high power is not available or not desirable, the pulses can be replaced by suitable low-power pulses that…
High-precision frequency estimation is an ubiquitous issue in fundamental physics and a critical task in spectroscopy. Here, we propose a quantum Ramsey interferometry to realize high-precision frequency estimation in spin-1 Bose-Einstein…
Ramsey spectroscopy in large, dense ensembles of ultra-cold atoms trapped in optical lattices suffers from dipole-dipole interaction induced shifts and collective superradiance limiting its precision and accuracy. We propose a novel…
We conceived a model experiment for a continuous separation strategy of chiral molecules (enantiomers) without the need of any chiral selector structure or derivatization agents: Micro-particles that only differ by their chirality are shown…