Related papers: Simultaneous Enantiomer-Resolved Ramsey Spectrosco…
Exceptional points (EPs) are remarkable spectral degeneracies in a non-Hermitian system's parameter space, where both eigenvalues and eigenstates coalesce. Here, we show that in non-Hermitian molecular chiral systems the position of EPs in…
The second-order nonlinear optical coefficients associated with chirality differ in sign for the two mirror-image forms (enantiomers) of a chiral material. Structures comprised of alternating stacks of the enantiomers can therefore be used…
We show that the position of the exceptional points (EPs) in the parameter space of a chiral molecule coupled to the photoionization continuum by a three-color field is enantiosensitive. Using a minimal model of a three-level system driven…
With their rich electronic, vibrational, rotational and hyperfine structure, molecular systems have the potential to play a decisive role in precision tests of fundamental physics. For example, electroweak nuclear interactions should cause…
We report anomalous circularly polarized Raman spectra of phonons in right- and left-handed quartzes. The phonon branches splitting from the E-mode at a finite wavenumber were found to be chiral with mutually opposite angular momenta. Our…
We devise a perturbation-immune version of Ramsey's method of separated oscillatory fields. Spectroscopy of an atomic clock transition without compromising the clock's accuracy is accomplished by actively balancing the spectroscopic…
A novel approach for the state-specific enantiomeric enrichment and the spatial separation of enantiomers is presented. Our scheme utilizes techniques from strong-field laser physics, specifically an optical centrifuge in conjunction with a…
We develop the method of Ramsey spectroscopy with the use of an additional field compensating the frequency shifts of clock optical transitions. This method in combination with the method of magnetically induced excitation of strongly…
We study a modified Ramsey spectroscopy technique employing slowly decaying states for quantum metrology applications using dense ensembles. While closely positioned atoms exhibit superradiant collective decay and dipole-dipole induced…
With a microwave-regime cyclic three-state configuration, an enantiomer-selective state transfer~(ESST) is carried out through the two-path interference between a direct one-photon coupling and an effective two-photon coupling. The…
Recently, two related three wave mixing experiments have been demonstrated that use allowed rotational transitions to produce a free induction decay signal with an amplitude linearly proportional to the enantiomeric excess of a chiral…
We propose a method to separate enantiomers using parity violation in the Casimir-Polder potential between chiral mirrors and chiral molecules. The proposed setup involves a molecular beam composed of chiral molecules passing through a…
Enantioselective orientation of chiral molecules excited by a shaped picosecond laser pulse and a delayed femtosecond pulse is considered. Using quantum mechanical simulations, we demonstrate a strong field-free enantioselective orientation…
We present a comprehensive study of enantioselective orientation of chiral molecules excited by a pair of delayed cross-polarized femtosecond laser pulses. We show that by optimizing the pulses' parameters, a significant (~ 10%) degree of…
Quantum entanglement is a powerful quantum resource for enhancing measurement precision beyond classical limit. % Here we propose an entanglement-enhanced symmetry-protected destructive many-body Ramsey interferometry for precise parameter…
Probing an atomic resonance without disturbing it is an ubiquitous issue in physics. This problem is critical in high-accuracy spectroscopy or for the next generation of atomic optical clocks. Ultra-high resolution frequency metrology…
When the weak-forces producing parity-violating effects are taken into account, there is a tiny energy difference between the total electronic energies of two enantiomers ($\Delta E_{PV}$), which might be the key to understand the evolution…
The spontaneous emission spectrum of a multi-level atom or molecule with nonreciprocal transition is investigated. It is shown that the nonreciprocal transition can lead to the elimination of a spectral line in the spontaneous emission…
Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…
We proposed a spectroscopic method that extends Ramsey's atomic spectroscopy to detect the transition frequency of a qubit fabricated on a superconducting circuit. The method uses a multi-interval train of qubit biases to implement an…