Related papers: Simultaneous Enantiomer-Resolved Ramsey Spectrosco…
The weak interaction does not conserve parity and therefore induces energy shifts in chiral enantiomers that should in principle be detectable in molecular spectra. Unfortunately, the magnitude of the expected shifts are small and in…
Determination of enantiomeric excess is important and remains challenges. We theoretically propose a new spectroscopic method for this issue based on the chirality-dependent AC Stark effects in cyclic three-level models under the…
Microwave three-wave mixing allows for enantiomer-selective excitation of randomly oriented chiral molecules into rotational states with different energy. The random orientation of molecules is reflected in the degeneracy of the rotational…
Molecular matter-wave interferometry enables novel strategies for manipulating the internal mechanical motion of complex molecules. Here, we show how chiral molecules can be prepared in a quantum superposition of two enantiomers by…
We propose a method for enantio-detection of chiral molecules based on a cavity-molecule system, where the left- and right-handed molecules are coupled with a cavity and two classical light fields to form cyclic three-level models. Via the…
We present a brief review of our progress towards measuring parity violation in heavy-metal chiral complexes using mid-infrared Ramsey interferometry. We discuss our progress addressing the main challenges, including the development of…
We propose a method to realize enantiodiscrimination of chiral molecules based on quantum correlation function in a driven cavity-molecule system, where the chiral molecule is coupled with a quantized cavity field and two classical light…
We investigate enantiodetection for both a single cyclic three-level chiral molecule and finite ensembles of such molecules by monitoring the steady-state intracavity photon number in a cavity-QED platform. Our scheme exploits the intrinsic…
We have extended Ramsey spectroscopy by stepping the probe frequency during the two Ramsey excitation pulses to compensate frequency shifts induced by the excitation itself. This makes precision Ramsey spectroscopy applicable even for…
An interesting class of molecules is that in which the molecules do not possess a stereogenic center but can become chiral due to their spatial arrangement. These molecules can be seen as chiral conformers, whose two non-superimposable…
We solve numerically a kinetic model of chiral polymerization in systems closed to matter and energy flow, paying special emphasis to its ability to amplify the small initial enantiomeric excesses due to the internal and unavoidable…
We derive a pulse-area theorem for a cyclic three-level system, an archetypal model for exploring enantioselective state transfer (ESST) in chiral molecules driven by three linearly polarized microwave pulses. By dividing the closed-loop…
Chiral discrimination that is efficient to tiny amounts of chiral substances, especially at the single-molecule level, is highly demanded. Here, we propose a single-shot nondestructive quantum sensing method addressing such an issue. Our…
We propose an accurate and convenient method to achieve 100\% discrimination of chiral molecules with Lewis-Riesenfeld invariant. By reversely designing the pulse scheme of handed resolution, we obtain the parameters of the three-level…
We prove complete controllability for rotational states of an asymmetric top molecule belonging to degenerate values of the orientational quantum number M. Based on this insight, we construct a pulse sequence that energetically separates…
Fundamental weak interactions have been shown to violate parity in both nuclear and atomic systems. However, observation of parity violation in a molecular system has proven an elusive target. Nuclear spin dependent contributions of the…
We study the enantio-specific state transfer in a four-level model for symmetric-top chiral molecules. Such a model is formed by coupling the electric-dipole transitions among four appropriate working states with three electromagnetic…
We introduce chiral rotational spectroscopy: a new technique that enables the determination of the orientated optical activity pseudotensor components $B_{XX}$, $B_{YY}$ and $B_{ZZ}$ of chiral molecules, in a manner that reveals the…
Ramsey interferometry is a key technique for precision spectroscopy and to probe the coherence of quantum systems. Typically, an interferometer is constructed using two quantum states and involves a time-dependent interaction with two short…
Ramsey interferometry is a widely used tool for precisely measuring transition frequencies between two energy levels of a quantum system, with applications in time-keeping, precision spectroscopy, quantum optics, and quantum information.…