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Coupled cluster theory produced arguably the most widely used high-accuracy computational quantum chemistry methods. Despite the approach's overall great computational success, its mathematical understanding is so far limited to results…

Algebraic Geometry · Mathematics 2024-03-29 Fabian M. Faulstich , Mathias Oster

A simple ``brute-force'' parallelisation procedure for the computational implementation of high-order coupled cluster method (CCM) calculations is presented here. This approach is investigated and illustrated by an application of high-order…

Strongly Correlated Electrons · Physics 2007-05-23 D. J. J. Farnell , R. F. Bishop

The Fermi-Hubbard model is a plausible target to be solved by a quantum computer using the variational quantum eigensolver algorithm. However, problem sizes beyond the reach of classical exact diagonalisation are also beyond the reach of…

Quantum Physics · Physics 2020-06-22 Ashley Montanaro , Stasja Stanisic

In the context of Rydberg anti-blockade, this paper proposes a new scheme for a high-fidelity controlled-unitary gate based on non-adiabatic holonomic quantum computation. Under specific detuning and interaction conditions, the scheme…

Quantum Physics · Physics 2026-03-19 Le-Jiang Yu , Jia Zheng , Kun Pu , Chao Gao

We introduce an efficient method to construct optimal and system adaptive basis sets for use in electronic structure and quantum Monte Carlo calculations. The method is based on an embedding scheme in which a reference atom is singled out…

Strongly Correlated Electrons · Physics 2016-02-02 Sandro Sorella , Nicolas Devaux , Mario Dagrada , Guglielmo Mazzola , Michele Casula

The quantum computing scheme described in Phys. Rev. Lett. 98, 190504 (2007), when viewed as a cluster state computation, features a 3-D cluster state, novel adjustable strength error correction capable of correcting general errors through…

Quantum Physics · Physics 2009-07-16 Austin G. Fowler , Kovid Goyal

The fundamental non-Hermitian nature of the forms of coupled-cluster (CC) theory widely used in quantum chemistry has usually been viewed as a negative, but the present letter shows how this can be used to advantage. Specifically, the…

We present the coherent states of the harmonic oscillator in the framework of the generalized (gravitational) uncertainty principle (GUP). This form of GUP is consistent with various theories of quantum gravity such as string theory, loop…

High Energy Physics - Theory · Physics 2013-03-04 Pouria Pedram

In this paper, we have developed a unitary variant of a double exponential coupled cluster theory, which is capable of mimicking the effects of connected excitations of arbitrarily high rank, using only rank-one and rank-two parametrization…

Chemical Physics · Physics 2022-11-23 Dipanjali Halder , V. S. Prasannaa , Rahul Maitra

Counterdiabatic (CD) protocols enable fast driving of quantum states by invoking an auxiliary adiabatic gauge potential (AGP) that suppresses transitions to excited states throughout the driving process. Usually, the full spectrum of the…

Strongly Correlated Electrons · Physics 2022-11-09 Q Xie , Kazuhiro Seki , Seiji Yunoki

We propose a quantum computer structure based on coupled asymmetric single-electron quantum dots. Adjacent dots are strongly coupled by means of electric dipole-dipole interactions enabling rapid computation rates. Further, the asymmetric…

Quantum Physics · Physics 2009-10-31 G. D. Sanders , K. W. Kim , W. C. Holton

Defining a computational basis of pseudo-number states, we interpret a coherent state of large amplitude, $|\alpha|\gg\frac{d}{2\pi}$, as a qudit --- a $d$-level quantum system --- in a state that is an even superposition of $d$…

Quantum Physics · Physics 2010-12-30 Jaewan Kim , Juhui Lee , Se-Wan Ji , Hyunchul Nha , Petr M. Anisimov , Jonathan P. Dowling

We study the application of various forms of the coupled cluster method to systems with paired fermions. The novel element of the analysis is the study of the breaking and eventual restoration of particle number in the CCM variants. We…

Quantum Physics · Physics 2010-11-24 Chris Snape , Niels R. Walet

The Jastrow-modified antisymmetric geminal power (JAGP) ansatz in Hilbert space successfully overcomes two key failings of other pairing theories, namely a lack of inter-pair correlations and a lack of multiple resonance structures, while…

Strongly Correlated Electrons · Physics 2015-06-17 Eric Neuscamman

We report an experimental realization of one-way quantum computing on a two-photon four-qubit cluster state. This is accomplished by developing a two-photon cluster state source entangled both in polarization and spatial modes. With this…

Quantum Physics · Physics 2012-10-30 Kai Chen , Che-Ming Li , Qiang Zhang , Yu-Ao Chen , Alexander Goebel , Shuai Chen , Alois Mair , Jian-Wei Pan

Attention is focused on antisymmetrized versions of quantum spaces that are of particular importance in physics, i.e. two-dimensional quantum plane, q-deformed Euclidean space in three or four dimensions as well as q-deformed Minkowski…

High Energy Physics - Theory · Physics 2014-11-18 Dzo Mikulovic , Alexander Schmidt , Hartmut Wachter

Simulating quantum many-body systems is a highly demanding task since the required resources grow exponentially with the dimension of the system. In the case of fermionic systems, this is even harder since nonlocal interactions emerge due…

Many quantum algorithms rely on a quality initial state for optimal performance. Preparing an initial state for specific applications can considerably reduce the cost of probabilistic algorithms such as the well studied quantum phase…

Quantum Physics · Physics 2024-12-10 Alexandre Fleury , James Brown , Erika Lloyd , Maritza Hernandez , Isaac H. Kim

The integration of diverse quantum resources and the exploitation of more degrees of freedom provide key operational flexibility for universal fault-tolerant quantum computation. In this work, we propose a flexible…

Quantum Physics · Physics 2026-03-20 Peilin Du , Jing Zhang , Tiancai Zhang , Rongguo Yang , Kui Liu , Jiangrui Gao

The unitary coupled cluster (UCC) approximation is one of the more promising wave-function ans\"atze for electronic structure calculations on quantum computers via the variational quantum eigensolver algorithm. However, for large systems…

Quantum Physics · Physics 2021-09-30 Jia Chen , Hai-Ping Cheng , James K. Freericks