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Nonlinear photoluminescence (N-PL) is a broadband photon emission arising from non-equilibrium electron distribution generated at the surface of metallic nanostructures by an ultrafast pulsed laser illumination. N-PL is sensitive to surface…

Individual monolayers of metal dichalcogenides are atomically thin two-dimensional crystals with attractive physical properties different from their bulk layered counterpart. Here we describe the direct synthesis of WS2 monolayers with…

Metamaterials exhibiting hyperbolic dispersion enable unprecedented control over light-matter interactions, from sub-diffraction imaging to enhanced spontaneous emission. However, conventional plasmonic hyperbolic metamaterials suffer from…

The monolayer transition metal dichalcogenides are an emergent semiconductor platform exhibiting rich excitonic physics with coupled spin-valley degree of freedom and optical addressability. Here, we report a new series of low energy…

Recent advancements in transition metal dichalcogenides (TMDs) have unveiled exceptional optical and electronic characteristics, opened up new opportunities, and provided a unique platform for exploring light-matter interactions under the…

Plasmonic devices, with their ultra-high integration density and data-carrying capacity comparable to optical devices, are currently a hot topic in the field of nanophotonic devices. Photodetectors, non-volatile memories, and ultra-compact…

Optics · Physics 2024-03-12 Xinghui Liu , Kaili Chang , Jiarong Guo , Mengfei Xue , Ran Zhou , Ke Chen , Jianing Chen

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 N. Lundt , A. Maryński , E. Cherotchenko , A. Pant , X. Fan , G. Sęk , S. Tongay , A. V. Kavokin , S. Höfling , C. Schneider

Emerging photo-induced excitonic processes in transition metal dichalcogenide (TMD) heterobilayers, e.g., coupling, dephasing, and energy transfer of intra- and inter-layer excitons, allow new opportunities for ultrathin photonic devices.…

Aluminum, as a metallic material for plasmonics, is of great interest because it extends the applications of surface plasmon resonance into the ultraviolet (UV) region and excels noble metals in the natural abundance, cost and compatibility…

Materials Science · Physics 2014-12-11 Hsuan-Wei Liu , Fan-Cheng Lin , Shi-Wei Lin , Jau-Yang Wu , Sheng-Di Lin , Jer-Shing Huang

Strong-coupling of monolayer metal dichalcogenide semiconductors with light offers encouraging prospects for realistic exciton devices at room temperature. However, the nature of this coupling depends extremely sensitively on the optical…

Localized states in two-dimensional (2D) transition metal dichalcogenides (TMDCs) have been the subject of intense study, driven by potential applications in quantum information science. Despite the rapidly growing knowledge surrounding…

The realization and control of polaritons is of paramount importance in the prospect of novel photonic devices. Here, we investigate the emergence of plasmon-exciton polaritons in hybrid structures consisting of a two-dimensional (2D)…

Mesoscale and Nanoscale Physics · Physics 2018-01-10 P. A. D. Gonçalves , L. P. Bertelsen , Sanshui Xiao , N. Asger Mortensen

We discuss coupling of site-selectively induced quantum emitters in exfoliated monolayers of WSe$_2$ to plasmonic nanostructures. Squared and rectangular gold nanopillars, which are arranged in pitches of \SI{4}{\micro\meter} on the…

One of the most fundamental devices for electronics and optoelectronics is the PN junction, which provides the functional element of diodes, bipolar transistors, photodetectors, LEDs, and solar cells, among many other devices. In…

Mesoscale and Nanoscale Physics · Physics 2014-03-28 Britton W. H. Baugher , Hugh O. H. Churchill , Yafang Yang , Pablo Jarillo-Herrero

Quantum emitters in transition metal dichalcogenides (TMDs) have recently emerged as a promising platform for generating single photons for optical quantum information processing. In this work, we present an approach for deterministically…

Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of…

The unique gate-voltage dependent optical properties of graphene make it a promising electrically-tunable plasmonic material. In this work, we proposed in-situ control of the polarization of nanoantennas by combining plasmonic structures…

Optics · Physics 2018-03-26 Yuwei Qin , Xiaoyan Y. Z. Xiong , Wei E. I. Sha , Li Jun Jiang

We studied multi-exciton dynamics in monolayer WSe2 using nonlinear photoluminescence (PL) spectroscopy and Monte Carlo simulations. We observed strong nonlinear saturation behavior of exciton PL with increasing excitation power density,…

Mesoscale and Nanoscale Physics · Physics 2014-11-05 Shinichiro Mouri , Yuhei Miyauchi , Minglin Toh , Weijie Zhao , Goki Eda , Kazunari Matsuda

Transition-metal dichalcogenides monolayers exhibit strong exciton resonances that enable intense light-matter interactions at room temperature (RT). However, the sensitivity of these materials to the surrounding environment and their…

Coupling single photon emitters to surface plasmons provides a versatile ground for on chip quantum photonics. However, achieving good coupling efficiency requires precise alignment of both the position and dipole orientation of the emitter…