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The number of compact structures of a single condensed polymer (SCP), with similar free energies, grows exponentially with the degree of polymerization. In analogy with structural glasses (SGs), we expect that at low temperatures chain…

Soft Condensed Matter · Physics 2021-04-07 Hyun Woo Cho , Guang Shi , T. R. Kirkpatrick , D. Thirumalai

In order to design tougher materials, it is crucial to understand the relationship between their composition and their resistance to fracture. To this end, we investigate the fracture toughness of usual sodium silicate glasses (NS) and…

Materials Science · Physics 2014-10-14 M. Bauchy , M. J. Abdolhosseini Qomi , C. Bichara , F. -J. Ulm , R. J. -M. Pellenq

The rapid collapse of a polymer, due to external forces or changes in solvent, yields a long-lived `crumpled globule.' The conjectured fractal structure shaped by hierarchical collapse dynamics has proved difficult to establish, even with…

Soft Condensed Matter · Physics 2015-10-07 Guy Bunin , Mehran Kardar

The crazing behavior of polymer nanocomposites formed by blending polymer grafted nanoparticles with an entangled polymer melt is studied by molecular dynamics simulations. We focus on the three key differences in the crazing behavior of a…

Soft Condensed Matter · Physics 2016-10-04 Dong Meng , Sanat K. Kumar , Ting Ge , Mark O. Robbins , Gary S. Grest

Fracture initiation in glassy polymers with no notch is studied together with the evolution at zero stress in the glassy state. Confocal microscopy observations and auto-correlation methods are used to characterize specimens of polymethyl…

Materials Science · Physics 2014-12-02 S. Mbarek , P. Baroni , L. Noirez

Glassy polymers show strain hardening: at constant extensional load, their flow first accelerates, then arrests. Recent experiments under such loading have found this to be accompanied by a striking dip in the segmental relaxation time.…

Soft Condensed Matter · Physics 2015-06-11 S. M. Fielding , R. L. Moorcroft , R. G. Larson , M. E. Cates

We prove that the empirical density of states of quantum spin glasses on arbitrary graphs converges to a normal distribution as long as the maximal degree is negligible compared with the total number of edges. This extends the recent…

Mathematical Physics · Physics 2016-10-25 László Erdős , Dominik Schröder

The dynamic structure factor of semiflexible polymers in solution is derived from the wormlike chain model. Special attention is paid to the rigid constraint of an inextensible contour and to the hydrodynamic interactions. For the cases of…

Soft Condensed Matter · Physics 2009-10-28 Klaus Kroy , Erwin Frey

We describe simulations of the quantum dynamics of a confocal cavity QED system that realizes an intrinsically driven-dissipative spin glass. A close connection between open quantum dynamics and replica symmetry breaking is established, in…

We present an exact and Monte Carlo renormalization group (MCRG) study of semiflexible polymer chains on an infinite family of the plane-filling (PF) fractals. The fractals are compact, that is, their fractal dimension $d_f$ is equal to 2…

Statistical Mechanics · Physics 2013-05-29 Ivan Zivic , Suncica Elezovic-Hadzic , Sava Milosevic

Simulations are used to examine the microscopic origins of strain hardening in polymer glasses. While traditional entropic network models can be fit to the total stress, their underlying assumptions are inconsistent with simulation results.…

Materials Science · Physics 2009-11-13 Robert S. Hoy , Mark O. Robbins

We study snapping and shaky polyhedra which consist of antiprismatic skeletons covered by polyhedral belts composed of triangular faces only. In detail, we generalize Wunderlich's trisymmetric sandglass polyhedron in analogy to the…

Metric Geometry · Mathematics 2022-03-09 Georg Nawratil

We introduce a lattice model of glass transition in polymer globules. This model exhibits a novel scenario of ergodicity breaking in which the disjoint regions of phase space do not arise uniformly, but as small chambers whose number…

Disordered Systems and Neural Networks · Physics 2009-10-31 Rose Du , Alexander Yu. Grosberg , Toyoichi Tanaka , Michael Rubinstein

Unstable systems of fluidized grains in a very-narrow vertical tube can auto-defluidize after some time, the settling particles forming either a glass- or crystal-like structure. We carried out experiments using different polymer spheres,…

Soft Condensed Matter · Physics 2026-03-17 Vinícius Pereira da S. Oliveira , Danilo S. Borges , Erick M. Franklin , Jorge Peixinho

Unlike crystals, glasses age or devitrify over time, reflecting their non-equilibrium nature. This lack of stability is a serious issue in many industrial applications. Here, we show by numerical simulations that the devitrification of…

Soft Condensed Matter · Physics 2021-11-25 Taiki Yanagishima , John Russo , Roel P A Dullens , Hajime Tanaka

Dilute magnetic nanoparticle systems exhibit slow dynamics [1] due to a broad distribution of relaxation times that can be traced to a correspondingly broad distribution of particle sizes [1]. However, at higher concentrations interparticle…

Disordered Systems and Neural Networks · Physics 2007-05-23 Derek Walton

We investigate the properties of the glass phase of a recently introduced spin glass model of soft spins subjected to an anharmonic quartic local potential, which serves as a model of low temperature molecular or soft glasses. We solve the…

Disordered Systems and Neural Networks · Physics 2025-11-11 Giampaolo Folena , Pierfrancesco Urbani

Recent step strain experiments in well-entangled polymeric liquids demonstrated a bulk fracture-like phenomenon. We have studied this instability using a modern version of the Doi-Edwards theory for entangled polymers, and we find close…

Fluid Dynamics · Physics 2015-06-04 Okpeafoh S. Agimelen , Peter D. Olmsted

Plastically deforming crystals exhibit scale-free fluctuations that are similar to those observed in driven disordered elastic systems close to depinning, but the nature of the yielding critical point is still debated. Here, we study the…

Statistical Mechanics · Physics 2018-01-03 Markus Ovaska , Arttu Lehtinen , Mikko J. Alava , Lasse Laurson , Stefano Zapperi

We report observations of unusal \emph{first} plastic events in silica and metallic glasses in the shear startup regime at applied strain two orders of magnitude smaller than yield strain. The (non-Affine) particle displacement field during…