Related papers: Unexpected dipole instabilities in small molecules…
Recent real-time TDDFT calculations have reported an unexpected delayed growth of molecular dipole oscillations some time after an extreme-ultraviolet (XUV) pulse is applied. We show that numerical and analytical arguments suggest that this…
The release of conduction-band electrons from a metal surface by a sub-femtosecond extreme ultraviolet (XUV) pulse, and their propagation through the solid, provokes a dielectric response in the solid that acts back on the photoelectron…
We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…
We observe and control a molecular vibrational wave packet in an electronically excited state of the neutral hydrogen molecule. In an extreme-ultraviolet (XUV) transient-absorption experiment we launch a vibrational wave packet in the $D…
Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…
The goal to control short-wavelength radiation for the investigation and manipulation of ultrafast dynamics in quantum systems coevolves with the growing availability of extreme-ultraviolet (XUV) and x-ray sources from high-harmonic…
The open inner-shell electronic structure of lanthanides with large magnetic moments gives rise to a rich spectrum of transitions available for laser cooling, trapping, and coherent control. Despite this, the large number of ultraviolet…
Ultra-intense lasers that ionize and accelerate electrons in solids to near the speed of light can lead to kinetic instabilities that alter the laser absorption and subsequent electron transport, isochoric heating, and ion acceleration.…
Bare-state population inversion is demonstrated in a two-level system with all dipole matrix elements nonzero. A laser field is resonantly driving the sample whereas a second weaker and lower frequency coherent field additionally pumps it…
We develop a fully quantum mechanical methodology to describe the static properties and the dynamics of a single anharmonic vibrational mode interacting with a quantized infrared cavity field in the strong and ultrastrong coupling regimes.…
We present a novel time- and phase-resolved, background-free scheme to study the extreme ultraviolet dipole emission of a bound electronic wavepacket, without the use of any extreme ultraviolet exciting pulse. Using multiphoton transitions,…
The effect of the dipole-dipole interaction on the far-off-resonance optical dipole trapping scheme is calculated by a mean-field approach. The trapping laser field polarizes the atoms and the accompanying dipole-dipole energy shift deepens…
We show the existence of ultra-long-range giant dipole molecules formed by a neutral alkali ground state atom that is bound to the decentered electronic wave function of a giant dipole atom. The adiabatic potential surfaces emerging from…
An autoionizing resonance in molecular N$_2$ is excited by an ultrashort XUV pulse and probed by a subsequent weak IR pulse, which ionizes the contributing Rydberg states. Time- and angular-resolved photoelectron spectra recorded with a…
A two-dimensional model atom is employed to study the ionization behavior of initially excited atomic states in highly-frequent intense laser pulses beyond the dipole approximation. An additional regime of ionization suppression is found at…
The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…
Collisions of polar $^{1}\Sigma$ state molecules at ultralow energies are considered, within a model that accounts for long-range dipole-dipole interactions, plus rotation of the molecules. We predict a substantial suppression of…
XUV nonlinear spectroscopy has recently discovered that there is more than one collective dipole resonance state in the energy range of the giant dipole resonance (GDR) of atomic Xe. This resonance-state substructure, hidden in the linear…
The role of a large dipole moment in rotating neutral molecules interacting with low-energy electrons is studied using an accurate {\it ab initio} approach accounting for electronic and rotational degrees of freedom. It is found that theory…
We devise an ab initio formalism for the quantum dynamics of Auger decay by laser-dressed atoms which are inner-shell ionized by extreme ultraviolet (XUV) light. The optical dressing laser is assumed to be sufficiently weak such that…