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Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

Mesoscale and Nanoscale Physics · Physics 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

We apply low temperature confocal optical microscopy to spatially resolve, and spectroscopically study a single self assembled quantum dot. By comparing the emission spectra obtained at various excitation levels to a theoretical many body…

Strongly Correlated Electrons · Physics 2009-10-31 E. Dekel , D. Gershoni , E. Ehrenfreund , D. Spektor J. M. Garcia , P. M. Petroff

We study spin dynamics of excitons confined in self-assembled CdSe quantum dots by means of optical orientation in magnetic field. At zero field the exciton emission from QDs populated via LO phonon-assisted absorption shows a circular…

Materials Science · Physics 2015-06-24 S. Mackowski , T. Gurung , H. E. Jackson , L. M. Smith , J. K. Furdyna , M. Dobrowolska

Colloidal Quantum dots (CQDs) are nowadays one of the cornerstones of modern photonics as they have led to the emergence of new optoelectronic and biomedical technologies. However, the full characterization of these quantum emitters is…

We measure the photoluminescence (PL) lifetime, $\tau$, of excitons in colloidal PbSe nanocrystals (NCs) at low temperatures to 270~mK and in high magnetic fields to 15~T. For all NCs (1.3-2.3~nm radii), $\tau$ increases sharply below 10~K…

Mesoscale and Nanoscale Physics · Physics 2010-08-24 R. D. Schaller , S. A. Crooker , D. A. Bussian , J. M. Pietryga , J. Joo , V. I. Klimov

The ability to generate mode-engineered single photons to interface with disparate quantum systems is of importance for building a quantum network. Here we report on the generation of a pulsed, heralded single photon source with a sub-GHz…

We experimentally probe the non-resonant feeding of photons into the optical mode of a two dimensional photonic crystal nanocavity from the discrete emission from a quantum dot. For a strongly coupled system of a single exciton and the…

Mesoscale and Nanoscale Physics · Physics 2011-06-02 A. Laucht , N. Hauke , A. Neumann , T. Günthner , F. Hofbauer , A. Mohtashami , K. Müller , G. Böhm , M. Bichler , M. -C. Amann , M. Kaniber , J. J. Finley

The unique anisotropic properties of colloidal quantum wells (CQWs) make them highly promising as components in nanocrystal-based devices. However, the limited performance of green and blue light-emitting diodes (LEDs) based on CQWs has…

We report an efficient method to observe single photon emissions in monolayer WSe2 by applying hydrostatic pressure. The photoluminescence peaks of typical two-dimensional (2D) excitons show a nearly identical pressure-induced blue-shift,…

Materials Science · Physics 2017-07-05 Yanxia Ye , Xiuming Dou , Kun Ding , Yu Chen , Desheng Jiang , Fuhua Yang , Baoquan Sun

Quantum emitters in hexagonal boron nitride (hBN) have recently emerged as promising bright single photon sources. In this letter we investigate in details their optical properties at cryogenic temperatures. In particular, we perform…

Mesoscale and Nanoscale Physics · Physics 2017-09-27 Bernd Sontheimer , Merle Braun , Niko Nikolay , Nikola Sadzak , Igor Aharonovich , Oliver Benson

We report micro-photoluminescence studies of single GaN/AlN quantum dots grown along the (0001) crystal axis by molecular beam epitaxy on Si(111) substrates. The emission lines exhibit a linear polarization along the growth plane, but with…

Other Condensed Matter · Physics 2008-07-07 Richard Bardoux , Thierry Guillet , B. Gil , P. Lefebvre , T. Bretagnon , T. Taliercio , Sébastien Rousset , F. Semond

Exciton-phonon coupling limits the homogeneous emission linewidth of nanocrystals. Hence, a full understanding of it is crucial. In this work, we statistically investigate exciton-phonon coupling by performing single-particle spectroscopy…

A very long lifetime emission with non-single exponential decay characteristic has been reported for single InAs/GaAs quantum dot (QD) samples, in which there exists a long-lived metastable state in the wetting layer (WL) [ACS Photonics…

The light emission of self-assembled (In,Ga)As/GaAs quantum dots embedded in single GaAs-based micropillars has been studied by time-resolved photoluminescence spectroscopy. The altered spontaneous emission is found to be accompanied by a…

We report on the exciton spin dynamics of nanowire embedded GaN/AlN Quantum Dots (QDs) investigated by time-resolved photoluminescence spectroscopy. Under a linearly polarized quasiresonant excitation we evidence the quenching of the…

Materials Science · Physics 2015-05-28 A. Balocchi , J. Renard , C. T. Nguyen , B. Gayral , T. Amand , H. Mariette , B. Daudin , G. Tourbot , X. Marie

Quantum dots are promising candidates for telecom single photon sources due to their tunable emission across the different low-loss telecommunications bands, making them compatible with existing fiber networks. Their suitability for…

Quantum confinement profoundly affects the properties and interactions of electrons, holes, and excitons in nanomaterials. We apply first-principles calculations to study the effects of extreme quantum confinement on the electronic,…

Materials Science · Physics 2019-10-07 Dylan Bayerl , Emmanouil Kioupakis

Currently, two optical processes are mainly used to realize single photon sources: deterministic transitions in a semiconductor quantum dot (QD) placed in a microcavity and spontaneous frequency down-conversion in materials with intrinsic…

Mesoscale and Nanoscale Physics · Physics 2024-12-02 I. V. Krainov , M. V. Rakhlin , A. I. Veretennikov , T. V. Shubina

The total spontaneous emission rate of a quantum emitter in the presence of an infinite MoS\textsubscript{2} monolayer is enhanced by several orders of magnitude, compared to its free-space value, due to the excitation of surface exciton…

Single dot photoluminescence excitation spectroscopy provides an insight into energy structure of individual quantum dots, energy transfer processes within and between the dots and their surroundings. The access to single dot energy…

Instrumentation and Detectors · Physics 2019-05-10 Paweł Podemski , Aleksander Maryński , Paweł Wyborski , Artem Bercha , Witold Trzeciakowski , Grzegorz Sęk
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