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We describe a new approach to precision NMR with hyperpolarized gases designed to mitigate NMR frequency shifts due to the alkali spin exchange field. The electronic spin polarization of optically pumped alkali atoms is square-wave…

Atomic Physics · Physics 2015-12-23 Anna Korver , Daniel Thrasher , Mike Bulatowicz , Thad Walker

Magnetic field imaging is a valuable resource for signal source localization and characterization. This work reports an optically pumped magnetometer (OPM) based on the free-induction-decay (FID) protocol, that implements microfabricated…

In order to probe the transitions of a nuclear spin $s$ from one of its substate quantum numbers $m$ to another substate $m'$, the experimenter applies a magnetic field ${\bm B}_0$ in some particular direction, such along $\hat{\bm z}$, and…

Quantum Physics · Physics 2022-03-17 Zhichen Liu , Sunghyun Kim , Richard A. Klemm

We present a general theory for using an optically pumped diamond nitrogen-vacancy center as a tunable, non-equilibrium bath to control a variety of nuclear spin dynamics (such as dephasing, relaxation, squeezing, polarization, etc.) and…

Quantum Physics · Physics 2019-08-17 Ping Wang , Jiangfeng Du , Wen Yang

Nuclear Magnetic Resonance (NMR) spans diverse fields from biology to quantum science. Employing NMR on a floating object could unveil novel possibilities beyond conventional operational paradigms. Here, we observe Nuclear Magnetic…

Quantum Physics · Physics 2024-07-30 J. Voisin , A. Durand , T. Copie , M. Perdriat , G. Hétet

In nuclear magnetic resonance (NMR), the bulk magnetization of a sample is commonly assumed to be proportional to spin polarization, with each spin of the same type contributing equally to the measured signal. In this work, we prove the…

Chemical Physics · Physics 2025-06-16 Danila A. Barskiy , Andrey Pravdivtsev

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic…

Characterization of noise of a quantum harmonic oscillator is important for many experimental platforms. We experimentally demonstrate motional spin-locking spectroscopy, a method that allows us to directly measure the motional noise…

The negatively charged boron vacancy center in 2D hexagonal boron nitride has emerged as a promising quantum sensor. However, its sensitivity is constrained due to ubiquitous nuclear spins in the environment. The nuclear spins, hyperfine…

Quantum Physics · Physics 2025-12-23 Basanta Mistri , Saksham Mahajan , Felix Donaldson , Rama K. Kamineni , Siddharth Dhomkar

Alkali-noble-gas comagnetometers have become an essential tool for tests of fundamental physics and offer a compact platform for precision gyroscopy. They are, however, limited by technical noise at low frequencies, commonly due to their…

Quantum Physics · Physics 2025-04-07 Morgan Hedges , Ankit Papneja , Karun Paul , Ben C Buchler

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

The concept of entanglement, in which coherent quantum states become inextricably correlated, has evolved from one of the most startling and controversial outcomes of quantum mechanics to the enabling principle of emerging technologies such…

We propose to implement a solid-state rotation sensor by employing a many-body quantum spin system which takes the advantages of the easy controllability of the electron spin and the robustness provided by the collective nuclear spin state.…

Quantum Physics · Physics 2020-09-16 Wenkui Ding , Wenxian Zhang , Xiaoguang Wang

Coherent oscillations between any two levels from four nuclear spin states of I=3/2 have been demonstrated in a nanometre-scale NMR semiconductor device, where nuclear spins are all-electrically controlled. Using this device, we discuss…

Quantum Physics · Physics 2009-08-04 S. K. Ozdemir , A. Miranowicz , T. Ota , G. Yusa , N. Imoto , Y. Hirayama

The nuclear magnetic resonance (NMR) spectrum of spin-3/2 nuclei in a static magnetic field aligned with one of the electric field gradient (EFG) principal axes is developed analytically, based on fictitious spin-1/2 formalism. Compact…

Superconductivity · Physics 2024-12-17 Jaafar N. Ansari , Karen L. Sauer

A self-oscillating magnetometer based on nonlinear magneto-optical rotation using amplitude-modulated pump light and unmodulated probe light (AM-NMOR) in 87Rb has been constructed and tested towards a goal of airborne detection of magnetic…

Atomic Physics · Physics 2015-05-18 Chris Hovde , Brian Patton , Eric Corsini , James Higbie , Dmitry Budker

We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear…

Mesoscale and Nanoscale Physics · Physics 2008-04-04 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

Atomic magnetometers based on Zeeman shift measurement have the potential for high sensitivity and long-term stability. Like other atomic sensors including atomic clocks and atom interferometers, the atomic magnetometer could in principle…

Quantum Physics · Physics 2025-02-17 Jinyang Li , Gour Pati , Renu Tripathi , Selim M Shahriar

Nuclear spin comagnetometers offer exceptional precision in measurements of spin energy levels and exhibit long-term stability, making them powerful tools for probing spin-dependent physics beyond the Standard Model as well as for inertial…

We report an electronic magnetization measurement of a quantum point contact (QPC) based on nuclear magnetic resonance (NMR) spectroscopy. We find that NMR signals can be detected by measuring the QPC conductance under in-plane magnetic…

Mesoscale and Nanoscale Physics · Physics 2015-07-16 Minoru Kawamura , Keiji Ono , Peter Stano , Kimitoshi Kono , Tomosuke Aono