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Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order…

We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

Materials Science · Physics 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…

The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single…

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

Inversion symmetry eliminates the second-order nonlinear responses in materials commonly used in silicon photonics with electric-dipole approximation. The lack of effective methods to induce the second-order nonlinearity in silicon photonic…

Optics · Physics 2024-05-22 Ru Wang , Yue Dai , Jinsong Cheng , Ruoyu Wang , Xiaoqin Shen

Two-dimensional Transition-Metal Dichalcogenides (TMDs) are of great interest for second harmonic (SH) generation due to their large second-order susceptibility, atomically thin structure, and relaxed phase-matching conditions. TMDs are…

Metasurfaces have long served as a cornerstone technique to enhance nonlinear processes, enabling frequency conversion, efficient light manipulation and integrated photonic devices. However, traditional bulk materials often suffer from high…

The PhD thesis is devoted to the study of second harmonic generation of narrow beams in photonic crystals. The basic idea is that if both frequencies, the fundamental and second harmonics are in the region of self-collimation, then the…

Optics · Physics 2013-11-06 Cristian Nistor

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Tunable biphoton quantum entanglement generated from nonlinear processes is highly desirable for cutting-edge quantum technologies, yet its tunability is substantially constrained by the symmetry of material nonlinear tensors. Here, we…

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

Condensed Matter · Physics 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

The geometric phase is a universal concept in modern physics and has enabled the development of metasurfaces for versatile wavefront shaping. However, its realization in metasurfaces has been restricted to circularly polarized light,…

Optics · Physics 2025-11-11 Yubin Gao , Qikai Chen , Yaoguang Ma

In this work, we utilize thin dielectric meta-atoms placed on a silver substrate to efficiently enhance and manipulate the third harmonic generation. We theoretically and experimentally reveal that when the structural symmetry of the…

Optical systems breaking Lorentz reciprocity have attracted broad attention due to their intriguing physics and applications. Nonreciprocal metasurfaces can enable one-way light transmission and reflection with essential applications in…

Optics · Physics 2024-11-26 Zheng Yang , Wanyue Xiao , Hengzhi Li , Hao Pan , Shubo Wang

We introduce a new mechanism for second-harmonic generation through geometrically rectifying-funneling-ballistic electrons in THz optical resonators. Our resonant rectifiers inherently act as second-order harmonic generators, rectifying…

Mesoscale and Nanoscale Physics · Physics 2025-05-01 Hue T. B. Do , Gregory K. Ngirmang , Wu Lin , Michel Bosman

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

We study the nonlinear process of second harmonic generation in photonic time-crystals, materials with refractive index that varies abruptly and periodically in time, and obtain the phase matching condition for this process. We find…