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This extended article presents a thermomechanical approach for calculating the stress tensor from the thermodynamic potential of inhomogeneous fluids and some applications to ionic fluids. The technique, based on the invariance of the…

Soft Condensed Matter · Physics 2024-12-25 Yu. A. Budkov , N. N. Kalikin , P. E. Brandyshev

Based on the variational field theory framework, we extend our previous mean-field formalism, taking into account the electrostatic correlations of the ions. We employ a general covariant approach and derive a total stress tensor that…

Soft Condensed Matter · Physics 2024-05-09 Yury A. Budkov , Petr E. Brandyshev

In this paper, we present a covariant approach that utilizes Noether's second theorem to derive a symmetric stress tensor from the grand thermodynamic potential functional. We focus on the practical case where the density of the grand…

Statistical Mechanics · Physics 2023-05-17 P. E. Brandyshev , Yu. A. Budkov

The Poisson-Boltzmann mean-field description of ionic solutions has been successfully used in predicting charge distributions and interactions between charged macromolecules. While the electrostatic model of charged fluids, on which the…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Daniel Harries , Rudi Podgornik

Non-local electrostatic interactions associated with the finite solvent size and ion polarizability are investigated within the mean-field linear response theory. To this end, we introduce a field theoretic model of a polar liquid composed…

Soft Condensed Matter · Physics 2015-06-15 Sahin Buyukdagli , Tapio Ala-Nissila

In this paper we propose a nonlinear elasticity model of macromolecular conformational change (deformation) induced by electrostatic forces generated by an implicit solvation model. The Poisson-Boltzmann equation for the electrostatic…

Analysis of PDEs · Mathematics 2010-01-12 Yongcheng Zhou , Michael Holst , James Andrew McCammon

Ionic microgels are soft colloidal particles, composed of crosslinked polymer networks, that ionize and swell when dispersed in a good solvent. Swelling of these permeable, compressible particles involves a balance of electrostatic,…

Soft Condensed Matter · Physics 2020-01-29 Alan R. Denton , Mohammed O. Alziyadi

In this paper, we introduce a statistical field theory that describes the macroscopic mechanical forces in inhomogeneous Coulomb fluids. Our approach employs the generalization of Noether's first theorem for the case of fluctuating order…

Statistical Mechanics · Physics 2023-10-31 P. E. Brandyshev , Yu. A. Budkov

Following the arguments presented by Mansuripur [Opt. Express 16, 14821-14835 (2008)], we suggest a form for the macroscopic electromagnetic stress tensor appropriate for ionized media. The generalized Lorentz force includes the effects of…

Plasma Physics · Physics 2011-04-29 Robert W. Johnson

The description of a conducting medium in thermal equilibrium, such as an electrolyte solution or a plasma, involves nonlinear electrostatics, a subject rarely discussed in the standard electricity and magnetism textbooks. We consider in…

Chemical Physics · Physics 2018-08-01 C. G. Gray , P. J. Stiles

We have developed a molecular mean-field theory -- fourth-order Poisson-Nernst-Planck-Bikerman theory -- for modeling ionic and water flows in biological ion channels by treating ions and water molecules of any volume and shape with…

Soft Condensed Matter · Physics 2020-05-18 Jinn-Liang Liu , Bob Eisenberg

We study the derivation of ion dynamics, namely, the ionic Euler--Poisson system, from kinetic descriptions. The kinetic framework consists of the ionic Vlasov--Poisson equation coupled with either a nonlinear Fokker--Planck operator or a…

Analysis of PDEs · Mathematics 2025-08-13 Young-Pil Choi , Dowan Koo , Sihyun Song

We study theoretically the osmotic pressure of a suspension of charged objects (e.g., colloids, polyelectrolytes, clay platelets, etc.) dialyzed against an electrolyte solution using the cell model and linear Poisson-Boltzmann (PB) theory.…

Soft Condensed Matter · Physics 2009-11-07 Markus Deserno , Hans-Hennig von Grunberg

The properties of ionic solutions between charged surfaces are often studied within the Poisson-Boltzmann framework, by finding the electrostatic potential profile. For example, the osmotic pressure between two charged planar surfaces can…

Soft Condensed Matter · Physics 2022-08-04 Ram M. Adar , David Andelman

In this paper we extend the homogenization results obtained in (G. Allaire, A. Mikeli\'c, A. Piatnitski, J. Math. Phys. 51 (2010), 123103) for a system of partial differential equations describing the transport of a N-component electrolyte…

Analysis of PDEs · Mathematics 2020-09-14 Andro Mikelic , Andrey Piatnitski

The behavior of electrolyte solutions close to a charged surface is studied theoretically. A modified Poisson-Boltzmann equation which takes into account the volume excluded by the ions in addition to the electrostatic interactions is…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland

In aqueous solutions, dissolved ions interact strongly with the surrounding water, thereby modifying the solution properties in an ion-specific manner. These ion-hydration interactions can be accounted for theoretically on a mean-field…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Rudi Podgornik , Daniel Harries

Mobile charge in an electrolytic solution can in principle be represented as the divergence of ionic polarization. After adding explicit solvent polarization a finite volume of electrolyte can then be treated as a composite non-uniform…

Soft Condensed Matter · Physics 2021-03-03 Michiel Sprik

In traditional hydrodynamic theories for ionic fluids, conservation of the mass and linear momentum is not properly taken care of. In this paper, we develop hydrodynamic theories for a viscous, ionic fluid of $N$ ionic species enforcing…

Fluid Dynamics · Physics 2018-11-08 Xiaogang Yang , Yuezheng Gong , Jun Li , Robert S. Eisenberg , Qi Wang

We present a fully analytical integration of the Maxwell stress tensor and derive exact relations for interparticle forces in systems of multiple dielectric spheres immersed in a polarizable ionic solvent, within the framework of the…

Soft Condensed Matter · Physics 2025-12-12 Sergii V. Siryk , Walter Rocchia
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