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Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

The identification of quantum spin liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there are great…

Kitaev exchange, a new paradigm in quantum magnetism research, occurs for 90$^{\circ}$ metal-ligand-metal links, $t_{2g}^5$ transition ions, and sizable spin-orbit coupling. It is being studied in honeycomb compounds but also on triangular…

Strongly Correlated Electrons · Physics 2023-10-11 Pritam Bhattacharyya , Nikolay A. Bogdanov , Satoshi Nishimoto , Stephen D. Wilson , Liviu Hozoi

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

We construct a physically realistic and analytically tractable model for spin-1 systems with orbital degeneracy on the honeycomb lattice, relevant to honeycomb materials with large Hund's and weak spin-orbit couplings, and two electrons in…

Strongly Correlated Electrons · Physics 2026-04-01 Lucile Savary

Recently, realizations of Kitaev physics have been sought in the A2IrO3 family of honeycomb iridates, originating from oxygen-mediated exchange through edge-shared octahedra. However, for the j = 1/2 Mott insulator in these materials…

Strongly Correlated Electrons · Physics 2014-03-18 Jeffrey G. Rau , Eric Kin-Ho Lee , Hae-Young Kee

We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $\beta$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic…

While $U$(1) spin liquids have been extensively studied in both quantum and classical regimes, exact classical $\mathbb{Z}_2$ spin liquids arising from models with nearest-neighbor, bilinear spin interactions are still rare. In this Letter,…

Strongly Correlated Electrons · Physics 2025-03-12 Han Yan , Rico Pohle

We explore a large $N$ generalization of the Kitaev model on the honeycomb lattice with a simple nearest-neighbor interacting Hamiltonian. In particular, we focus on the $\mathbb{Z}_4$ case with isotropic couplings, which is characterized…

Strongly Correlated Electrons · Physics 2025-01-16 Yu-Xin Yang , Meng Cheng , Ji-Yao Chen

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

Strongly Correlated Electrons · Physics 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

Recently, Co-based honeycomb magnets have been proposed as promising candidate materials to host the Kitaev spin liquid state. One of the front-runners is BaCo$_2$(AsO$_4$)$_2$ (BCAO), where it was suggested that the exchange processes…

We investigate the phase diagrams of the spin-orbital $d^9$ Kugel-Khomskii model for a bilayer and a monolayer square lattice using Bethe-Peierls-Weiss method. For a bilayer we obtain valence bond phases with interlayer singlets, with…

Strongly Correlated Electrons · Physics 2022-01-25 Wojciech Brzezicki , Andrzej M. Oleś

We study the effective spin-orbital model for honeycomb-layered transition metal compounds, applying the second-order perturbation theory to the three-orbital Hubbard model with the anisotropic hoppings. This model is reduced to the Kitaev…

Strongly Correlated Electrons · Physics 2018-04-04 Akihisa Koga , Shiryu Nakauchi , Joji Nasu

$\alpha$-RuCl$_3$ has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a…

Strongly Correlated Electrons · Physics 2025-07-15 Jiefu Cen , Hae-Young Kee

The Kitaev spin liquid realizes an emergent static $\mathbb{Z}_2$ gauge field with vison excitations coupled to Majorana fermions. We consider Kitaev models stacked on top of each other, weakly coupled by Heisenberg interaction $\propto…

Strongly Correlated Electrons · Physics 2024-08-20 Aprem P. Joy , Achim Rosch

When spin-orbit-entangled $d$-electrons reside on a honeycomb lattice, rich quantum states are anticipated to emerge, as exemplified by the $d^5$ Kitaev materials. Distinct yet equally intriguing physics may be realized with a $d$-electron…

Recent numerical work (Nature 464, 847 (2010)) indicates the existence of a spin liquid phase (SL) that intervenes between the antiferromagnetic and semimetallic phases of the half filled Hubbard model on a honeycomb lattice. To better…

Strongly Correlated Electrons · Physics 2011-08-18 B. K. Clark , D. A. Abanin , S. L. Sondhi

In the quest for realizations of quantum spin liquids, the exploration of Kitaev materials - spin-orbit entangled Mott insulators with strong bond-directional exchanges - has taken center stage. However, in these materials the local…

Kitaev interactions underlying a quantum spin liquid have been long sought, but experimental data from which their strengths can be determined directly is still lacking. Here, by carrying out inelastic neutron scattering measurements on…

The Kitaev model, characterized by bond-dependent Ising spin interactions among spin-orbit entangled dipole moments in Mott insulators, offered a new approach to quantum spin liquids. Motivated by another type of bond-dependent interaction…

Strongly Correlated Electrons · Physics 2023-03-08 Ahmed Rayyan , Derek Churchill , Hae-Young Kee
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