Related papers: Triplet-Pair Spin Signatures from Macroscopically …
The discovery of noncentrosymmetric superconductors, such as CePt$_3$Si, and chiral superconductors, such as Sr$_2$RuO$_4$, calls for experimental methods to identify the presence of spin-triplet pairing. We here demonstrate a method which…
Singlet fission may boost photovoltaic efficiency [by transforming a singlet exciton into two triplet excitons and thereby doubling the number of excited charge carriers. The primary step of singlet fission is the ultrafast creation of the…
Singlet Fission (SF) into two triplets offers exciting avenues for high-efficiency photovoltaics and optically initializable qubits. While the chemical space of SF chromophores is ever-expanding, the mechanistic details of…
We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…
Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. Such applications require protection of the spin states against quantum decoherence due to interactions with…
We propose a microscopic mechanism for triplet pairing due to spin-orbit-assisted electron interaction with optical phonons in a crystal with a complex unit cell. Using two examples of electrons with symmetric Fermi surfaces in crystals…
Spin-entaglement has been proposed and extensively used in the case of correlated triplet pairs which are intermediate states in singlet fission process in select organic semiconductors. Here, we employ quantum process tomography of…
We report transient electron paramagnetic resonance (trEPR) measurements with sub-microsecond time resolution performed on a P3HT:PCBM blend at low temperature. The trEPR spectrum immediately following photoexcitation reveals signatures of…
Identifying multi-exciton states generated from singlet fission is key to understanding the carrier multiplication process, which presents a strategy for improving the efficiency of photovoltaics and bio-imaging. Broadband optically…
Spin-triplet superconductivity is a condensate of electron pairs with spin-1 and an odd-parity wavefunction. A particularly interesting manifestation of triplet pairing is a chiral p-wave state which is topologically non-trivial and a…
The spin dynamics in two electron double quantum dots embedded in two dimensional electron gas at the interface between SrTiO$_3$ and LaAlO$_3$ is studied by an exact numerical solution of the time-dependent Schr\"odinger equation, in the…
We study the Andreev bound states in a Josephson junction between a singlet and a triplet superconductors. Because of the mismatch in the spin symmetries of pairing, the energies of the spin up and down quasiparticles are generally…
In conventional superconductors, electrons of opposite spins are bound into Cooper pairs. However, when the superconductor is in contact with a non-uniformly ordered ferromagnet, an exotic type of superconductivity can appear at the…
Several recent electron spin resonance studies have observed a quintet multiexciton state during the singlet fission process. Here we provide a general theoretical explanation for the generation of this state by invoking a time-varying…
Spin-triplet superconductivity is an intriguing quantum coherent state with both spin and orbital degrees of freedom, which holds significant potential for future applications in quantum technology. However, how the spin of the triplet…
Singlet fission is a spin-allowed exciton multiplication process in organic semiconductors that converts one spin-singlet exciton to two triplet excitons. It offers the potential to enhance solar energy conversion by circumventing the…
Recent advances in time- and angle-resolved photoemission spectroscopy (tr-ARPES) allow for the probing of multiparticle excited-states in reciprocal space. While neutral two-particle excitations (excitons) have been observed in tr-ARPES,…
We have investigated the proximity effect in superconductor/ferromagnet junctions in a systematic manner to discuss the relationship between the zero-energy peak (ZEP) of the local density of states (LDOS) and spin-triplet odd-frequency…
The increased capabilities of coupling more and more materials through functional interfaces are paving the way to a series of exciting experiments and extremely advanced devices. Here we focus on the capability of magnetically…
Motivated by a recent angle-resolved thermal conductivity experiment that shows a twofold gap symmetry in the high-field and low-temperature C phase in the heavy-fermion superconductor UPt$_3$, we group-theoretically identify the pairing…