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We present a theoretical study of transient absorption and reshaping of extreme ultraviolet (XUV) pulses by helium atoms dressed with a moderately strong infrared (IR) laser field. We formulate the atomic response using both the…

Atomic Physics · Physics 2013-03-25 Mette B. Gaarde , Christian Buth , Jennifer L. Tate , Kenneth J. Schafer

Attosecond streaking is one of the most fundamental processes in attosecond science allowing for a mapping of temporal (i.e. phase) information on the energy domain. We show that on the single-particle level attosecond streaking time shifts…

Attosecond streaking camera is an ex situ technique in which a linearly polarized (LP) XUV attopulse produces an electron wavepacket by photoionization in the presence of an IR femtopulse. By moving the two synchronous oppositely circularly…

Atomic Physics · Physics 2025-11-27 M. A. H. B. Md Yusoff , H. B. Ambalampitiya , J. M. Ngoko Djiokap

The dynamics of autoionizing Rydberg states of oxygen are studied using attosecond transient absorption technique, where extreme ultraviolet (XUV) initiates molecular polarization and near infrared (NIR) pulse perturbs its evolution.…

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…

Atomic Physics · Physics 2015-05-18 C. P. J. Martiny , M. Abu-samha , L. B. Madsen

First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…

Other Condensed Matter · Physics 2015-05-13 C. Lemell , B. Solleder , K. Tokesi , J. Burgdoerfer

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We generalize the one electron attosecond streaking camera to time-resolve the correlated two-electron escape dynamics during a collision process involving a deep core electron. The collision process is triggered by an XUV attosecond pulse…

Atomic Physics · Physics 2010-03-09 A. Emmanouilidou , A. Staudte , P. B. Corkum

To solve the time-dependent Schr\"odinger equation in spatially inhomogeneous pulses of electromagnetic radiation, we propose an iterative semi-classical complex trajectory approach. In numerical applications, we validate this method…

Atomic and Molecular Clusters · Physics 2020-01-29 Jianxiong Li , Uwe Thumm

With the development of laser technology, pulse length enters the optical cycle regime and hence the interaction time between laser pulse and atoms becomes prominent. We investigate this problem in this Letter through the photoelectron…

Optics · Physics 2010-04-13 Yang Xiang , Yueping Niu , Yihong Qi , Shangqing Gong

We present an {\it ab initio} and non-perturbative time-dependent approach to the problem of double ionization of a general atom driven by intense XUV laser pulses. After using a highly flexible $B$-Spline $R$-matrix method to generate…

Atomic Physics · Physics 2016-11-17 Xiaoxu Guan , O Zatsarinny , C J Noble , K Bartschat , B I Schneider

We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared (IR) fields, where the IR…

Atomic Physics · Physics 2024-01-31 Yijie Liao , Edvin Olofsson , Jan Marcus Dahlström , Liang-Wen Pi , Yueming Zhou , Peixiang Lu

The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient…

Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…

We perform numerical simulations for photoionization of the argon atom when exposed to a combined field of an infrared laser (abbreviated IR) and its 13th harmonic (H13) by solving the Time-Dependent Schr\"odinger Equation (TDSE)], noting…

Atomic Physics · Physics 2022-08-26 Soumia Chqondi , Souhaila Chaddou , Abdelkader Makhoute

We present the design, implementation and alignment procedure for a two-stage time delay compensating monochromator. The setup spectrally filters the radiation of a high-order harmonic generation source providing wavelength-selected XUV…

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen