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We propose a method to study the tunneling process by analyzing the time-dependent ionization yield in circularly polarized laser. A numerical calculation shows that for an atom exposed to a long laser pulse, if its initial electronic state…

Atomic Physics · Physics 2016-06-08 MingHu Yuan , PeiPei Xin , TianShu Chu , HongPing Liu

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

We theoretically demonstrate a one-to-one mapping between the direction of electron ionization and the phase delay between a linearly polarized VUV and a circular IR laser pulse. To achieve this, we use an ultrashort VUV pulse that defines…

Atomic Physics · Physics 2022-10-26 M. Mountney , G. P. Katsoulis , S. H. Møller , K. Jana , P. Corkum , A. Emmanouilidou

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

Atomic and Molecular Clusters · Physics 2015-05-20 C. -H. Zhang , U. Thumm

We solve the time-dependent Schr\"odinger equation describing a water molecule driven by a superposition of the XUV and IR pulses typical for a RABBITT experiment. This solution is obtained by a combination of the time-dependent coordinate…

Atomic Physics · Physics 2018-01-17 Vladislav V. Serov , A. S. Kheifets

We propose an attosecond XUV-pump IR-probe photoionization protocol that employs pairs of counter-rotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing direct measurement of ionization phases. The…

Atomic Physics · Physics 2019-10-02 Stefan Donsa , Nicolas Douguet , Joachim Burgdörfer , Iva Březinová , Luca Argenti

We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…

We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…

Atomic Physics · Physics 2020-03-24 Fengzheng Zhu , Genliang Li , Aihua Liu

Light-matter interaction is exploited in spectroscopic techniques to access information about molecular, atomic or nuclear constituents of the sample of interest. While scattered light carries both amplitude and phase information of the…

We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…

We present theoretical studies on real-time probing the electron density evolution of an atom in a strong infrared (IR) laser field with few-cycle near-infrared (NIR) and attosecond extreme-ultraviolet (XUV) pulses. Our results indicate…

Atomic Physics · Physics 2015-06-04 Yunpei Deng , Xinhua Xie

We consider an electron in an atom driven by an infrared (IR) elliptically polarized laser field after its ionization by an ultrashort extreme ultraviolet (XUV) pulse. We find that, regardless of the atom species and the laser ellipticity,…

Atomic Physics · Physics 2021-11-24 Jonathan Dubois , Angel Jorba

Streaked photoelectron emission spectra access the correlated dynamics of photoelectrons and residual target electrons with attosecond temporal resolution. We calculated ab initio single-ionization spectra for photoemission from helium…

Atomic Physics · Physics 2024-09-06 Hongyu Shi , Uwe Thumm

Coherent, broadband pulses of extreme ultraviolet (XUV) light provide a new and exciting tool for exploring attosecond electron dynamics. Using photoelectron streaking, interferometric spectrograms can be generated that contain a wealth of…

Atomic Physics · Physics 2020-08-26 Luca Pedrelli , Phillip D. Keathley , Laura Cattaneo , Franz X. Kärtner , Ursula Keller

Streaked photoemission metrology allows the observation of an apparent relative time delay between the detection of photoelectrons from different initial electronic states. This relative delay is obtained by recording the photoelectron…

Other Condensed Matter · Physics 2015-05-28 Chang-hua Zhang , Uwe Thumm

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

A strong helicity dependence of reconstruction of attosecond bursts by beating of two-photon transitions (RABBITT) with circularly polarized XUV and IR pulses was reported by Han et al. [Nature Physics 19, 230 and arXiv 2302.04137 (2023)].…

Atomic Physics · Physics 2026-03-03 Anatoli Kheifets

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

Using ab-initio non-Born-Oppenheimer simulations, we demonstrate amplification of XUV radiation in a high-harmonic generation type process using the example of the hydrogen molecular ion. A small fraction of the molecules is pumped to a…

Atomic Physics · Physics 2016-03-23 Timm Bredtmann , Szczepan Chelkowski , Andre. D. Bandrauk , Misha Ivanov