Related papers: Did bio-homochirality arise from spin-polarized el…
The homochirality of biomolecules remains one of the outstanding puzzles concerning the beginning of life. Chiral amplification of a randomly perturbed racemic mixture of chiral molecules is a well-accepted prerequisite for all routes to…
Homochirality, i.e. the dominance across all living matter of one enantiomer over the other among chiral molecules, is thought to be a key step in the emergence of life. Building on ideas put forward by Frank and many others, we proposed…
We propose a new mechanism for the achievment of homochirality in life without any autocatalytic production process. Our model consists of a spontaneous production together with a recycling cross inhibition in a closed system. It is shown…
To understand the chirality selection in the biological organic system, a simple lattice model of chemical reaction with molecular diffusion is proposed and studied by Monte Carlo simulations. In addition to a simple stochastic process of…
Biological systems reach hierarchical complexity that has no counterpart outside the realm of biology. Undoubtedly, biological entities obey the fundamental physical laws. Can today's physics provide an explanatory framework for…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
Chirality, handedness, is one of the most fundamental intriguing asymmetries in nature. By definition, chiral objects cannot be superimposed onto each other after mirror reflection operation. Numerous examples of chiral structures can be…
Chiral molecular junctions offer a promising platform for realizing chiral-induced spin selectivity (CISS), where spin filtering occurs without external magnetic fields. Here, we investigate spin transport in such junctions by combining…
Context. Homochirality is a generic and unique property of life on Earth and is considered a universal and agnostic biosignature. Homochirality induces fractional circular polarization in the incident light that it reflects. Because this…
The chirality induced spin selectivity effect remains a challenge to capture with theoretical modeling. While at least a decade was spent on independent electron models, which completely fail to reproduce the experimental results, the…
We study the non-equilibrium dynamics of electron transmission from a straight waveguide to a helix with spin-orbit coupling. Transmission is found to be spin-selective and can lead to large spin polarizations of the itinerant electrons.…
Chiral phases of matter, characterized by a definite handedness, abound in nature, ranging from the crystal structure of quartz to spiraling spin states in helical magnets. In $1T$-TiSe$_2$ a source of chirality has been proposed that…
Chirality manifests across multiple scales, yielding unique phenomena that break mirror symmetry. In chiral materials, unexpectedly large spin-filtering or photogalvanic effects have been observed even in materials composed of light…
We here present a variable-range hopping model to describe the chirality-induced spin selectivity along the DNA double helix. In this model, DNA is considered as a one-dimensional disordered system, where electrons are transported by chiral…
The observed single-handedness of biological amino acids and sugars has long been attributed to autocatalysis. However, the stability of homochiral states in deterministic autocatalytic systems relies on cross inhibition of the two chiral…
A recently proposed model of non-autocatalytic reactions in dipeptide reactions leading to spontaneous symmetry breaking and homochirality is examined. The model is governed by activation, polymerization, epimerization and depolymerization…
Electron chirality has been proposed as a microscopic quantity that characterizes electronic handedness, yet its underlying control parameter has not been clearly identified. Furthermore, its applicability is limited to systems with…
We investigate a geometrically symmetric gold-silicon sphere heterodimer and reveal its extrinsic chiroptical response caused by the interaction with a substrate. The chiroptical response is obtained for oblique incidence owing to the…
Low-energy spin-polarized electrons (SPEs) are thought to cause symmetry breaking and could explain the origin of homochirality of prebiotic molecules such as amino acids and sugars. Here we study the effect of cosmic rays (CRs) on the…
Chirality represents a kind of symmetry breaking characterized by the noncoincidence of an object with its mirror image and has been attracting intense attention in a broad range of scientific areas. The recent realization of spin-orbit…