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Related papers: Nonequilibrium dynamics of $\alpha$-RuCl$_{3}$ -- …

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{\alpha}-RuCl3 is a Kitaev material suggested to be a proximate quantum spin liquid in a certain temperature and magnetic field range. Nonequilibrium measurements of transient dynamics have been proposed to detect fractionalized particles…

Strongly Correlated Electrons · Physics 2024-08-23 Haochen Zhang , Subin Kim , Young-June Kim , Hae-Young Kee , Luyi Yang

Excitation by light pulses enables the manipulation of phases of quantum condensed matter. Here, we photoexcite high-energy holon-doublon pairs as a way to alter the magnetic free energy landscape of the Kitaev-Heisenberg magnet…

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

In a Hubbard model for the Kitaev spin-liquid candidate material $\alpha$-RuCl$_3$ with three $t_{2g}$ orbitals per Ru site, we calculate photoinduced dynamics based on the exact diagonalization method and interpret them with the help of a…

Strongly Correlated Electrons · Physics 2022-09-13 Kenji Yonemitsu

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

Strongly Correlated Electrons · Physics 2017-12-12 P. Lampen-Kelley , A. Banerjee , A. A. Aczel , H. B. Cao , M. B. Stone , C. A. Bridges , J. -Q. Yan , S. E. Nagler , D. Mandrus

$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

We present comprehensive inelastic neutron spectroscopic maps of the magnetic field-induced disordered phase of the Kitaev quantum spin liquid candidate material $\alpha$-RuCl$_3$. For fields along both in-plane high-symmetry directions we…

As one of the most promising Kitaev quantum-spin-liquid (QSL) candidates, $\alpha$-RuCl$_3$ has received a great amount of attention. However, its ground state exhibits a long-range zigzag magnetic order, which defies the QSL phase.…

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

Photoinduced hidden phases are often observed in materials with intertwined orders. Understanding the formation of these non-thermal phases is challenging and requires a resolution of the cooperative interplay between different orders on…

Strongly Correlated Electrons · Physics 2018-11-06 Jiajun Li , Hugo U. R. Strand , Philipp Werner , Martin Eckstein

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction…

The search for hidden orders in photoexcited lattice systems is an active research field driven by experimental reports of light-induced or light-stabilized phases. In this study, we investigate hidden electronic orders in strongly…

Strongly Correlated Electrons · Physics 2024-08-14 Sujay Ray , Philipp Werner

We present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material $\alpha$-RuCl$_3$, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered…

Competition between ordered phases, and their associated phase transitions, are significant in the study of strongly correlated systems. Here we examine one aspect, the nonequilibrium dynamics of a photoexcited Mott-Peierls system, using an…

Strongly Correlated Electrons · Physics 2016-02-26 Yao Wang , Brian Moritz , Cheng-Chien Chen , Chunjing Jia , Michel van Veenendaal , Thomas P. Devereaux

We study the photoinduced ultrafast dynamics in relativistic Mott insulators, i.e., Mott insulators with strong spin-orbit coupling. For this purpose, we consider a minimal one-band Hubbard model on lattices with square and triangular…

Strongly Correlated Electrons · Physics 2020-10-20 Jiajun Li , Nagamalleswararao Dasari , Martin Eckstein

We present a theoretical study of field-induced magnetic phases in the honeycomb Kitaev-Heisenberg model, which is believed to describe the essential physics of Mott insulators with strong spin-orbit coupling such as $A_2$IrO$_3$ and…

Strongly Correlated Electrons · Physics 2017-04-26 Gia-Wei Chern , Yuriy Sizyuk , Craig Price , Natalia B. Perkins

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

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