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Coupled cluster methods are widely regarded as the gold standard of computational quantum chemistry as they are perceived to offer the best compromise between computational cost and a high-accuracy resolution of the ground state eigenvalue…

Numerical Analysis · Mathematics 2025-12-03 Muhammad Hassan , Yvon Maday

The applicability of the factorization method is extended to the case of quantum fractional-differential Hamiltonians. In contrast with the conventional factorization, it is shown that the `factorization energy' is now a…

Mathematical Physics · Physics 2016-05-05 Fernando Olivar-Romero , Oscar Rosas-Ortiz

Among the many loopholes that might be invoked to reconcile local realism with the experimental violations of Bell's inequalities, the space-dependence of the correlation functions appears particularly relevant for its connections with the…

Quantum Physics · Physics 2025-02-14 F. Benatti , R. Floreanini , H. Narnhofer

Type-and-effect systems incorporate information about the computational effects, e.g., state mutation, probabilistic choice, or I/O, a program phrase may invoke alongside its return value. A semantics for type-and-effect systems involves a…

Programming Languages · Computer Science 2018-04-11 Ohad Kammar , Dylan McDermott

We consider models of quantum computation that involve operations performed on some fixed resourceful quantum state. Examples that fit this paradigm include magic state injection and measurement-based approaches. We introduce a framework…

Quantum Physics · Physics 2025-08-18 Benjamin D. M. Jones , Noah Linden , Paul Skrzypczyk

We introduce an approach to improve single-reference coupled cluster theory in settings where the Aufbau determinant is absent from or plays only a small role in the true wave function. Using a de-excitation operator that can be efficiently…

Chemical Physics · Physics 2024-07-03 Harrison Tuckman , Eric Neuscamman

Interest in combinatorial interpretations of mathematical entities stems from the convenience of the concrete models they provide. Finding a bijective proof of a seemingly obscure identity can reveal unsuspected significance to it. Finding…

Quantum Algebra · Mathematics 2007-05-23 Jeffrey Morton

I introduce several simplified schemes for the approximation of the self-consistency condition of the dynamical cluster approximation. The applicability of the schemes is tested numerically using the fluctuation-exchange approximation as a…

Strongly Correlated Electrons · Physics 2012-04-25 J. P. Hague

Current quantum computing hardware is restricted by the availability of only few, noisy qubits which limits the investigation of larger, more complex molecules in quantum chemistry calculations on quantum computers in the near-term. In this…

We show that all non-relativistic quantum processes, whether open or closed, are either unitary or probabilistic unitary, i.e., probabilistic combination of unitary evolutions. This means that for open quantum systems, its continuous…

Quantum Physics · Physics 2024-12-16 Le Hu , Andrew N. Jordan

Quantum periodic cluster methods for strongly correlated electron systems are reformulated and developed. The reformulation and development are based on a canonical transformation which periodizes the fermions in the cluster space. The…

Strongly Correlated Electrons · Physics 2007-05-23 Tran Minh-Tien

We consider a Trotter-type-product formula for approximating the solution of a linear abstract Cauchy problem (given by a strongly continuous semigroup), where the underlying Banach space is a product of two spaces. In contrast to the…

Functional Analysis · Mathematics 2023-07-04 Artur Stephan

The electronic states of the Hubbard model are investigated by use of the Composite Operator Method. In addition to the Hubbard operators, two other operators related with two-site composite excitations are included in the basis. Within the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Avella , F. Mancini , S. Odashima

We show that for dual-unitary kicked chains, built upon a pair of complex Hadamard matrices, correlators of strictly local, traceless operators vanish identically for sufficiently long chains. On the other hand, operators supported at pairs…

Statistical Mechanics · Physics 2020-01-07 Boris Gutkin , Petr Braun , Maram Akila , Daniel Waltner , Thomas Guhr

The distinguishable cluster approximation applied to coupled cluster doubles equations greatly improves absolute and relative energies. We apply the same approximation to the triples equations and demonstrate that it can also improve…

Chemical Physics · Physics 2019-05-01 Daniel Kats , Andreas Köhn

A new model of quantum computing has recently been proposed which, in analogy with a classical lambda-calculus, exploits quantum processes which operate on other quantum processes. One such quantum meta-operator takes N unitary…

Quantum Physics · Physics 2016-06-17 Timothy Rambo , Joseph Altepeter , Giacomo Mauro D'Ariano , Prem Kumar

The Coupled-Cluster theory is one of the most successful high precision methods used to solve the stationary Schr\"odinger equation. In this article, we address the mathematical foundation of this theory with focus on the advances made in…

Chemical Physics · Physics 2019-09-04 Andre Laestadius , Fabian M. Faulstich

We present a review of the Unitary Coupled Cluster (UCC) ansatz and related ans\"atze which are used to variationally solve the electronic structure problem on quantum computers. A brief history of coupled cluster (CC) methods is provided,…

The standard and renormalized coupled cluster methods with singles, doubles, and noniterative triples and their generalizations to excited states, based on the equation of motion coupled cluster approach, are applied to the He-4 and O-16…

Nuclear Theory · Physics 2009-11-10 K. Kowalski , D. J. Dean , M. Hjorth-Jensen , T. Papenbrock , P. Piecuch

I present a derivation of form factors in the Algebraic Cluster Model for an arbitrary number of identical clusters. The form factors correspond to representation matrix elements which are derived in closed form for the harmonic oscillator…

Nuclear Theory · Physics 2017-11-02 Roelof Bijker
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