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Many of the anomalous properties of water are amplified in the deeply supercooled region. Here we present neutron scattering measurements of the density of heavy water confined in a nanoporous silica matrix MCM-41-S (\approx15 {\AA} pore…

We develop a series of molecular dynamics computer simulations of liquid water, performed with a polarizable potential model, to calculate the spinodal line and the curve of maximum density inside the metastable supercooled region. After…

Soft Condensed Matter · Physics 2009-11-11 P. Gallo , M. Minozzi , M. Rovere

Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

Disordered Systems and Neural Networks · Physics 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

We study the statistical mechanics of supercooled liquids when the system evolves at a temperature $T$ with a field $\epsilon$ linearly coupled to its overlap with a reference configuration of the same liquid sampled at a temperature $T_0$.…

Statistical Mechanics · Physics 2022-04-05 Benjamin Guiselin , Ludovic Berthier , Gilles Tarjus

Over the last decade, an increasing body of evidence has emerged, supporting the existence of a metastable liquid-liquid critical point in supercooled water, whereby two distinct liquid phases of different densities coexist. Analysing long…

Soft Condensed Matter · Physics 2024-08-20 Cesare Malosso , Natalia Manko , Maria Grazia Izzo , Stefano Baroni , Ali Hassanali

The effect of temperature on friction and slip at the liquid-solid interface has attracted attention over the last twenty years, both numerically and experimentally. However, the role of temperature on slip close to the glass transition has…

Soft Condensed Matter · Physics 2023-02-22 Suzanne Lafon , Alexis Chennevière , Frédéric Restagno , Samy Merabia , Laurent Joly

Superfluidity---the suppression of scattering in a quantum fluid at velocities below a critical value---is one of the most striking manifestations of the collective behaviour typical of Bose-Einstein condensates. This phenomenon, akin to…

We report a dynamic light scattering study of the fluctuation modes in a thermotropic liquid crystalline mixture of monomer and dimer compounds that exhibits the twist-bend nematic ($\mathrm{N_{TB}}$) phase. The results reveal a spectrum of…

We consider theoretically the possibility of observing unusual quantum fluid behavior in liquid $^{3}$He and solutions of $^{3}$He in $^{4}$He systems confined to nano-channels. In the case of pure ballistic flow at very low temperature…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 G. Lambert , G. Gervais , W. J. Mullin

Using determinantal quantum Monte Carlo, we compute the properties of a lattice model with spin $\frac 1 2$ itinerant electrons tuned through a quantum phase transition to an Ising nematic phase. The nematic fluctuations induce…

Strongly Correlated Electrons · Physics 2017-05-24 Samuel Lederer , Yoni Schattner , Erez Berg , Steven A. Kivelson

In the supercooled regime at elevated pressure two forms of liquid water, high-density (HDL) and low-density (LDL), have been proposed to be separated by a coexistence line ending at a critical point, but a connection to ambient conditions…

Soft Condensed Matter · Physics 2011-06-27 K. T. Wikfeldt , A. Nilsson , L. G. M. Pettersson

Water, in its three phases, is ubiquitous, and the surface properties of ice is important to clarifying the process of melting, as well as to various other fields, including geophysics. As such, the subject has been studied both…

Other Condensed Matter · Physics 2019-01-16 Takahisa Mitsui , Kenichiro Aoki

The existence of a 'crossover region' in glass-forming liquids has long been considered as a general phenomenon that is as important as the glass transition. One potential origin for the crossover behavior is a liquid-to-liquid phase…

Materials Science · Physics 2015-09-14 S. Lan , M. Blodgett , K. F. Kelton , X. -L. Wang

High precision measurements of the complex sheet conductivity of superconducting Mo77Ge23 thin films have been made from 0.4 K through Tc. A sharp drop in the inverse sheet inductance, 1/L(T), is observed at a temperature, Tc, which lies…

Superconductivity · Physics 2009-10-31 Stefan J. Turneaure , Thomas R. Lemberger , John M. Graybeal

We investigate the superfluid phase transition in a gas of Fermi atoms loaded on a three-dimensional optical lattice. When the lattice potential is strong, this system can be well described by an attractive Hubbard model. In this model, we…

Materials Science · Physics 2008-03-17 H. Tamaki , Y. Ohashi , K. Miyake

The application of amorphous chalcogenide alloys as data-storage media relies on their ability to undergo an extremely fast (10-100 ns) crystallisation once heated at sufficiently high temperature. However, the peculiar features that make…

Disordered Systems and Neural Networks · Physics 2015-06-05 Gabriele C. Sosso , Joerg Behler , Marco Bernasconi

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

Materials Science · Physics 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

The liquid-liquid critical point scenario of water hypothesizes the existence of two metastable liquid phases---low-density liquid (LDL) and high-density liquid (HDL)---deep within the supercooled region. The hypothesis originates from…

We investigate the properties of water along the liquid/vapor coexistence line in the supercooled regime down to the no-man's land. Extensive molecular dynamics simulations of the TIP4P/2005 liquid/vapor interface in the range 198 -- 348 K…

Soft Condensed Matter · Physics 2023-02-15 Alexander Gorfer , Christoph Dellago , Marcello Sega

Local environment of fluorescent dyes could strongly affect emission dynamics of the latter. In particular, both signal intensities and emission lifetimes are highly sensitive to solvent temperatures. Here, temperature-dependent behavior…

Soft Condensed Matter · Physics 2017-09-13 Ivan Shishkin , Tmiron Alon , Ronen Dagan , Pavel Ginzburg